Volcanic plume understanding and forecasting: Integrating remote-sensing, in-situ observations and models (V-PLUS)

Lead Research Organisation: University of Cambridge
Department Name: Chemistry

Abstract

The 2010 Eyjafjallajökull and 2011 Grimsvötn eruptions in Iceland were stark reminders that society is increasingly vulnerable to volcanic hazards. Since 2012, volcanic eruptions are listed in the UK National Risk Register for Civil Emergencies, recognising the high potential for societal disruption and economic loss. Volcano observatories and regulatory bodies, including the nine Volcanic Ash Advisory Centres (VAACs), use a variety of tools and data to mitigate the impacts of eruptions, and ensure aviation safety. Some of the most important tools are atmospheric models that simulate the atmospheric transport and removal of volcanic plume constituents and form the backbone of the regulatory response. The accuracy of these model predictions relies on:

i) accurate input data, mainly derived from ground-based measurements and satellites;
ii) the accuracy of the model representation of volcanic plume transport and plume processes.

The overarching aims of V-PLUS are to transform our understanding of volcanic plumes and deliver methods and tools that enhance monitoring and forecasting capabilities in the UK and beyond. Our project partners and subcontractor include the Icelandic Met Office, the UK Met Office and Etna volcano observatory, which ensures that our new research breakthroughs will be used operationally by VAACs and volcano observatories. This will enhance our capabilities to mitigate the economic and societal hazards posed by volcanic eruptions.

To achieve our aims, V-PLUS will exploit data from a recently launched satellite sensor called TROPOspheric Monitoring Instrument (TROPOMI). The exceptional spectral and spatial resolution of TROPOMI, 12 times better than the previous generation of instruments, is for the first time comparable to ground-based measurements, and will be a game-changer in volcanology, providing an unprecedented opportunity to characterise and track volcanic plumes. V-PLUS will combine this new data with ground-based and other satellite data, as well as atmospheric modelling to study volcanic plumes with unprecedented fidelity. To improve our ability to measure volcanic ash from satellite imagery we will conduct experiments on volcanoes, directly sampling volcanic ash during volcanic explosions using unmanned aerial vehicles, and test numerical models of volcanic activity.

Aside from volcanic ash hazards, toxic volcanic sulphur species can degrade air quality, negatively affect human health, and potentially increase the cost of ownership of aircraft engines due to an increase in maintenance cycles. However, there is at present extremely limited knowledge of exposure thresholds and durations at which negative human health effects occur and the functioning of aircraft engines is compromised. While none of the VAACs are currently required to forecast the dispersion of volcanic sulphur, there is increasing recognition of the potential hazards from volcanic gases and their chemical conversion products. Thus, the requirement for VAACs could change in future. The chemical evolution of gases and aerosol particles controls the health and climatic impact of eruptions, and we will study this chemical evolution through experiments in accessible volcanic gas plumes.

In summary, the new atmospheric models and tools created by the V-PLUS will be rigorously tested using case study eruptions and translated into tools for direct use by VAACs and volcano observatories. Therefore, the V-PLUS project will have societal and economic benefits primarily through creating enhanced national and international capability to predict the dispersion of volcanic ash and gas plumes including their impacts on air quality, human health, climate and aviation.

Planned Impact

Given the London Volcanic Ash Advisory Centre (VAAC) is hosted by the Met Office in Exeter, the UK has a central role in understanding and forecasting volcanic plumes. V-PLUS will have societal and economic impacts through the following key deliverables:

(i) an improved understanding of volcanic plumes and their impacts on air quality, aviation, human health, the environment, and climate, and

(ii) enhanced monitoring capabilities and national capability to forecast volcanic ash and gas dispersion enabled due to the exploitation of newly-available satellite data (such as the TROPOspheric Monitoring Instrument) and the testing and refinement of dispersion and aerosol-chemistry-climate models against a wide range of measurements.

In V-PLUS we are actively engaged with the Met Office at every stage of the project, so that the research methods and outcomes are appropriately tailored to allow an efficient pull through to operations. The direct involvement of the Met Office will also allow us to anticipate at an early stage how our findings, data and methods may impact their current practices of forecasting volcanic plume dispersion and assimilating satellite data into their forecasts. Several team members have a proven track-record of creating impact: they are involvement in hazards assessments at volcano observatories, and they advise UK Government on the risks and effects of volcanic eruptions.

We have identified three potential pathways to impact:

1. Impact on national capabilities to forecast volcanic plume dispersion and chemical evolution at the Met Office/London VAAC. The tested and refined modelling capacities produced in V-PLUS can improve the Met Office/London VAAC capabilities for its central role of forecasting volcanic ash concentrations (needed to ensure aviation safety) by delivering improved models and ways to derive eruption source terms, a critical input. Several VAACs forecast the dispersion of volcanic sulphur in order to inform their ash forecasts. This combined with the increasing recognition of the potential hazards from volcanic gases and their chemical conversion products means volcanic gas dispersal forecasting is the subject of ongoing investigation by the International Civil Aviation Organization. The 2014-15 Holuhraun eruption also highlighted a UK requirement for such capability. The V-PLUS deliverables mean that the Met Office would have a well-tested and validated system to carry out near-real time forecasting of gas-rich volcanic plumes and their potential impacts to inform Government and aviation.

2. Impact on understanding and capabilities to forecast hazards from volcanic eruptions to the UK. Since 2012, volcanic eruptions are listed on the UK National Risk Register for Civil Emergencies. In the UK, civil contingency planning and response to volcanic hazards is based on scientific evidence of the potential impacts of a volcanic eruption. In V-PLUS we will carry out impact assessments for both explosive multi-phase eruptions as well as long-lasting, gas-rich Icelandic eruptions based on the refined modelling tools created. Provision of and output from these models can have an impact on decision-making and the level of preparedness in the event of a volcanic crisis affecting the UK or UK overseas territories.

3. Impact on volcano monitoring practices. V-PLUS aims to impact on practices at volcano observatories who are charged with monitoring volcanic activity using satellite- and ground-based remote sensing. In V-PLUS, we will assess the effect of utilising new models and methods to forecast volcanic plume dispersion on practices at the London VAAC, which will benefit other VAACs and volcano observatories worldwide. For instance, we expect the automated method to derive mass fluxes and plume heights we develop in V-PLUS to create enhanced capabilities at volcano observatories around the world including ODA-listed countries (e.g. Nicaragua).

Publications

10 25 50

publication icon
Christensen MW (2022) Opportunistic experiments to constrain aerosol effective radiative forcing. in Atmospheric chemistry and physics

publication icon
Ilyinskaya E (2021) Rapid metal pollutant deposition from the volcanic plume of Kilauea, Hawai'i in Communications Earth & Environment

publication icon
Marshall L (2022) Volcanic effects on climate: recent advances and future avenues in Bulletin of Volcanology

publication icon
Staunton-Sykes J (2021) Co-emission of volcanic sulfur and halogens amplifies volcanic effective radiative forcing in Atmospheric Chemistry and Physics

 
Title Movie of the 2019 Raikoke volcanic eruption: Sulfur dioxide and sulfate dispersion as simulated by NAME 
Description Included are 4 movies showing the Vertical Column Density (VCD) evolution for the 2019 Raikoke volcanic cloud between 21-06-2019 and 16-07-2019 as simulated by the Met Office's Numerical Atmospheric-dispersion Modelling Environment (NAME) (all showing VCD values in DU): StratProfile_SO2.mov: The dispersion of sulfur dioxide based on the StratProfile vertical emission profile. StratProfile_SO4.mov: The dispersion of sulfate based on the StratProfile vertical emission profile. VolRes15_SO2.mov: The dispersion of sulfur dioxide based on the VolRes1.5 vertical emission profile. VolRes15_SO4.mov: The dispersion of sulfate based on the VolRes1.5 vertical emission profile. 
Type Of Art Film/Video/Animation 
Year Produced 2020 
URL https://zenodo.org/record/3992052
 
Title Movie of the 2019 Raikoke volcanic eruption: Sulfur dioxide and sulfate dispersion as simulated by NAME 
Description Included are 4 movies showing the Vertical Column Density (VCD) evolution for the 2019 Raikoke volcanic cloud between 21-06-2019 and 16-07-2019 as simulated by the Met Office's Numerical Atmospheric-dispersion Modelling Environment (NAME) (all showing VCD values in DU): StratProfile_SO2.mov: The dispersion of sulfur dioxide based on the StratProfile vertical emission profile. StratProfile_SO4.mov: The dispersion of sulfate based on the StratProfile vertical emission profile. VolRes15_SO2.mov: The dispersion of sulfur dioxide based on the VolRes1.5 vertical emission profile. VolRes15_SO4.mov: The dispersion of sulfate based on the VolRes1.5 vertical emission profile. 
Type Of Art Film/Video/Animation 
Year Produced 2020 
URL https://zenodo.org/record/3992051
 
Description Key achievements
WP1:
• In WP1 we have made strong progress towards scientific objectives and achieved several successes. The main work has been deployed in developing the PlumeTraj platform which allows flux time series to be retrieved from satellite imagery. This is now fully developed and working efficiently, producing very high quality data. We have had some important eruptions in 2021 which have shown the full potential of the plumetraj approach. The eruption of St Vincent produced some of the highest gas fluxes ever measured. The ongoing eruption of la Palma has produced a fantastic opportunity to compare satellite measured gas amounts and heights with ground based observations, as the plume advected over N Europe on 19/20 October. These observations also permit comparison with plume dispersion model initialised with a source term generated by plumetraj, work which we hope will show that we achieve better forecasts with our retrieved heights and gas amounts.
• New physically-based models of volcanic umbrella clouds have been developed within V-PLUS (WP1.2), and implementation of these within the widely-used Met Office dispersion code 'NAME' is well underway (deliverable 3.3). NAME has also been integrated into the algorithms for back-trajectory modelling (WP1.1), allowing these improved umbrella cloud descriptions to be used in satellite inversions (deliverable 1.3).
• The collaborations instigated by V-PLUS have led to a joint MSc research project between the Met Office and V-PLUS Co-I Chris Johnson at the University of Manchester, which extended V-PLUS work to describe the vertical distribution of ash within a volcanic plume using a Suzuki distribution. Code written during this project is now checked in to the NAME source code and scheduled to be included in the next public release, providing a template for similar dissemination of the V-PLUS plume modelling work through additions and improvements to NAME capability.
• The IASI linear and iterative retrievals developed in Oxford have been applied to over a decade of IASI spectra (mid 2007 - mid 2019) with some gaps still to be filled. This provides a rich dataset for studying volcanic plumes and to facilitate collaborations. Analysis of the results has looked at the global distribution and the vertical distribution of these emissions. This is useful for investigating the impacts of these plumes of climate/atmosphere, looking at long term volcanic activity and for assessing the potential long-term effects on aircraft. Manuscript looking at the results is in preparation. Open access dataset planned.
• The IASI SO2 retrievals have been applied to over a month of spectra following the eruption of La Soufrière in April 2021. Study looks at the transport of this plume, the total mass of SO2 emitted and the vertical distribution of the emission. Manuscript in preparation for special issue on this eruption.
• The Raikoke eruption in 2019 emitted large quantities of SO2 and ash into the atmosphere. It has been a great case study for highlighting some of the strengths and limitations of the IASI SO2 retrievals. One issue identified was the height results tending to the a priori over time as the amount of SO2 fell (loss of information in the spectra). Some adaptations have been made to the retrieval in light of these results. The results following these changes look promising and show some interesting dynamics within the plume. Manuscript in preparation for special issue (ACP) on this eruption. Data from this eruption has also been used in WP3 (e.g. de Leeuw et al. 2021)



WP2:
• Development of a fast retrieval algorithm for SO2, aerosols and ash from OP-FTIR mesurements in emission mode. The aim is to provide a method that would enable gas measurements in periods when UV measuremenst are difficult or impossible (including night-time or when plume is aerosol-laden). Data has been collected in various viewing geometries, and with simultaneous UV measurements for validation. Results are being written for publication (expected early 2022).
• Two rapid-response field campaigns at Fagradalsfjall in Iceland: (1) March-April 2021 (E. Ilyinskaya) Samples of volcanic emissions (gas and particulate matter) collected at the eruptive vent and in several distal locations. Analyses are in progress. The aim is to understand the volcanic and atmospheric processes that govern the dispersion and deposition of environmentally-reactive species such as Se, As, Cd, Pb. (2) August 2021 (J-F. Smekens) Focused on ground-based remote measurements of gas and aerosol emissions. UV traverses (for SO2 fluxes) and FTIR solar occultation measurements (for gas ratios, SO2, HCl, HF) during periods of relative intensity vs quiescence. Data analysis is in progress. The aim is to determine whether the composition of gas emissions changes on short timescales during rapid changes of the eruptive activity.
WP3:
• A paper on the Raikoke eruption plume led by the WP3 PDRA has been published (de Leeuw et al, 2021, https://doi.org/10.5194/acp-21-10851-2021), with a second companion paper led by Met Office under review (https://acp.copernicus.org/articles/21/10851/2021/).
• The PlumeTraj approach being developed under WP1 was trialled as part of the MO's initial response to the Krysuvik eruption in early 2021, with promising indications.
• The underpinning work on both these aspects has informed a Met Office report for the International Civil Aviation Organization (ICAO) on global volcanic SO2 forecasting for aviation, including aspects of model performance, model chemistry and data-fusion techniques (Witham et al, 2021). This will be discussed at an ICAO meeting in November 2021.
• Tools for statistical comparison of model output to satellite retrievals developed under WP3.3 have been provided to the Met Office and are being used as part of an assessment of the use of ensemble meteorology.


Overall progress
• Overall progress is good. New tools and capabilities have been developed in the past year, which are now being increasingly applied across work packages. Travel restrictions due to COVID had a significant impact on our ability to collect data in the field but on several occasions we have now managed to collect data albeit at different locations than originally proposed. For further details see Section on notable issues below.

Notable issues
• Travel restrictions during the Covid-19 crisis have prevented measurement campiagns on original schedule. Several opportunities have arisen in the recent months (Iceland, Italy, La Palma field work) to progress despite these delays in terms of data collection, but analysis and publication will still be significantly impacted. These opprotunities came about at short notice and it is still very desirable to undertake coordinated campaigns, which require more complicated logistics (combining ground-based remote sensing and in-situ sampling), within the time frame of the grant.
• IASI data access - due to licensing change meaning that new data could not be accessed at CEDA (summer 2019-February 2021). This has significantly slowed down work as data had to be directly ordered from EUMETSAT.
Exploitation Route See above under key achievements
Sectors Aerospace, Defence and Marine,Environment

 
Title PlumeTraj results for Piton de la Fournaise April 2020 eruption 
Description PlumeTraj SO2 flux results for the April 2020 eruption of Piton de la Fournaise volcano, La Reunion, France 
Type Of Material Database/Collection of data 
Year Produced 2022 
Provided To Others? Yes  
URL https://figshare.com/articles/dataset/PlumeTraj_results_for_Piton_de_la_Fournaise_April_2020_eruptio...
 
Title PlumeTraj results for Piton de la Fournaise April 2020 eruption 
Description PlumeTraj SO2 flux results for the April 2020 eruption of Piton de la Fournaise volcano, La Reunion, France 
Type Of Material Database/Collection of data 
Year Produced 2022 
Provided To Others? Yes  
URL https://figshare.com/articles/dataset/PlumeTraj_results_for_Piton_de_la_Fournaise_April_2020_eruptio...