Improving the chronology of early human evolution

Lead Research Organisation: University of Oxford
Department Name: School of Archaeology

Abstract

The Turkana and Awash basins in the East African Rift, preserve an exceptional fossil and archaeological record and to a large extent, form the basis for our current understanding of early hominin environments. Ancient volcanic activity has left numerous ash deposits (tuffs) that can be dated using the radiometric dating method 40Ar/39Ar. Although precise, dates obtained by this method only provide broad envelopes with significant temporal gaps because volcanism is episodic, and tuffs do not always survive across the landscape. Furthermore, despite the abundance of archaeological finds and animal fossils in this region, datable tuffs are rare in the East African Rift. Consequently, age estimation often relies on imprecise relative methods, such as magnetostratigraphy and biostratigraphy. A method for obtaining absolute dates is urgently required in order to correlate all the sedimentary sequences within the eastern rift, as well as across Africa, and to help clarify the wider picture of early human biological and cultural events during the Plio-Pleistocene. Likewise, the South African sites also suffer from dating problems, albeit from different issues. In most of these cases they are karstic infills and only recently, have any absolute methods based on cosmogenic and uranium/lead isotope systems been applied. These techniques also leave huge gaps and/or do not precisely date the fossil or archaeological event of interest. For instance, U/Pb dates generally reflect the ages of over- or underlying flowstone and not that of a fossil.

We propose to apply a novel luminescence-based method known as infrared-radiofluorescence (IR-RF), which the named researcher co-investigator on this proposal helped to develop, in order to determine the age (i.e. time of deposition) of fossil- and artefact-bearing sediments and/or volcanic tuffs in Kenya, Ethiopia and South Africa and to fill in the time gaps omitted by radiometric techniques. The IR-RF method is widely applicable due to the ubiquitous occurrence of sand sized feldspar mineral grains required for dating and the technique targets potassium- (K-) rich feldspar, one of the most common types of mineral on earth. Recent studies suggest that this methodology has the potential to extend the age range of luminescence dating from 0.5 million years to 4 million years, thus encompassing the majority of the time range over which the human family evolved.

Methods of recording and analyzing luminescence data have developed significantly over the last five years, including improved light detection and more advanced analytical and statistical techniques, all of which have led to new approaches and more flexible ways of processing and visualizing data. Recent technological advances including the development of single photon imaging systems based on electron multiplying charge coupled devices (EMCCD) also suggest that the time is right to bring together and apply some of these new cutting-edge innovations to help achieve more reliable chronologies for early hominin evolution.

This research will dramatically increase the number of well-dated sequences in areas archiving key evidence for early human evolution and it will enable us to provide significant improvements in correlating human fossil records across Africa. A new and more refined chronological framework will greatly improve our understanding of the diversity of adaptive challenges faced by early hominins since the Pliocene and it will help to shed more light on the hotly debated question of the role of climatic and ecological changes in driving hominin evolution.

Planned Impact

The record of past climate change and its impacts on human evolution provides an ideal context for considering issues surrounding human adaptability, the effects of future climate change, and the response of our species to environmental change. Although, research into chronology and past environments is of no immediate commercial value, it seeks to understand events and processes that despite being lost in time, are of deep interest to most people. We believe that our research can provide a very powerful tool for education and public engagement and we wish to focus the impact of our work on science enrichment. In particular, we would like to target children of primary school age, based on the premise that our research can provide a good vehicle for showcasing how science 'works', and how we know what we think we know. We will develop an educational resource for schools which can be made freely available as a download from our project website. In conjunction with our project partners in the field, we will also seek to directly engage with primary schools situated in the vicinity of our archaeological sites in Kenya, Ethiopia and South Africa by organising visits, giving talks and participating in activities with the children and their teachers. The proposed study will hopefully benefit such local communities for whom cultural heritage relating to human prehistory is a matter of local pride but whom we feel are significantly under-served in current efforts to disseminate scientific knowledge whilst at the same time, being held responsible for taking care of globally important archaeological sites.

Our research in geochronology will also directly add value to fossil collections housed within national institution, and it has the potential to transform the archaeological and geological heritage of each country by providing critical context to many previously undatable collections of fossils and archaeological remains. We are particularly keen to build bridges between higher education and research institutions and we will seek to strengthen collaborative networks between research groups spanning the European and African continents. The project links the major fossil repositories of various countries including the National Museums of Kenya and the Maropeng Visitor Center in the 'Cradle of Humankind World Heritage Site' in South Africa. We are convinced that the proposed new luminescence dating methodology can have a similar impact on human evolutionary studies as the radiocarbon revolution had on archaeology. Although, this project will by no means solve all of the many dating issues, it will aim to provide a template and guidance for how to approach this kind of chronometric work and we expect it to leave a long lasting legacy. We aim to provide site-based data illustrating the power of our new methodological approach and to document our research with powerful case studies representing best practice in the field. To facilitate intellectual exchange between each community, chronological and environmental databases will be made freely available on the Oxford based ORAU Data Service databases (see data management plan). Our academic publication plan will see publications across a range of geology, physical and archaeological science journals. This will demonstrate the opening of a considerable research frontier that can reflect the diversity of analytical work needed to fully understand the driving forces behind human evolution.
 
Description Characterization of the main dosimetric trap in K-feldspar mineral grains for application in infrared radiofluorescence dating. 
Organisation Brookhaven National Laboratory
Department National Synchrotron Light Source
Country United States 
Sector Public 
PI Contribution Our role in this collaboration is to supply and prepare suitable samples for analysis, to examine the physical origin of the infrared radiofluorescence (IR-RF) emission in K-feldspar mineral grains and to assess whether the grain geochemistry and crystallography influence the age limit of the IR-RF dating method. We propose to examine individual K-feldspar grains previously screened and characterized using our existing IR-RF luminescence reader, by high resolution µ-XRF and µ-XANES at the SRX beamline of the National Synchrotron Light Source-II (NSLS) at Brookhaven National Laboratory (BNL) in Upton, New York. As part of this experiment we also intend to use XRD at the XPD beamline to investigate the structural properties of K-feldspar and to help determine how the atomic arrangement may influence the luminescence properties for scientific dating purposes.
Collaborator Contribution Our partner in this collaboration is Dr Juergen Thieme, Science coordinator for the imaging and microscopy program at NSLS-II and who will assist with the loading of samples, data collection, learning of specialist software tools and analysis of data. The extraordinary high brilliance of the synchrotron X-ray source wil allow us to see more detail inside individual feldspar grains and with greater precision compared to what is achievable with standard X-ray sources fitted inside laboratory instruments. For micro-XRF and Xanes analyses, BNL are providing access to beamline 5-ID and for high resolution XRD analysis, we requested access to beamline 28-ID over the 1-year lifetime of the proposal.
Impact We completed a first set of analyses in November 2021 (six out of 18 shifts). The experiment is ongoing and we are currently analyzing the initial set of data. We will not be in a position to report any outputs until the experiment is completed.
Start Year 2021
 
Description Radiation detection with a silicon-based time-pixelated quantum counting/imaging detector: implications for luminescence dating 
Organisation University of Oxford
Department Particle Physics
Country United Kingdom 
Sector Academic/University 
PI Contribution Testing the potential use of the Timepix4 detector for applications in trapped charge dating
Collaborator Contribution Access to specialist technology and expertise
Impact This collaboration has not yet produced any tangible outcome but we hope to present initial findings of our experiments at a forthcoming internaltional conference in Denmark.
Start Year 2022
 
Title OxGamma 
Description OxGamma is a simple and user-friendly MATLAB based application, available for both Windows OS and macOS which allows easy and speedy calibration of portable gamma-ray spectrometers and calculation of the concentrations of radioisotopes (K, U and Th) from recorded field spectra. The application provides output using both a windows and a threshold approach and crucially, without requiring the user to have any previous experience in programming or excel wizardry. The list below provides some of the key features: - Quick and easy to perform the initial energy and efficiency calibration of a portable gamma-ray spectrometer using appropriate standards (U, Th, K & background). The user can opt to apply a baseline correction (exponential or linear) and multiple field spectra can be processed. - The MATLAB application is compatible with Windows and macOS and is able to process data from common file types (e.g. .cnf or .chn) associated with two of the main nuclear instrument manufacturers (i.e Mirion/Canberra and Ametec/EG&G Ortec). Alternatively, the spectral data can be imported as an ASCII text file (i.e .txt). - The application utilises an effective algorithm to correct for drift in the recorded field spectra which is often caused by changes in the environmental conditions (e.g. temperature). - The relevant calibration results are saved for reference. - To calculate the external gamma dose rate, the user can choose between different conversion factors. - The software tool enables to determine the concentrations of radioisotopes (K, U and Th) using the windows method or to calculate gamma dose-rates using the threshold approach. 
Type Of Technology Webtool/Application 
Year Produced 2022 
Impact This software aims to make it easier for non specialists to determine reliable external gamma dose rates when collecting samples for trapped charge dating methods such as luminescence and electron spin resonance dating 
URL https://sites.google.com/view/oxgamma
 
Description A synchrotron study of the defects associated with the principal trap in feldspar: initial findings 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact This was an oral presentation given to delegates of the annual UK Luminescence and Electron Spin Resonance Dating Conference held at Royal Holloway, University of London 7-9 September 2022.
Year(s) Of Engagement Activity 2022
 
Description Further investigations into IR-RF and IR-PL 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Poster presentation given at the 16th International Luminescence and ESR Dating Conference in Burgos (Spain) during session 2: Insights into feldspar luminescence processes. This was an opportunity to share some initial findings for dating K-feldspar mineral grains using infrared radio-fluorescence.
Year(s) Of Engagement Activity 2021
 
Description IR-OSL/PL/RF emissions in feldspar 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Dr Raju Kumar was an invited speaker at the IR-RF workshop held in Giessen (Germany) from 1-3 June 2022
Year(s) Of Engagement Activity 2022
 
Description Mapping oxidation states of Fe and Pb at micron-level in naturally occurring aluminosilicates (feldspars) for application in luminescence dating 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Study participants or study members
Results and Impact This was a poster presentation given at the online User's Metting of the U.S. National Synchrotron Light Source II (NSLS-ll) and Center for Functional Nanomaterials (CFN) held from 23rd - 26th May 2022.
Year(s) Of Engagement Activity 2022
 
Description OxGamma: a MATLAB based application for gamma spectrum analysis 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Poster presentation given at the 16th International Luminescence and ESR Dating Conference in Burgos (Spain) during session 4: Advances in instrumentation and dose rate determination. This was an opportunity to introduce the audience to a new software tool which our team developed to facilitate the calibration of field gamma-ray spectrometers and the analysis of spectra for trapped charge dating.
Year(s) Of Engagement Activity 2021
 
Description Participation in specialist IR-RF/IR-PL Working Group 
Form Of Engagement Activity A formal working group, expert panel or dialogue
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact To advance the use of infrared fluorescence and infrared photoluminescence as dating techniques through the exchange of knowledge and to serve as a platform for the start of collaborative work.
Year(s) Of Engagement Activity 2021
 
Description Work experience for local sixth form students 
Form Of Engagement Activity Participation in an open day or visit at my research institution
Part Of Official Scheme? No
Geographic Reach Regional
Primary Audience Schools
Results and Impact This was a two day placement of two local sixth form students who visited the laboratory in order to gain hands on practical experience as aprt of a work experience programme.
Year(s) Of Engagement Activity 2023