Non-Ergodic Quantum Manipulation

Lead Research Organisation: University College London
Department Name: London Centre for Nanotechnology

Abstract

The subject of electron transport when states are localized by disorder has been an important topic in physics for a considerable time. It was first realized in 2006 that a closed quantum system in which there is both disorder and many body interactions shows a completely new regime of behaviour termed Many Body Localization, MBL. This regime is characterised by a breakdown of equilibrium statistical mechanics, it predicts a zero conductance state at a finite temperature, entanglement can spread although there is a lack of thermalisation due to the breakdown of ergodicity expressed as a violation of the Eigenstate Thermalisation Hypothesis, ETH. Ergodicity is assumed in many areas of condensed matter science, namely that a sub-system of the whole is typical of the whole and that the behaviour averaged over time is identical to that averaged over space. Consequently the fact that it does not hold in this situation allows new phenomena as does the lack of equilibration due to the ETH no longer holding. Possible new states can be formed by the application of high frequencies to MBL and these will be investigated in the project.
To date there has been no sustained experimental investigation of these predictions in condensed matter systems although there is considerable activity using cold atoms which naturally form a closed quantum system. Enormous theoretical interest has been expressed in the hundreds of papers published on the topic.
It is in the area of condensed matter that this new state of matter would have a major impact if realised - which is the purpose of the project. We will comprehensively investigate this regime of behaviour using semiconductor technology and the fabrication techniques used in investigating mesoscopic devices and semiconductor nanostructures.
By fabricating free standing nanostructures we will ensure a closed system by drastically reducing the coupling to the phonons which act as a heat bath. The temperature of measurements will be down the milliKelvin region and the length scale of the disorder will be varied as will other parameters such as dimensionality. Electrical and thermal techniques will be utilised as probes of the MBL state.
In addition to the importance for basic physics this work will be extremely significant in quantum information and topological physics as this new state provides a means of quantum protection not presently available.

Planned Impact

The following areas will benefit from the project which has an impact in different fields.
Knowledge
The exploration of non-ergodicity and its consequences in a condensed matter system is a scientific advance on existing knowledge. The breakdown of the Eigenstate Thermalization Hypothesis has not been observed or investigated in condensed matter systems before and is confined to the area of Cold Atoms. This grant combines theory and experiment to make rapid progress which should stimulate other groups both experimental and theoretical to enter this field. As the results will be complementary to the work in Cold Atoms we suggest that a new field of Non-Ergodic Physics will emerge which transcends the division between the atomic work and solid state. The net effect is a rapid increase in knowledge with possible applications in Quantum Technologies.
The fabrication of multi-layer free standing devices and growth techniques for compensated layers all involve advances in techniques which may be of interest to others involved in both physics and material science. As an example, cantilever structures are used as sensitive mass spectrometers and have applications as molecular detectors in the biological/medical area.
Skills
People employed on the project will learn new skills, particularly as they will spend time in each of the collaborating departments, ie low temperature techniques, lithography and semiconductor fabrication. The system we will implement also means that RAs will acquire management and organisational skills, the collaboration with distinguished visitors means that their scientific understanding will increase. The people pipeline will be augmented by our training Ph.D students and offering projects to those in CDTs.
Economy
Success in our project leading to advances in Quantum Technologies will bring a benefit in wealth creation as quantum advances will benefit data processing, security, large data base searching and calculations. These advantages have resulted in the EPSRC quantum initiative. Success in condensed matter physics in the past succeeded in bringing inward investment as Sharp, Hitachi and Toshiba set up laboratories in the UK, one of us, MP, was involved in the Toshiba case. Future success may well bring in more inward investment and our experience will assist in making this a success, we also have experience in making the presentations required. In the consortium we have established 4 companies and have experience in negotiations with venture capital organisations, if the results of the project are sufficiently encouraging we will investigate new company formation. In addition to the benefits of success in quantum information the project may generate spin-off advances in other areas associated with the technology we use, such as spintronics or applications involving thin films, thus there will be advantages to a range of products and procedures.
Society
This project has considerable societal benefits, a major advance in quantum information would benefit healthcare by enhancing more rapid design of new molecules, this would then benefit quality of life. International development will benefit as explained in the letter of support from our collaborator Dr Mark Blumenthal, Lecturer in Physics Capetown University. There are few opportunities for Ph.D students in South Africa to work with physics groups in the developed world, working at the frontiers of physics, and those in Capetown have already benefited from our collaboration and discussions which will be the case in future. Success in a project which is oriented towards basic research, but has benefits in inward investment and new products/technologies, will impact on policy makers and help to convince them to defend the science budget and continue to increase it.

Publications

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Description The work is in very early stages and we are preparing samples for measurements, we have found that free standing cantilever structures behave differently to normal structures. This finding was unexpected and we are in the process of investigating it further.
Unfortunately due to the impact of Covid on the progress of the work little progress has been made on the above although we have found that the electron-electron interaction effects on Localization were very pronounced with Graphene. this is being investigated further.
Exploitation Route The technology of sample fabrication may be useful to other research groups. It will be published in due course. Interesting data has been found on the effects of the interaction on localization which are being pursued.
Sectors Digital/Communication/Information Technologies (including Software),Electronics

 
Title Data supporting "Cooling Low-Dimensional Electron Systems into the Microkelvin Regime" article 
Description This dataset combines all the supporting data under single DOI. The individual files contain:Te_vs_dotQe.dat - modelled electron temperature as a function of heat leak to the electrons.Rsquare_vs_T.dat - temperature dependence of the 2DEG sheet resistance before and after illumination..R_NT-Iminus_vs_T.dat - temperature dependence of the resistance between NT and I- ohmic contacts before and after illumination.dQnt_dTnt.dat - thermal conductance between 2DEG NT and 3He bath before and after illumination.dQnt_dTnt.dat - non-local thermal conductance, describing the response of 2DEG NT to heating the 2DEG before and after illumination.dotQe_vs_t.dat - time dependence of the heat leak to the 2DEG before and after illumination.NT_tau.dat - temperature dependence of the 2DEG NT thermalisation time constant, with the NT both connected to the 2DEG and running on its own. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Important contribution to ultra low temperature technology for low dimensional physics 
URL https://figshare.com/articles/dataset/Data_supporting_Cooling_Low-Dimensional_Electron_Systems_into_...
 
Title Data supporting "Cooling Low-Dimensional Electron Systems into the Microkelvin Regime" article 
Description This dataset combines all the supporting data under single DOI. The individual files contain:Te_vs_dotQe.dat - modelled electron temperature as a function of heat leak to the electrons.Rsquare_vs_T.dat - temperature dependence of the 2DEG sheet resistance before and after illumination..R_NT-Iminus_vs_T.dat - temperature dependence of the resistance between NT and I- ohmic contacts before and after illumination.dQnt_dTnt.dat - thermal conductance between 2DEG NT and 3He bath before and after illumination.dQnt_dTnt.dat - non-local thermal conductance, describing the response of 2DEG NT to heating the 2DEG before and after illumination.dotQe_vs_t.dat - time dependence of the heat leak to the 2DEG before and after illumination.NT_tau.dat - temperature dependence of the 2DEG NT thermalisation time constant, with the NT both connected to the 2DEG and running on its own. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Important contribution to development of ultra low temperature techniques for physics of electron transport in nanostructures 
URL https://figshare.com/articles/dataset/Data_supporting_Cooling_Low-Dimensional_Electron_Systems_into_...
 
Title Dependence of electron temperature in the 2DEG on the applied power 
Description Electron temperature as a function of applied power (i.e. heat leak), derived from the thermal model based on thermal transport measurements. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Confirmation of model of electron heating based on phonon emission 
URL https://figshare.com/articles/dataset/Dependence_of_electron_temperature_in_the_2DEG_on_the_applied_...
 
Title Dependence of electron temperature in the 2DEG on the applied power 
Description Electron temperature as a function of applied power (i.e. heat leak), derived from the thermal model based on thermal transport measurements. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Important check on electron heating as a function of applied field 
URL https://figshare.com/articles/dataset/Dependence_of_electron_temperature_in_the_2DEG_on_the_applied_...
 
Title Evolution of heat leak to 2DEG with time before and after illumination 
Description Heat leak to the 2DEG inferred from the temperatures of the 2DEG NT and 3He bath (included in the dataset) before and after illumination of the 2DEG. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Illumination is a standard method of decreasing disorder but can give rise to problems of leakage currents 
URL https://figshare.com/articles/dataset/Evolution_of_heat_leak_to_2DEG_with_time_before_and_after_illu...
 
Title Evolution of heat leak to 2DEG with time before and after illumination 
Description Heat leak to the 2DEG inferred from the temperatures of the 2DEG NT and 3He bath (included in the dataset) before and after illumination of the 2DEG. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Describes some of the practical problems which can arise 
URL https://figshare.com/articles/dataset/Evolution_of_heat_leak_to_2DEG_with_time_before_and_after_illu...
 
Title Research data supporting 'Giant Magnetoresistance in a CVD Graphene Constriction' 
Description The zipped file contains the resistance and conductance data from measurements of graphene channels as a function of magnetic field, temperature, and source-drain bias. Data are provided in separate .txt files for each figure. The README.txt file contains the column information and units for plotting. Specific data included are: Figure 1: (1) Resistance of the primary graphene channel as a function of back gate voltage at magnetic field B = 0 T and temperature T = 0.29 K. (2) Derivative of resistance as a function of back gate voltage at different magnetic fields and back gate voltages. Figure 2: The graphene conductance as a function of magnetic field at temperatures T = 0.29, 0.6, 1, 2, 5, 8, 11.3, 14, 17.8 and 25 K. Figures 3 and 4: Graphene resistance as a function of total source-drain bias applied to the circuit at different back gate voltages V_G = 0.2, 0.26, and 0.32 V, at temperature T = 0.29 K. The graphene resistance at charge neutrality as a function of total source-drain bias is also provided at different temperatures T = 0.29, 2, 5, 8, 11.2, 14.1, 17.8, and 25 K. These data are measured at B = 0 T. Figure 5: Transfer characteristics from a second graphene device. (1) The resistance is given as a function of back gate voltage at magnetic fields B = 0, 3, 6, 9, and 12 T, at temperature T = 1.5 K. (2) The resistance as a function of back gate voltage and magnetic field. (3) The resistance as a function of back gate voltage at different temperatures T = 1.5, 5, 11, and 30 K, and magnetic field B = 12 T. (4) The maximum resistance of the charge neutrality peak 'a' near gate voltage ~42 V, and peak 'b' at gate voltage 18 V, as a function of B at T = 1.5 K. (5) The resistance of peaks 'a' and 'b' as a function of temperature at B = 12 T. Data contained in the supporting information is also provided. This includes: (1) The conductance of the primary graphene channel as magnetic field is swept at high carrier density, for temperatures from 0.29 to 25 K. (2) Graphene resistance as a function of total source-drain bias applied to the circuit at different back gate voltages V_G = 0.2, 0.28, 0.3, 0.32, 0.34, 0.38, 0.4, and 0.5 V, at temperature T = ~1.4 K. (3) Raman spectra of the graphene as a function of location over a 10 by 10 micron square area with a 1 micron grid spacing. 
Type Of Material Database/Collection of data 
Year Produced 2022 
Provided To Others? Yes  
Impact Further information on electrons as dimensionality is reduced. 
URL https://www.repository.cam.ac.uk/handle/1810/332887
 
Title Research data supporting 'High-Throughput Electrical Characterisation of Nanomaterials From Room to Cryogenic Temperatures' 
Description  
Type Of Material Database/Collection of data 
Year Produced 2020 
Provided To Others? Yes  
URL https://www.repository.cam.ac.uk/handle/1810/311600
 
Title Response of 2DEG NT to heating 2DEG; non-local thermal condutance 
Description Response of noise thermometer, connected to 2DEG to Joule heating of the 2DEG, converted to corresponding non-local thermal conductance. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Informative on way energy is transferred in nanostructures 
URL https://figshare.com/articles/dataset/Response_of_2DEG_NT_to_heating_2DEG_non-local_thermal_condutan...
 
Title Response of 2DEG NT to heating 2DEG; non-local thermal condutance 
Description Response of noise thermometer, connected to 2DEG to Joule heating of the 2DEG, converted to corresponding non-local thermal conductance. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Increases understanding of electronic processes at the nano scale 
URL https://figshare.com/articles/dataset/Response_of_2DEG_NT_to_heating_2DEG_non-local_thermal_condutan...
 
Title Supporting data for "High-yield parallel fabrication of quantum-dot monolayer single-electron devices displaying Coulomb staircase, contacted by graphene" 
Description The data used in the accompanying paper are included here. Please see readme file for more details 
Type Of Material Database/Collection of data 
Year Produced 2022 
Provided To Others? Yes  
Impact Demonstrates control of device fabrication. 
URL https://www.repository.cam.ac.uk/handle/1810/342252
 
Title Thermal conductance between 2DEG NT and 3He bath 
Description Thermal conductance at ultra-low temperatures with two parallel channels: 1) via 2DEG and ohmic contacts, 2) via contact between the thermometer and liquid 3He bath. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Important for understanding how to mount sample in low temperature chamber 
URL https://figshare.com/articles/dataset/Thermal_conductance_between_2DEG_NT_and_3He_bath/17026952
 
Title Thermal conductance between 2DEG NT and 3He bath 
Description Thermal conductance at ultra-low temperatures with two parallel channels: 1) via 2DEG and ohmic contacts, 2) via contact between the thermometer and liquid 3He bath. 
Type Of Material Database/Collection of data 
Year Produced 2021 
Provided To Others? Yes  
Impact Important information on energy flow in nanostructures 
URL https://figshare.com/articles/dataset/Thermal_conductance_between_2DEG_NT_and_3He_bath/17026952/1