Solid State Superatoms

Lead Research Organisation: Durham University
Department Name: Physics

Abstract

The modern digital world relies on classical two-level systems - binary bits. A major theme of current physics research is the development of their quantum equivalent "qubits" - isolated two-level quantum systems, for applications in computing, sensing, measurement and communication. A logical quantum bit may be encoded using the physical states of an ensemble of many individual atoms. A powerful way to carry out such a collective encoding is to exploit highly excited electronic states, known as Rydberg states that have strong long-range interactions with neighbouring atoms. So far, this method has been demonstrated in a laser-cooled atomic gas, but not in the solid state.

We propose to use atom-like electronic states known as excitons, in a semiconducting signal. Excitons couple to light and can be excited to a Rydberg state, where their wavefunction can encapsulate billions of lattice sites. Using methods from solid state physics (strain engineering) and atomic physics (microwave control), we aim to isolate collective solid state two-level systems (superatoms), and prove their existence using the quantum properties of the light they emit. Finally we plan to exploit the translational symmetry of the bulk crystal environment to create tailored arrays of superatoms.

Planned Impact

Short term: The primary beneficiary of the proposed work is the UK Quantum technology community (scientists, engineers and companies), in the following ways:
-People: The project will directly train two PDRAs in the cutting-edge skills needed in the quantum technology arena, and provide a training opportunity for at least two graduate students, as well as undergraduates.
-Knowledge: We open up a new research direction in the solid state that exploits atom-like highly excited states, with applications that include quantum optics and quantum interfaces. The proposal combines methods from solid state and atomic physics, with impact in both. We plan to use this project link these communities more closely.

Medium and long term: Economic impact could result in the medium to long term, through applications of the proposed research to sources of non-classical light and interfaces to superconducting quantum circuits such as those used in the first commercial quantum computer (D-Wave).

Publications

10 25 50

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Gallagher L (2022) Microwave-optical coupling via Rydberg excitons in cuprous oxide in Physical Review Research

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Ogden T (2019) Quasisimultons in Thermal Atomic Vapors in Physical Review Letters

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Adams C (2020) Rydberg atom quantum technologies in Journal of Physics B: Atomic, Molecular and Optical Physics

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Lynch S (2021) Rydberg excitons in synthetic cuprous oxide Cu 2 O in Physical Review Materials

 
Description We have discovered three things so far:
1. Electrons and holes can bind together in a semiconductor to form excitons, which are like hydrogen atoms. We have shown that just like real atoms, these excitons can couple strongly to microwave radiation that drives transitions between the excitonic energy levels. This could be used to couple light to microwave fields inside quantum computers.
2. Until now, naturally occurring crystals of the material we use (cuprous oxide) have performed better than synthetic ones. By measuring a wide range of parameters we have shown this is due to copper vacancies in the synthetic material, and we have shown that we can reduce their concentration using annealling.
3. Using a spectroscopy technique known as second harmonic generation, we were able to eliminate the background absorption of light due to phonons from our signals, potentially increasing our chances of seeing quantum light.
Exploitation Route In the longer term this work could be developed to couple together superconducting microwave circuits and light. DSTL may also choose to investigate possible applications
Sectors Digital/Communication/Information Technologies (including Software)

URL https://www.dur.ac.uk/qlm/research/rydbergsystems/
 
Description CASE studentship with DSTL 
Organisation Defence Science & Technology Laboratory (DSTL)
Country United Kingdom 
Sector Public 
PI Contribution Working with DSTL exploring microwave sensing with excitons in cuprous oxide
Collaborator Contribution Partner for industrial CASE - stipend enhancement and hosting of placement
Impact This award helped support the two publications produced from the Solid State Superatoms grant, by part-funding the PhD of Liam Gallagher. These are https://journals.aps.org/prmaterials/abstract/10.1103/PhysRevMaterials.5.084602 and https://journals.aps.org/prresearch/abstract/10.1103/PhysRevResearch.4.013031
Start Year 2017
 
Description Celebrate Science 2019 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach Regional
Primary Audience Public/other audiences
Results and Impact Celebrate Science is an annual science festival aimed at school children held in Durham in the October half term. It is well established, and attended by >1000 people over typically four days.
Staff employed on this project contributed to an activity on optics (polarization) and spectroscopy
Year(s) Of Engagement Activity 2019
URL https://www.dur.ac.uk/celebrate.science/