Impact of the biosphere on atmospheric aerosol and climate
Lead Research Organisation:
University of Leeds
Department Name: School of Earth and Environment
Abstract
Understanding climate change is one of the most important challenges facing science today. Atmospheric particles (aerosols) have an important cooling impact on the Earth, partly counteracting greenhouse gas warming over the industrial period. Quantifying this aerosol cooling is a critical step to making more accurate predictions of climate change. Considerable effort has been put into assessing the climate impact of anthropogenic (man-made) particle emissions. This proposal focuses on natural biogenic aerosol, which has been much less studied and is poorly understood. However, we need to understand the natural situation before we can fully understand how mankind is changing the atmosphere and the climate. Vegetation emits organic species to the atmosphere (the cause of the well known forest pine smell) where they can react to form particles. Vegetation also directly emits particles such as pollen and fungal spores. Observations have shown that these natural biogenic aerosol emissions can dominate the total particle load in much of the atmosphere. The particles cool the climate by reflecting sunlight and by making clouds thicker and more reflective. We also know that rain droplets form on these tiny biological particles and so they can play a role in controlling worldwide rainfall patterns. Despite such obvious importance, current climate models have a very limited representation of biological particle sources and so their importance for regulating climate is not well known. As the climate changes ecosystems will respond: plant activity such as photosynthesis is modified and vegetation distributions are changed. These changes modify biogenic aerosol emissions changing the amount of particles in the atmosphere with consequent impacts on aerosol cooling. Such climate feedbacks may dampen or amplify anthropogenic global warming. That is, as the world warms particle emissions from the forests may increase helping to cool the climate. In this way forests may act as a global 'air conditioner'. But we don't know how important this effect is because these interactions have not yet been treated by climate models. Tropical deforestation is rapidly changing land-cover but the impacts on climate are not well known because climate models do not treat all the necessary interactions between vegetation and climate. There is also interest in intentionally modifying land-use to mitigate climate change. For example, afforestation absorbs carbon dioxide into vegetation and could be used as a carbon-sink to offset greenhouse gas emissions from fossil fuel use. But the impact to climate of such changes to land-use is poorly known. Recent studies suggest that afforestation at high-latitudes (for example, in Europe) may actually warm the climate because dark forest vegetation absorbs more sunlight than snow-covered farmland. But these previous studies ignored particle emissions from the forest and their impact on climate. My own research has shown that these forest-derived particles result in an important cooling that can play a significant role in the net climate impact of land-use change. In this fellowship I will substantially improve our understanding of natural particles from the biosphere. I will include a comprehensive treatment of vegetation particle emissions in climate models for the first time. I will answer the fundamental question of how terrestrial biosphere emissions regulate global aerosol and climate. Finally, through an integrated assessment of different ecosystem-climate interactions I will improve our understanding of how changes to land-use alter climate.
People |
ORCID iD |
Dominick Spracklen (Principal Investigator) |
Publications
Arnold S
(2010)
Relationships between atmospheric organic compounds and air-mass exposure to marine biology
in Environmental Chemistry
Betha R
(2013)
Observations of new aerosol particle formation in a tropical urban atmosphere
in Atmospheric Environment
Bonn B
(2014)
The link between atmospheric radicals and newly formed particles at a spruce forest site in Germany
in Atmospheric Chemistry and Physics
Breider T
(2010)
Impact of BrO on dimethylsulfide in the remote marine boundary layer IMPACT OF BRO + DMS IN RMBL
in Geophysical Research Letters
Carslaw K
(2010)
A review of natural aerosol interactions and feedbacks within the Earth system
in Atmospheric Chemistry and Physics
Carslaw KS
(2013)
Large contribution of natural aerosols to uncertainty in indirect forcing.
in Nature
Crippa P
(2013)
Satellite-derived estimates of ultrafine particle concentrations over eastern North America
in Journal of Geophysical Research: Atmospheres
D'Andrea S
(2013)
Understanding global secondary organic aerosol amount and size-resolved condensational behavior
in Atmospheric Chemistry and Physics
Dougill AJ
(2012)
Lessons from community-based payment for ecosystem service schemes: from forests to rangelands.
in Philosophical transactions of the Royal Society of London. Series B, Biological sciences
Fiore AM
(2012)
Global air quality and climate.
in Chemical Society reviews
Heald CL
(2015)
Land use change impacts on air quality and climate.
in Chemical reviews
Jo D
(2013)
Effects of chemical aging on global secondary organic aerosol using the volatility basis set approach
in Atmospheric Environment
Laakso L
(2013)
Boundary layer nucleation as a source of new CCN in savannah environment
in Atmospheric Chemistry and Physics
Lapina K
(2011)
Investigating organic aerosol loading in the remote marine environment
in Atmospheric Chemistry and Physics
Lee L
(2013)
The magnitude and causes of uncertainty in global model simulations of cloud condensation nuclei
in Atmospheric Chemistry and Physics
Lee L
(2011)
Emulation of a complex global aerosol model to quantify sensitivity to uncertain parameters
in Atmospheric Chemistry and Physics
Manktelow P
(2010)
The impact of dust on sulfate aerosol, CN and CCN during an East Asian dust storm
in Atmospheric Chemistry and Physics
Mann G
(2010)
Description and evaluation of GLOMAP-mode: a modal global aerosol microphysics model for the UKCA composition-climate model
in Geoscientific Model Development
Mann G
(2012)
Intercomparison of modal and sectional aerosol microphysics representations within the same 3-D global chemical transport model
in Atmospheric Chemistry and Physics
Mann G
(2014)
Intercomparison and evaluation of global aerosol microphysical properties among AeroCom models of a range of complexity
in Atmospheric Chemistry and Physics
Martin S
(2010)
Sources and properties of Amazonian aerosol particles
in Reviews of Geophysics
Merikanto J
(2010)
Effects of boundary layer particle formation on cloud droplet number and changes in cloud albedo from 1850 to 2000
in Atmospheric Chemistry and Physics
Metzger A
(2010)
Evidence for the role of organics in aerosol particle formation under atmospheric conditions.
in Proceedings of the National Academy of Sciences of the United States of America
Perring A
(2015)
Airborne observations of regional variation in fluorescent aerosol across the United States
in Journal of Geophysical Research: Atmospheres
Pierce J
(2013)
Weak global sensitivity of cloud condensation nuclei and the aerosol indirect effect to Criegee + SO<sub>2</sub> chemistry
in Atmospheric Chemistry and Physics
Rap A
(2013)
Natural aerosol direct and indirect radiative effects
in Geophysical Research Letters
Reddington C
(2011)
Primary versus secondary contributions to particle number concentrations in the European boundary layer
in Atmospheric Chemistry and Physics
Reddington C
(2013)
The mass and number size distributions of black carbon aerosol over Europe
in Atmospheric Chemistry and Physics
Reddington C
(2014)
Contribution of vegetation and peat fires to particulate air pollution in Southeast Asia
in Environmental Research Letters
Riccobono F
(2014)
Oxidation products of biogenic emissions contribute to nucleation of atmospheric particles.
in Science (New York, N.Y.)
Schmidt A
(2012)
Importance of tropospheric volcanic aerosol for indirect radiative forcing of climate
in Atmospheric Chemistry and Physics
Scott C
(2015)
Impact of gas-to-particle partitioning approaches on the simulated radiative effects of biogenic secondary organic aerosol
in Atmospheric Chemistry and Physics
Scott C
(2014)
The direct and indirect radiative effects of biogenic secondary organic aerosol
in Atmospheric Chemistry and Physics
Scott CE
(2017)
Impact on short-lived climate forcers (SLCFs) from a realistic land-use change scenario via changes in biogenic emissions.
in Faraday discussions
Scott CE
(2018)
Impact on short-lived climate forcers increases projected warming due to deforestation.
in Nature communications
Spracklen B
(2013)
Regeneration of native broadleaved species on clearfelled conifer plantations in upland Britain
in Forest Ecology and Management
Spracklen BD
(2015)
A Global Analysis of Deforestation in Moist Tropical Forest Protected Areas.
in PloS one
Spracklen D
(2013)
Erratum: Corrigendum: Observations of increased tropical rainfall preceded by air passage over forests
in Nature
Spracklen D
(2010)
Explaining global surface aerosol number concentrations in terms of primary emissions and particle formation
in Atmospheric Chemistry and Physics
Spracklen D
(2014)
Tropical montane forests are a larger than expected global carbon store
in Biogeosciences
Spracklen D
(2012)
Observations of increased tropical rainfall preceded by air passage over forests
in Nature
Spracklen D
(2013)
Tropical montane forests are a larger than expected global carbon store
Spracklen D
(2013)
Natural aerosol-climate feedbacks suppressed by anthropogenic aerosol
in Geophysical Research Letters
Spracklen D
(2011)
Aerosol mass spectrometer constraint on the global secondary organic aerosol budget
in Atmospheric Chemistry and Physics
Spracklen D
(2016)
Carbon storage and sequestration of re-growing montane forests in southern Ecuador
in Forest Ecology and Management
Spracklen D
(2014)
The contribution of fungal spores and bacteria to regional and global aerosol number and ice nucleation immersion freezing rates
in Atmospheric Chemistry and Physics
Spracklen D
(2009)
Impacts of climate change from 2000 to 2050 on wildfire activity and carbonaceous aerosol concentrations in the western United States
in Journal of Geophysical Research
Spracklen D
(2011)
Global cloud condensation nuclei influenced by carbonaceous combustion aerosol
in Atmospheric Chemistry and Physics
Description | Findings from research have influenced UK government biofuel policy. |
First Year Of Impact | 2009 |
Sector | Environment |
Impact Types | Societal |
Description | Environmental Audit Committee |
Geographic Reach | National |
Policy Influence Type | Contribution to a national consultation/review |
Impact | Change to UK Biofuel Policy to include mandatory sustainability criteia |
URL | http://www.publications.parliament.uk/pa/cm200708/cmselect/cmenvaud/76/76.pdf |
Description | United Bank of Carbon |
Organisation | United Bank of Carbon |
Country | United Kingdom |
Sector | Private |
PI Contribution | Our research contributes to the overall aim of the United Bank of Carbon: "to protect the world's forests and their peoples". |
Collaborator Contribution | United Bank of Carbon has contributed funds towards a PhD studentship. |
Impact | Collaboration has facilitated £1.8 million public and private sector investment in forest conservation, managed 15 forest conservation projects worldwide and contributed to the protection of over 250,000 hectares of the world's forests. |
Start Year | 2009 |
Company Name | United Bank of Carbon |
Description | Not-for-profit registered charity |
Year Established | 2009 |
Impact | UBoC facilitated £1.8 million public and private sector investment in forest conservation, managed 15 forest conservation projects worldwide and contributed to the protection of over 250,000 hectares of the world's forests. |
Website | http://www.unitedbankofcarbon.com |
Description | Environment Audit Committee |
Form Of Engagement Activity | A formal working group, expert panel or dialogue |
Part Of Official Scheme? | Yes |
Geographic Reach | National |
Primary Audience | Policymakers/politicians |
Results and Impact | Gave expert evidence at the Environment Audit Committee on "Are biofuels sustainable?" The Environmental Audit Committee produced a report "Are Biofuels Sustainable?" http://www.publications.parliament.uk/pa/cm200708/cmselect/cmenvaud/76/76.pdf The report influenced Uk government biofuel policy to include mandatory sustainability criteria, |
Year(s) Of Engagement Activity | 2008 |
URL | http://www.publications.parliament.uk/pa/cm200708/cmselect/cmenvaud/76/76.pdf |
Description | Media |
Form Of Engagement Activity | A press release, press conference or response to a media enquiry/interview |
Part Of Official Scheme? | No |
Geographic Reach | International |
Primary Audience | Media (as a channel to the public) |
Results and Impact | Research has been covered in national and International media including print and on-line newspapers, radio and TV. I was interviewed twice on BBC Breakfast. Broader understanding of environmental issues |
Year(s) Of Engagement Activity | 2009,2010,2011,2012,2013,2014 |
Description | United Bank of Carbon Presentations |
Form Of Engagement Activity | A formal working group, expert panel or dialogue |
Part Of Official Scheme? | No |
Geographic Reach | National |
Primary Audience | Professional Practitioners |
Results and Impact | Presentations have been made to various businesses across the UK on the role of forests in climate mitigation and adaptation. Talks facilitated £1.8 million public and private sector investment in forest conservation. |
Year(s) Of Engagement Activity | 2008,2009,2010,2011,2012,2013,2014 |
Description | Various public presentations |
Form Of Engagement Activity | A talk or presentation |
Part Of Official Scheme? | No |
Geographic Reach | Regional |
Primary Audience | Public/other audiences |
Results and Impact | Discussion and short write-up in local newsletter Increased interest from members of the public, enquiries |
Year(s) Of Engagement Activity | 2009,2010,2011,2012,2013,2014 |