SEANA -Shipping Emissions in the Arctic and North Atlantic atmosphere

Lead Research Organisation: University of Birmingham
Department Name: Sch of Geography, Earth & Env Sciences

Abstract

Shipping is the largest means of moving freight globally. Ships consume dirty fuels, making them one of the most important sources of anthropogenic aerosol in the marine atmosphere. Aerosols from shipping can affect the climate directly through absorption and scattering of radiation, with an overall cooling effect to the atmosphere. They can also indirectly influence the climate by changing cloud properties, e.g., albedo and lifetime, which further cools the atmosphere.

Two key challenges for assessing future climate impact of shipping emission are (i) knowing the status of the present-day aerosol system - as a baseline from which any climate predictions are made and (ii) quantifying the amount of pollutants emitted.

Currently little consensus exists on the impact of shipping emissions in the Arctic and North Atlantic Atmosphere (ANAA) primarily due to a lack of observations and insufficient model skills. Recent modelling work suggests that the Arctic aerosol baseline should account for a disparate range of natural sources. Few models are sufficiently comprehensive, and while some models can reproduce aerosol in some Arctic regions, there is evidence that models can produce similar results via different sources and processes. An inability to reflect the aerosol baseline processes can have significant impact on the reliability of future climate projections.

Shipping is also undergoing significant changes. In January 2020, a new International Maritime Organisation (IMO) regulation comes into force, which reduces, by more than 80%, the sulphur content in maritime fuel oils. Superimposed on that, recent climate induced changes in Arctic sea ice are opening up new seaways enabling shorter sea passages between key markets. Significant growth in shipping via the North West Passage (NWP) is anticipated in the coming years. Thus, there is a short window of opportunity to define current atmospheric conditions, against which the impact of these changes must be determined.

SEANA will take advantage of the above-mentioned opportunity to make multiple atmospheric measurements over multiple platforms to understand the present-day baselines - sources of aerosol particles including the contribution from shipping - and to determine the response of ANAA aerosol to new fuel standards after 2020. Extended measurements will be conducted at two stations adjacent to the NWP enabling the source of particles to be apportioned using receptor modelling approaches. In addition, SEANA will participate in a Korean cruise to the west side of the NWP, and a NERC cruise to the east, to measure both natural and anthropogenic particles and aerosol processes in two contrasting Arctic environments.

These new observations will be integrated with recent / ongoing measurements at partner ANAA stations to generate a benchmark dataset on aerosol baseline in ANAA to constrain processes in the UK's leading global aerosol model, ensuring that the model is reproducing the baseline aerosol in the ANAA faithfully. We will then test the models' response to significant reductions in shipping sulphur emissions using observations taken during the transition to low-sulphur fuels in 2020. The revised model, which can reproduce current "baselines" and accurately predict the response of emission changes in the ANAA, will then be used to predict the future impact of shipping on air quality, clouds and radiative forcing under multiple sea-ice and shipping scenarios.

SEANA will deliver a major enhancement of UK's national capacity in capturing baseline ANAA aerosol and responses to emission regulations, results of which will inform shipping policy at high-latitudes.

Planned Impact

The principal beneficiaries include government agencies including UK Met Office, Faroe Islands and Greenland Environment Agency; Arctic Council; Intergovernmental Panel on Climate Change (IPCC); and International Maritime Organisation (IMO) and the shipping industry.

Government agencies: Across the Arctic regions, observations are extremely sparse, either continuous or on a focussed-intensive basis. The lack of observations severely hinders progress towards understanding/managing the regional environment. For example, the recent (2017) Scientific Report from DCE - Danish Centre for Environment and Energy demonstrates the need for information on the impact of shipping in Greenland. SEANA will provide new data and model tools to improve the assessment on the impact of shipping on the Greenland environment. The Faroese Environment Agency operate long-term monitoring activities to capture information on air pollutants, including those from shipping activities in the region. Their activities will be considerably enhanced by the more detailed observations on the Faroe Islands as part of SEANA, enabling them to better understand the sources of air pollution. This will support the development of potential air pollution mitigation strategies, including the control of shipping emissions. Improvements to numerical models, underpinned by robust measurements, will provide more confidence that future projections of air quality/climate are reliable - currently this is not the case.

Arctic Council: The Arctic Council is a high-level intergovernmental forum which addresses issues faced by the Arctic governments and people living in the Arctic region. SEANA results will provide benchmark data on aerosol baselines and predictions of future shipping impact that can support policy-making in slowing down Arctic climate change.

IPCC: IPCC would benefit from an improved global climate model with a better understanding of the aerosol and climate in the high latitudes, which is highly uncertain in models.

International Maritime Organisation and the Shipping industry: Shipping industry and IMO will need evidence of the impact of their sulphur-reduction policy on air quality and its benefits to human health, as well as on the climate. SEANA will also provide fundamental information and modelling tool that can be used by IMO in the future to assess impacts of shipping for years to come and to develop future policies.


Wider Beneficiaries include the general public and the indigenous people living in the Arctic.

General public: It is expected that the IMO's new regulation on shipping fuel limit will deliver a cleaner air and health improvement globally, in particular in the coastal regions. The general public will be interested in knowing whether it actually delivers what it was predicted by the IMO. Furthermore, there is a considerable interest/awareness within the wider general public over the status of the Arctic region, in particular in light of changing sea ice. Future changes to the Arctic climate system is a sensitive issue that has direct impact on daily life, as demonstrated by the occasional Arctic snow blasts of the UK, causing major disruption to transport. We expect SEANA result will excite the next generation of scientists and likely capture the imagination of a plethora of young people.

Indigenous people living in the Arctic: They will benefit from an improved understanding and prediction of climate change in the Arctic, which has direct impact on their life in the future. They will also benefit from an improved understanding of the likely impact of future shipping on local air quality, which directly affects their health. SEANA's outcomes will support future policy actions to control future climate change and air pollution in the Arctic, which will directly improve their welfare.

Publications

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Park J (2019) Arctic Primary Aerosol Production Strongly Influenced by Riverine Organic Matter. in Environmental science & technology

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Zhang C (2021) Impact of air emissions from shipping on marine phytoplankton growth. in The Science of the total environment

 
Description 1) Aerosol mixing states in Arctic aerosol: We found that 74% of non-sea-salt sulfate particles were coated with organic matter and a fifth of these particles also had soot inclusions in the organic coating. Our studies discovered this organic matter coating on individual sulfate particles, which may affect reactions between reactive gases and sulfate particles in the Arctic air. It may also have a significant influence on the absorption properties of individual particles, depending on the optical properties of the organic matter.

2) Sources of coarse particles in the Arctic: We carried out a cluster analysis of multiyear (2015-2019) aerodynamic volume size distributions, with diameter ranging from 0.5 to 20 µm, measured continuously at the Gruvebadet Observatory in the Svalbard archipelago. Together with aerosol chemical composition data from several online and offline measurements, we apportioned the occurrence of the coarse-mode aerosols during the study period (mainly from March to October) to anthropogenic (two sources, 27 %) and natural (three sources, 73 %) origins. Specifically, two clusters are related to Arctic haze with high levels of black carbon, sulfate and accumulation mode (0.1-1 µm) aerosol. The first cluster (9 %) is attributed to ammonium sulfate-rich Arctic haze particles, whereas the second one (18 %) is attributed to larger-mode aerosol mixed with sea salt. The three natural aerosol clusters were open-ocean sea spray aerosol (34 %), mineral dust (7 %) and an unidentified source of sea spray-related aerosol (32 %). The results suggest that sea-spray-related aerosol in polar regions may be more complex than previously thought due to short- and long-distance origins and mixtures with Arctic haze, biogenic and likely blowing snow aerosols. Studying supermicrometer natural aerosol in the Arctic is imperative for understanding the impacts of changing natural processes on Arctic aerosol.

3) Sources of aerosols in Svalbard: We applied a receptor model and an explainable machine learning technique to understand the sources and drivers of particle numbers from 10 nm to 20 µm in Svalbard. Nucleation, biogenic, secondary, anthropogenic, mineral dust (two types), sea salt and blowing snow aerosols and their major drivers were identified. Our results show that the monthly variations of particles are highly size/source dependent and regulated by meteorology. Nucleation and secondary aerosols are the largest contributors to Arctic aerosol in number. Nonlinear responses to temperature were found for biogenic and local dust particles, highlighting the importance of melting sea ice and snow. These results indicate that each aerosol source will respond to rapid Arctic warming differently and in a non-linear fashionbe

4) During a research cruise to the Davis Strait, we observed several new particle formation events, where the particles grew bigger enough to be cloud condensation nuclei (CCN). These new CCN could increase the cloud cover and thus reduce the incoming lights, with the potential to cool the atmosphere over the ocean.

5) During a research cruise to the Davis Strait, we found some evidence of shipping emissions on the aerosol concentrations and chemical compositiion
Exploitation Route To be developed
Sectors Education,Environment

 
Description Changing Shipping Emissions: Impact on sulphate aerosol in the marine atmosphere
Amount £18,000 (GBP)
Organisation Natural Environment Research Council 
Sector Public
Country United Kingdom
Start 09/2019 
End 08/2021
 
Description Coupling of organic and inorganic aerosol systems in coastal atmosphere: the effect impact on secondary organic aerosol formation
Amount £110,000 (GBP)
Organisation The Royal Society 
Sector Charity/Non Profit
Country United Kingdom
Start 03/2019 
End 03/2022
 
Description LPDP Indonesia Endowment Fund for Education - PhD studentship
Amount £100,000 (GBP)
Organisation Layanan Beasiswa dan Pendanaan Riset Indonesia 
Sector Public
Country Indonesia
Start 10/2019 
End 09/2022
 
Description Reactive nitrogen chemistry and haze formation: towards the new WHO air quality guidelines
Amount £24,000 (GBP)
Funding ID IEC\NSFC\211160 
Organisation The Royal Society 
Sector Charity/Non Profit
Country United Kingdom
Start 03/2022 
End 03/2024
 
Description The UK-China Collaboration to Optimise Net Zero Policy options for Air Quality and Health
Amount £630,000 (GBP)
Funding ID 2021GRIP02COP-AQ 
Organisation Natural Environment Research Council 
Sector Public
Country United Kingdom
Start 11/2021 
End 03/2022
 
Title Research data supporting "Stimulation of oceanic phytoplankton growth by ship emitted particles" 
Description  
Type Of Material Database/Collection of data 
Year Produced 2020 
Provided To Others? Yes  
URL http://edata.bham.ac.uk/507/
 
Description Anhui Institute of Optics and Fine Mechanics 
Organisation Anhui Institute of Optics and Fine Mechanics
Country China 
Sector Public 
PI Contribution Joint research on air pollution related topics
Collaborator Contribution Data and human resources to research on air pollution sources and processes
Impact Royal Society - NSFC Travel Grant: IEC\NSFC\211160
Start Year 2022
 
Description Anhui Institute of Optics and Fine Mechanics 
Organisation Anhui Institute of Optics and Fine Mechanics
Country China 
Sector Public 
PI Contribution Joint research on air pollution related topics
Collaborator Contribution Data and human resources to research on air pollution sources and processes
Impact Royal Society - NSFC Travel Grant: IEC\NSFC\211160
Start Year 2022
 
Description SEANA Research Collaboration with CSIC-ICM 
Organisation Spanish National Research Council (CSIC)
Department Institute of Marine Sciences
Country Spain 
Sector Public 
PI Contribution Resources, instrumentation, and data analysis tools
Collaborator Contribution Manpower to contribute to SEANA project work New datasets collected in the Arctic Access to instrumentation that are not available
Impact New understanding on the sources and processes of aerosol particles in the Arctic
Start Year 2020
 
Description Tianjin University 
Organisation Tianjin University
Country China 
Sector Academic/University 
PI Contribution We designed the experiments.
Collaborator Contribution Professor Pingqing Fu's group supported the field sampling in both summer and winter.
Impact The project is ongoing with no direct output yet.
Start Year 2018
 
Description Zhejiang University: Weijun Li 
Organisation Zhejiang University
Country China 
Sector Academic/University 
PI Contribution Data analysis, unique samples, fieldwork support, student training, and paper writing
Collaborator Contribution Manpower in field and laboratory measurements, instruments for signle particle collection, data for joint publications
Impact Research focused on understanding the sources, aging and processes of airborne particles using single particle analysis techniques including TEM and NanoSIMS. Recent research aims to better understand what controls the solubility of iron in the fine particles in urban atmosphere.
Start Year 2018