Multi-scale Exploration of MultiPhase Physics In FlowS (MEMPHIS)

Lead Research Organisation: Imperial College London
Department Name: Chemical Engineering

Abstract

This project is an opportunity to harness the synergy between world-leading scientists from four prestigious institutions to create the next generation modelling tools for complex multiphase flows. These flows are central to micro-fluidics, virtually every processing and manufacturing technology, oil-and-gas and nuclear applications, and biomedical applications such as lithotripsy and laser-surgery cavitation. The ability to predict the behaviour of multiphase flows reliably will address a major challenge of tremendous economic, scientific, and societal benefit to the UK. The Programme will achieve this goal by developing a single modelling framework that establishes, for the first time, a transparent linkage between input (models and/or data) and prediction; this will allow systematic error-source identification, and, therefore, directed, optimal, model-driven experimentation, to maximise prediction accuracy. The framework will also feature optimal selection of massively-parallelisable numerical methods, capable of running efficiently on 10^5-10^6 core supercomputers, optimally-adaptive, three-dimensional resolution, and the most sophisticated multi-scale physical models. This framework will offer unprecedented resolution of multi-scale, multiphase phenomena, minimising the reliance on correlations and empiricism. The investigators' synergy, and their long-standing industrial collaborations, will ensure that this Programme will result in a paradigm-shift in multiphase flow research worldwide. We will demonstrate our capabilities in two areas of strategic importance to the UK: by providing insights into novel manufacturing processes, and reliable prediction of multiphase flow regime transitions in the oil-and-gas industry. Our framework will be sufficiently general to address a number of other industrial and environmental global challenges, which we detail herein.

Planned Impact

Our Programme will lead to the resolution of a number of fundamental open problems in multiphase flows leading to the development of validated simulation tools for the academic and industrial community, with impact on the UK economy, people and society. Our transformative research will impact:
- The FMCG and fine chemicals/catalysis sectors, via the ability to design novel flow processes to produce controlled, multiphase structures.
- The oil-and-gas sector, where it will lead to validated, powerful numerical predictive tools employed for flow assurance by industry, supplanting existing far less reliable ones.
- The nuclear industry, where our models and simulation tools will support the development of intensified evaporation and extractive separation processes.
We will also impact a number of other applications, e.g. atomisation and fuel release in engines (automotive), lava flows, ocean and tsunami modelling (geophysics).
We will impact the non-academic community through a number of industrial partners:
- Chevron: simulation of gas-liquid flow regime transitions in pipes of varying diameter.
- Johnson Matthey: multi-scale simulation of the blending of miscible and immiscible complex fluids in the manufacture of catalyst slurries and washcoats.
- Procter & Gamble: production of bespoke multiple-emulsions for structured-product manufacturing; simulation of downwards-annular flow reactors for personal care products manufacturing.
- CD-Adapco: rational development of state-of-the-art sub-grid models and closures, leading to significant improvement of CFD tools.
- AspenTech: the need to improve the predictive capabilities of pressure drop and heat transfer methods for liquid-liquid flows.
We will engage with our partners through a variety of ways:
- Our Steering Committee (SC) will advise on the results that can maximise industrial impact;
- Our existing consortium of industrial partners at Imperial (oil-and-gas) and Birmingham (FMCG, pharmaceuticals, fine chemicals) will be integrated to provide a platform for dissemination, identification of opportunities for technical solutions to problems, and cross-fertilization of ideas;
- CIKTN, special interest groups, ERC, EU FP networks will provide other dissemination platforms and mechanisms for technological transfer;
- Twice-yearly meetings with the most prominent scientists, engineers and industrialists in multiphase flow, including aerospace and automotive industries, civil engineering and geophysics; major symposia half-way through the Programme and in its final year to present our major findings, advertised as widely as possible.
- We will run training programmes and encourage secondments and/or extended visits by industrialists to our research groups, and ensure that our researchers spend secondments in our partner companies;
- Generic, commercially insensitive, software developed as part of the Programme will be released as open-source;
- An active Programme Manager will drive commercialisation, manage all secondments, and our dedicated website.
We will transfer technology through early release of research software and/or experimental techniques; the secondment of researchers and/or commercialisation. We will also disseminate our findings widely through papers in prestigious journals, presentations at national and international conferences, a seminar and webinar series to which the most prominent scientist, , engineers and industrialists in the area will be invited (including 'adjacent' disciplines), active national and international collaborations.
Delivery of this research programme will deliver societal impact via:
- Sustainable processing due to superior equipment design, reduced process scale, downtime and wastage;
- Public and young people engagement activities;
- Bespoke consumer goods with advanced properties.

Publications

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Che Z (2017) Impact of Droplets on Liquid Films in the Presence of Surfactant. in Langmuir : the ACS journal of surfaces and colloids

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Kovalchuk N (2018) Study of drop coalescence and mixing in microchannel using Ghost Particle Velocimetry in Chemical Engineering Research and Design

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Kovalchuk N (2018) Effect of soluble surfactant on regime transitions at drop formation in Colloids and Surfaces A: Physicochemical and Engineering Aspects

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Mohammed S (2018) Churn flow in high viscosity oils and large diameter columns in International Journal of Multiphase Flow

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Kovalchuk N (2018) Effect of surfactant on emulsification in microchannels in Chemical Engineering Science

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Kovalchuk NM (2018) Effect of soluble surfactants on pinch-off of moderately viscous drops and satellite size. in Journal of colloid and interface science

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Salinas P (2018) A robust mesh optimisation method for multiphase porous media flows in Computational Geosciences

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Xiao D (2019) A domain decomposition method for the non-intrusive reduced order modelling of fluid flow in Computer Methods in Applied Mechanics and Engineering

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Kovalchuk NM (2019) Mass Transfer Accompanying Coalescence of Surfactant-Laden and Surfactant-Free Drop in a Microfluidic Channel. in Langmuir : the ACS journal of surfaces and colloids

 
Description The key findings include: 3D unstructured, adaptive mesh-based software for solving multiphase flows; interface-tracking software, which is particularly adept at solving interfacial problems - massively parallelised and tested on 130,000 CPUs with very good scaling; codes that account for the presence of surfactants, non-Newtonian rheology, heat transfer, and phase change; deep, and exploitable insights into near-interface and interfacial behaviour in the presence of surfactants above and below the CMC - obtained experimentally; two-colour PIV studies for detailed measurements of the two phases in two-phase flows; detailed and exploitable understanding of interfacial phenomena in air-water channel, and annular flows, with a focus on disturbance wave dynamics, and droplet entrainment as well as bubble entrapment; detailed, and exploitable understanding of flow patterns in microfluidic devices for Newtonian and non-Newtonian fluids in devices featuring complex geometry; detailed and exploitable understanding of drop impact on miscible and immiscicble interfaces, accounding for the presence of surfactants as well as viscosity ratio.
Exploitation Route The findings from MEMPHIS were disseminated via 87 journal articles and >100 presentations at international conferences. They were also communicated to our industrial partners through presentations at steering committee meetings, as well as invited talks, and technology is currently being transferred via secondments, and fortnightly telecons in which the MEMPHIS code, Blue, is used to provide predictions for complex multiphase flows arising in industrial case studies. The code is being trialled in this manner with P&G and BP in 2018, and it is expected that licences will be sold in 2019 following the creation of a spinout company at Imperial College London.
Sectors Chemicals,Education,Electronics,Energy

 
Description Work from the MEMPHIS Programme has been disseminated widely in the form of 48 journal articles, 6 conference papers, and over 100 presentations at 34 national and international conferences; the latter include APS/DFD, AIChE, ChemEngDayUK, ICMF2016, Bubble & Drop 2017, ISMIP9, Droplets 2015, Microfluidics 2014, DEFI 2016, IMRET 2014, BIFD ESPCI 2016, 9th HEFAT. The talks include keynotes at IPHT2016, ICMF2016, ChemEngDayUK2017, and CFD2017. We have also disseminated our results via the MEMPHIS website (www.memphis-multiphase.org) and Twitter (@memphisProgram which has 247 followers currently). Our work has also been the subject of several outreach activities, e.g. at the Imperial May Festivals, UCL ChemE Summer Challenge, and SET for Britain in House of Parliament. Our research has been featured on the cover of Soft Matter, Chem. Eng. Sci., and Langmuir, and in The Chemical Engineer, and has won First Place at a National Photo Competition organised by the EPSRC. MEMPHIS has also provided a platform for leverage of research projects including the £1M EMFormR InnovateUK project (Birmingham - Unilever, Johnson Matthey), the projects at Imperial funded by Cameron, Petronas, Shell, and TOTAL, EPSRC Knowledge Transfer Scheme, and Impact Acceleration Account, and the Royal Academy of Engineering (through a Research Chair for OKM) worth over £1.7M, the £4.5M EPSRC CDT in Fluid Dynamics at Imperial, a £3M EPSRC project at UCL on nuclear waste management and liquid-liquid extractions (PACIFIC), a £1.9M EPSRC Future Formulations project at UCL on manufacturing of complex products (CORAL), an InnovateUK project at Nottingham worth £250k on multistage ejectors for flare gas recovery (involving separation of condensate from gas streams). Interest in the MEMPHIS work by P&G has also leveraged 6 months of funding to extend the work at UB, which has been matched by UB due to its strategic importance to create a 12-month extension to MEMPHIS. Transfer of MEMPHIS knowledge/technology was effected through a secondment at P&G (Feb.-August 2017) for Dr Lyes Kahouadji (ICL), and an inward secondment for Dr Andre Nicolle from BP at ICL. The interface-tracking code is also being commercialised at ICL, via a spinoff company currently being formed through IC Innovations.
First Year Of Impact 2013
Sector Aerospace, Defence and Marine,Agriculture, Food and Drink,Chemicals,Digital/Communication/Information Technologies (including Software),Education,Energy,Environment,Healthcare,Manufacturing, including Industrial Biotechology
Impact Types Societal,Economic

 
Description BP support for MEMPHIS Programme Grant
Amount $50,000 (USD)
Organisation BP (British Petroleum) 
Sector Private
Country United Kingdom
Start 01/2013 
End 01/2018
 
Description Detailed Understanding and Development of Wax Control Chemical
Amount £587,219 (GBP)
Organisation Petronas 
Sector Private
Country Malaysia
Start 10/2014 
End 10/2017
 
Description EPSRC Impact Acceleration Account 2012-2015
Amount £56,386 (GBP)
Funding ID EP/K503733/1 
Organisation Engineering and Physical Sciences Research Council (EPSRC) 
Sector Public
Country United Kingdom
Start 07/2015 
End 06/2016
 
Description Industrial grant
Amount £50,000 (GBP)
Organisation Procter & Gamble 
Sector Private
Country United States
Start 01/2018 
End 12/2018
 
Description Liquid-liquid horizontal flows
Amount £170,000 (GBP)
Organisation BP (British Petroleum) 
Sector Private
Country United Kingdom
Start 11/2013 
End 10/2016
 
Description Liquid-liquid mixers
Amount £80,000 (GBP)
Organisation Cameron International Corporation 
Sector Private
Country United States
Start 10/2014 
End 10/2017
 
Description Proof-of-concept funding
Amount £41,000 (GBP)
Organisation Imperial Innovations 
Sector Private
Country United Kingdom
Start 01/2018 
End 12/2018
 
Description Responsive mode (Fluids CDT)
Amount £4,280,000 (GBP)
Funding ID EP/L016230/1 
Organisation Engineering and Physical Sciences Research Council (EPSRC) 
Sector Public
Country United Kingdom
Start 04/2014 
End 04/2022
 
Description Responsive mode (Severe accidents modelling)
Amount £244,071 (GBP)
Funding ID EP/M012794/1 
Organisation Engineering and Physical Sciences Research Council (EPSRC) 
Sector Public
Country United Kingdom
Start 11/2014 
End 03/2017
 
Description Sand particle size management
Amount £589,806 (GBP)
Organisation Petronas 
Sector Private
Country Malaysia
Start 01/2015 
End 01/2018
 
Description Simulation of shear in grease kettles
Amount £122,000 (GBP)
Organisation Shell Global Solutions International BV 
Department Shell Global Solutions UK
Sector Private
Country Netherlands
Start 01/2015 
End 01/2016
 
Description Support for MEMPHIS Programme Grant (P and G)
Amount £100,000 (GBP)
Organisation Procter & Gamble 
Sector Private
Country United States
Start 01/2013 
End 01/2018
 
Description Surfactant effects on vertical gas-liquid flows
Amount £146,000 (GBP)
Organisation Shell Global Solutions International BV 
Department Shell Global Solutions UK
Sector Private
Country Netherlands
Start 09/2014 
End 09/2016
 
Title TMF database 
Description Database for multiphase flow data (e.g. flow regimes and their transitions for various flows as a function of system parameters). The data are collected as part of the TMF consortium, which compromises 14 oil-and-gas companies and design and software houses, led by Omar Matar. 
Type Of Material Database/Collection of data 
Provided To Others? Yes  
Impact TMF sponsors have access to the database and they have used it to improve their understanding of multiphase flows, which improves their design capabilities. The software houses that sponsor TMF use the data to validate the predictions of their codes. 
 
Description Strategic partnership with Procter and Gamble 
Organisation Procter & Gamble
Country United States 
Sector Private 
PI Contribution Engaged with P&G researchers to provide solutions to problems in the area of multiphase flows.
Collaborator Contribution Engaged with the research group to provide a constant source of good problems to work on, secondment opportunities for our researchers, and cash contribution.
Impact Procter and Gamble have provided £100000 cash contribution which was instrumental in our winning an EPSRC Programme Grant.
Start Year 2012
 
Description Imperial Festival 
Form Of Engagement Activity Participation in an open day or visit at my research institution
Part Of Official Scheme? No
Geographic Reach Regional
Primary Audience Public/other audiences
Results and Impact Our demonstrations of multiphase flows generated lots of excitement among the attendees (from the public).

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Year(s) Of Engagement Activity 2011,2014
 
Description MEMPHIS Showcase 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Industry/Business
Results and Impact The Showcase was held at Imperial College London on the 14th and 15th September 2017 and featured presentations by industrialists (BP and P&G), and researchers from the MEMPHIS partner universities: Imperial, Birmingham, Nottingham, and UCL. There was also an opportunity to engage in live demonstrations and gain hands-on experience/trial the MEMPHIS modelling tools developed. There was participation from BP, Johtnson Matthey, P&G, CPI, TOTAL, Siemens, and delegates from Cardiff and Newcastle universities, and Louisiana State University. There were approximately 60 delegates.
Year(s) Of Engagement Activity 2017
URL http://www.memphis-multiphase.org/showcase-event/
 
Description Next generation predictive tools for multiphase flows (BHRG) 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Type Of Presentation keynote/invited speaker
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Presented the next-generation predictive tools produced by the MEMPHIS Programme Grant to industrialists in the oil-and-gas sector at the BHRG conference in Cannes, June 2013. There was a lot of discussion following the presentation about the potential use of the MEMPHIS codes in providing solutions to flow assurance problems in the oil-and-gas industry.

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Year(s) Of Engagement Activity 2013
 
Description Rising bubbles in non-Newtonian fluids (Wales) 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Other academic audiences (collaborators, peers etc.)
Results and Impact Invited to present at the Wales Institute of Non-Newtonian Fluid Mechanics meeting in honour of Ken Walters' 80th birthday, at Lake Vyrnwy, Wales, April 14 - 16, 2014. The talk generated interest in the modelling rising bubbles in non-Newtonian fluids.

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Year(s) Of Engagement Activity 2014
 
Description TMF meetings 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Meetings of the Transient Multiphase Flow consortium, led by Omar Matar, are instrumental in facilitating tech. transfer. There are 14 companies within TMF (e.g. BP, Shell, Chevron, Petrobras, Statoil, TOTAL, Schlumberger, ENI, Cameron, etc.) and we have semi-annual sponsors' meetings in which sponsored students present their findings.

Continued funding of our multiphase flow activities.
Year(s) Of Engagement Activity Pre-2006,2006,2007,2008,2009,2010,2011,2012,2013,2014
 
Description Talk on MEMPHIS (Daresbury lab) 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Professional Practitioners
Results and Impact Gave a presentation on the capabilities being developed as part of the MEMPHIS Programme Grant. The talk generated considerable interest and led to a very useful discussion with colleagues from industry and academia.

After the talk, I was approached by company representatives for potential collaborations.
Year(s) Of Engagement Activity 2013
 
Description The next generation of predictive tools for multiphase flows (AICHE) 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Type Of Presentation keynote/invited speaker
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Presentation on the MEMPHIS capabilities in terms of modelling and simulation presented as an invited keynote at
the AIChE Spring Meeting, March 31 - April 3, New Orleans. In the audience were numerous practitioners and some academics. The talk stimulated a lengthy discussion and generated tremendous interest afterwards. There was a subsequent invitation to visit Louisiana State University to present a similar talk to a consortium of companies.

There was a subsequent invitation to visit Louisiana State University to present a similar talk to a consortium of companies.
Year(s) Of Engagement Activity 2014
 
Description The next generation of predictive tools for multiphase flows (LSU) 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach Regional
Primary Audience Professional Practitioners
Results and Impact Invited seminar presented as part of the Enabling Process Innovation through Computation seminar series, Louisiana State College of Engineering, Centre for Computation and Technology, April 4, 2014. This followed a talk given by OKM at the AICHE. The talk at LSU generated a lot of discussion on innovation through simulations and the use of MEMPHIS Programme Grant tools to do that. There was a lot of interest in this from the numerous academics and company reps in the audience.

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Year(s) Of Engagement Activity 2014