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Intrinsic Pinning in Magnetic Iron-Based Superconductors; a Route to High Critical Current Conductors at High Magnetic Fields

Lead Research Organisation: UNIVERSITY OF BATH
Department Name: Physics

Abstract

The discovery of superconductivity by Kamerlingh Onnes in 1911 was one of the most remarkable discoveries of the 20th century. A superconductor is a material that can carry large electrical currents without any resistance, that is without losing any energy. Although superconductors offered clear benefits for the transmission of electrical power, many problems needed to be solved before they could find mainstream applications. The first discovered superconductors had to be cooled to extremely low temperatures, close to absolute zero on the Kelvin scale, requiring the development of suitable cryogenic cooling systems which themselves had significant energy losses. Since the discovery of copper oxide-based superconductors in 1986 and iron-based superconductors in 2006 with much higher operation temperatures, this problem has been largely solved. However, we now know that only certain types of superconducting materials, so-called 'type II' ones, are capable of operation at the very high magnetic fields needed for medical magnetic resonance imaging or magnetic confinement in fusion reactors. However, these 'type II' materials are only able to achieve this by allowing tiny tubes of magnetic field called vortices to enter them which start to generate heat (and lose energy) if they are driven into motion by large flowing supercurrents. Fortunately nature has found a solution to this problem, and vortices can become trapped at defects present in the material preventing them from moving and losing energy. Developing high current superconducting wires therefore requires introducing as many defects into the material as possible without significantly degrading other useful superconducting properties. Even then the current carrying capacity of superconductors at very high magnetic fields (when they become flooded with many vortices) can still be too low for intended applications. In this project we will investigate new types of iron-based superconductors that have recently been discovered in which magnetism and superconductivity coexist. This behaviour is very unusual as magnetism and superconductivity are normally antagonistic phenomena; they involve opposite arrangements of the quantum spins of electrons. Each electron can be visualised as having a tiny compass 'needle' (the spin) attached to it; in ferromagnets all the 'needles' point in the same direction, while in conventional superconductors the electrons form pairs in which the 'needles' point in opposite directions. Remarkably, in these new iron-based materials the presence of ferromagnetism does not destroy superconductivity, and a patchwork of regions called domains where the magnetic 'needles' point in different directions coexists with the superconducting state. These magnetic domains and the boundaries between them represent a new type of defect that can strongly trap vortices, leading to enhanced current carrying capacities, even in very high magnetic fields.
In this project we will bring together a team of experts with a diverse range of skills that can grow, pattern, measure and undertake theoretical studies on magnetic iron-based superconductors. We will carefully investigate how the patchwork of magnetic domains present can trap superconducting vortices and control their dynamic properties and will develop advanced theoretical models to understand our results. Once the conditions have been established for achieving the highest current densities at high magnetic fields we will apply them to iron-based superconducting thin films grown by our partner in Karlsruhe (Germany) with the ultimate goal of realising high performance commercial wires that can be produced by very low-cost methods. Although the main motivation for this project is to develop new materials that meet the requirements for key applications, we will also generate a lot of new scientific knowledge that will be of great value to the wider research community working on superconducting materials.

Publications

10 25 50
 
Description New insights have been gained into the complex physics at play in ferromagnetic superconductors when a uniaxial ferromagnetic state orders well below the critical temperature, T_c, of a type II iron-based superconductor. We have demonstrated how the underlying magnetic structure controls the superconducting vortex dynamics in applied magnetic fields. Just below the ferromagnetic ordering temperature, T_FM, we have observed a pronounced peak in the creep activation energy due to the formation of vortex polarons for which we have developed a theoretical description. In contrast, we have been able to link strong magnetic irreversibility at low temperatures to a critical current governed by giant flux creep over an activation barrier for vortex antivortex annihilation near domain walls.
Exploitation Route Our work suggests new routes for the magnetic enhancement of vortex pinning in superconducting tapes and cables. It could potentially have important applications in high-current conductors for operation at very high magnetic fields.
Sectors Aerospace

Defence and Marine

Energy

Environment

Healthcare

Transport

 
Title Dataset for "Breakdown of the critical state in the ferromagnetic superconductor EuFe2(As1-xPx)2" 
Description Datasets underpinning five of the six Figures and four Supplementary Figures in "Breakdown of the critical state in the ferromagnetic superconductor EuFe2(As1-xPx)2" in Superconductor Science and Technology. The primary data (e.g. as in Figure 2) are low temperature Hall magnetometry measurements made at the University of Bath. The manuscript describes in detail how these measurements are made. There is further, secondary data (e.g. penetration field Hp) that are derived from analysis of these primary measurements. 
Type Of Material Database/Collection of data 
Year Produced 2025 
Provided To Others? Yes  
URL https://researchdata.bath.ac.uk/id/eprint/1597
 
Title Dataset for "Magnetically-controlled Vortex Dynamics in a Ferromagnetic Superconductor" 
Description Datasets underpinning the five Figures and six Supplementary Figures for "Magnetically-controlled Vortex Dynamics in a Ferromagnetic Superconductor" in Communications Materials. The primary data are a mixture of low temperature magnetisation data, taken using a SQUID magnetometer taken at the University of Bristol, and low temperature magnetic force microscopy (MFM) scan data taken at the University of Basel. Additionally, there are data derived from analysis of the magnetisation data, e.g. critical current, coercive field, as well as the results of magnetic relaxation measurements, i.e. Ueff. In addition to the MFM scan data are line profiles taken through regions of these scans. The supplementary data include further magnetisation data, as well as examples of magnetic relaxation data. Additionally, there is a further example of a line profile taken from MFM scan data, along with corresponding fitted data. 
Type Of Material Database/Collection of data 
Year Produced 2025 
Provided To Others? Yes  
URL https://researchdata.bath.ac.uk/id/eprint/1485
 
Description Argonne National Laboratories, supply of antiferromagnetic RbEuFe4As4 superconducting single crystals 
Organisation Argonne National Laboratory
Department Physics Division
Country United States 
Sector Academic/University 
PI Contribution Argonne National Laboratories are providing us with high quality RbEuFe4As4 single crystals for our investigations of the coexistence of superconductivity and helical antiferromagnetism. Our Bath group will be performing, magnetometry, magnetic relaxation and Hall array magnetometry to understand the vortex dynamics and critical state. We will also be imaging vortex stuctures by scanning Hall microscopy.
Collaborator Contribution Argonne National Laboratories are growing high quality RbEuFe4As4 single crystals which exhibit the coexistence of superconductivity and helical antiferromagnetism. They are providing these to us for our own physical studies of vortex dynamics and the critical state in this remarkable material.
Impact Observing the Suppression of Superconductivity in RbEuFe4As4 by Correlated Magnetic Fluctuations, D. Collomb, S. J. Bending, A. E. Koshelev, M. P. Smylie, L. S. Farrar, J. K. Bao, D. Y. Chung, M. G. Kanatzidis, W. K. Kwok, U. Welp, Physical Review Letters 26, 157001 (2021).
Start Year 2019
 
Description Karlesruhe Instutute of Technology; Supply of Ferromagnetic Fe-based superconducting tapes 
Organisation Karlsruhe Institute of Technology
Country Germany 
Sector Academic/University 
PI Contribution Karlsruhe Institute of Technology are providing us with EuFe2(As1-xPx)2 thin film tapes for our investigations of the coexistence of superconductivity and ferromagnetism. Our Bath group will be performing, critical current density measurements, magnetometry, magnetic relaxation and Hall array magnetometry to understand the vortex dynamics and critical state. We will also be imaging vortex structures by scanning Hall microscopy.
Collaborator Contribution Karlsruhe Institute of Technology are growing high quality EuFe2(As1-xPx)2 thin film tapes which exhibit the coexistence of superconductivity and ferromagnetism. They are providing these to us for our own physical studies of the critical current density, vortex dynamics and the critical state in this remarkable material.
Impact None up to now.
Start Year 2023
 
Description University of Antwerp 
Organisation Antwerp University Hospital
Department University Hospital Antwerp
Country Belgium 
Sector Hospitals 
PI Contribution Performed experiments in mesoscopic superconductivity and sa,ples exhibiting coexisting superconductivity and magnetism.
Collaborator Contribution Milorad Milosevic performed Ginzburg-Landau and analytic calculations to understand our experiments.
Impact Spontaneous symmetry breaking in vortex systems with two repulsive lengthscales, P.J. Curran, W.M. Desoky, M.V. Milosevic, A. Chaves, J.-B. Laloe, J.S. Moodera, S.J. Bending, Scientific Reports 5, 15569 (2015). Rayleigh instability of confined vortex droplets in critical superconductors, I. Lukyanchuk, V. M. Vinokur, A. Rydh, R. Xie, M. V. Miloševic, U. Welp, M. Zach, Z. L. Xiao, G. W. Crabtree, S. J. Bending, F. M. Peeters & W. K. Kwok, Nature Physics 11, 21 (2015).
Start Year 2006
 
Description University of Tokyo; Supply of EuFe2(As1-xPx)2 Superconducting Single Crystals 
Organisation University of Tokyo
Country Japan 
Sector Academic/University 
PI Contribution The University of Tokyo is providing us with high quality EuFe2(As1-xPx)2 single crystals for our investigations of the coexistence of superconductivity and ferromagnetism. Our Bath group will be performing, magnetometry, magnetic relaxation and Hall array magnetometry to understand the vortex dynamics and critical state. We will also be imaging vortex structures by scanning Hall microscopy.
Collaborator Contribution The University of Tokyo is growing high quality EuFe2(As1-xPx)2 single crystals which exhibit the coexistence of superconductivity and ferromagnetism. They are providing these to us for our own physical studies of vortex dynamics and the critical state in this remarkable material.
Impact None published yet
Start Year 2023