Measuring the electron electric dipole moment using an array of ultracold molecules
Lead Research Organisation:
IMPERIAL COLLEGE LONDON
Department Name: Physics
Abstract
The Standard Model of particle physics is one of the greatest achievements of modern science. It has been fabulously successful in classifying the fundamental particles and explaining how they behave. Nevertheless, it is widely accepted that the Standard Model is incomplete because it fails to explain several important observations. One prominent example is the excess of matter over antimatter in the universe. The Standard Model predicts almost equal amounts of matter and antimatter, but observations show the universe contains only matter. This contradiction is one of the great unsolved problems in modern physics and a major deficiency of our most fundamental theory.
To build a more complete picture of the universe, physicists are striving to reveal what lies beyond the Standard Model. This is an important objective of much of the research being done at gigantic particle accelerators. There is an alternative, and ingenious, way to explore the same problem - measure the shape of an electron. The new forces needed to explain the matter/antimatter imbalance also make electrons slightly non-spherical. This distortion - known as the electric dipole moment - changes the energy of an electron in an electric field, and that tiny change is amplified when the electron is bound to a molecule. I propose to build an apparatus that uses an array of molecules cooled to microkelvin temperatures to make an extremely precise measurement of the electron's shape. With very careful measurements, such table-top experiments enable us to probe energies equal to, or even above, those reached by the particle accelerators. Such marvellous precision has become possible by my recent success in cooling molecules to ultracold temperature. That technique is the foundation of this proposal.
My plan is to decelerate a beam of ytterbium monofluoride molecules to rest using the forces exerted by carefully tuned laser light, trap these molecules and cool them to a few microkelvin. Then, I will load them into an array of traps formed by standing waves of light. The array contains millions of individual traps and isolates the molecules from one another, creating a pristine environment for measuring the electron's electric dipole moment. This measurement is done by watching how the spin of the molecules precesses in applied magnetic and electric fields, similar to the precession of a gyroscope or spinning top in a gravitational field. An electric dipole moment changes this precession rate, though only by the tiniest amount. That tiny change is detected more easily if the spin precesses for a long time. Because molecules are confined and isolated in the array, the time can be thousands of times longer than in current experiments. That makes my measurement scheme far more sensitive than any other experiment, allowing me to search for new physics with unprecedented precision.
To build a more complete picture of the universe, physicists are striving to reveal what lies beyond the Standard Model. This is an important objective of much of the research being done at gigantic particle accelerators. There is an alternative, and ingenious, way to explore the same problem - measure the shape of an electron. The new forces needed to explain the matter/antimatter imbalance also make electrons slightly non-spherical. This distortion - known as the electric dipole moment - changes the energy of an electron in an electric field, and that tiny change is amplified when the electron is bound to a molecule. I propose to build an apparatus that uses an array of molecules cooled to microkelvin temperatures to make an extremely precise measurement of the electron's shape. With very careful measurements, such table-top experiments enable us to probe energies equal to, or even above, those reached by the particle accelerators. Such marvellous precision has become possible by my recent success in cooling molecules to ultracold temperature. That technique is the foundation of this proposal.
My plan is to decelerate a beam of ytterbium monofluoride molecules to rest using the forces exerted by carefully tuned laser light, trap these molecules and cool them to a few microkelvin. Then, I will load them into an array of traps formed by standing waves of light. The array contains millions of individual traps and isolates the molecules from one another, creating a pristine environment for measuring the electron's electric dipole moment. This measurement is done by watching how the spin of the molecules precesses in applied magnetic and electric fields, similar to the precession of a gyroscope or spinning top in a gravitational field. An electric dipole moment changes this precession rate, though only by the tiniest amount. That tiny change is detected more easily if the spin precesses for a long time. Because molecules are confined and isolated in the array, the time can be thousands of times longer than in current experiments. That makes my measurement scheme far more sensitive than any other experiment, allowing me to search for new physics with unprecedented precision.
Organisations
People |
ORCID iD |
| Jongseok Lim (Principal Investigator / Fellow) |
Publications
Athanasakis-Kaklamanakis M
(2025)
Slowing YbF molecules using radiation pressure
in Physical Review Research
Athanasakis-Kaklamanakis M
(2025)
Electron correlation and relativistic effects in the excited states of radium monofluoride.
in Nature communications
Athanasakis-Kaklamanakis M
(2024)
Radiative lifetime of the A ? 1 / 2 2 state in RaF with relevance to laser cooling
in Physical Review A
Collings F
(2025)
Low-noise environment for probing fundamental symmetries
in New Journal of Physics
Ho C
(2023)
Measuring the nuclear magnetic quadrupole moment in heavy polar molecules
in Frontiers in Physics
Ho C
(2023)
Systematic errors arising from polarization imperfections in measurements of the electron's electric dipole moment
in Physical Review Research
Peng G
(2025)
Large momentum transfer Raman atom interferometer without k -reversal
in Physical Review Research
Popa S
(2024)
Understanding Inner-Shell Excitations in Molecules through Spectroscopy of the 4 f Hole States of YbF
in Physical Review X
| Description | Meeting with South Korean Ambassador |
| Geographic Reach | Multiple continents/international |
| Policy Influence Type | Participation in a guidance/advisory committee |
| Description | Magnetometry for measuring the electric dipole moment of the electron |
| Amount | £46,404 (GBP) |
| Funding ID | ST/W005476/1 |
| Organisation | Science and Technologies Facilities Council (STFC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 12/2021 |
| End | 03/2022 |
| Description | Measuring the electron's electric dipole moment using molecules in a lattice |
| Amount | $1,200,000 (USD) |
| Funding ID | G-2023-21035 |
| Organisation | Alfred P. Sloan Foundation |
| Sector | Charity/Non Profit |
| Country | United States |
| Start | 12/2023 |
| End | 11/2028 |
| Description | Measuring the electron's electric dipole moment using molecules in a lattice |
| Amount | $900,000 (USD) |
| Funding ID | GBMF ID #12327 |
| Organisation | Gordon and Betty Moore Foundation |
| Sector | Charity/Non Profit |
| Country | United States |
| Start | 12/2023 |
| End | 11/2028 |
| Description | Testing fundamental physics using arrays of ultracold molecules |
| Amount | £920,790 (GBP) |
| Funding ID | MR/Z505122/1 |
| Organisation | United Kingdom Research and Innovation |
| Sector | Public |
| Country | United Kingdom |
| Start | 06/2024 |
| End | 07/2026 |
| Description | Ultra-low noise magnetic environments |
| Amount | £503,989 (GBP) |
| Funding ID | ST/Y509978/1 |
| Organisation | Science and Technologies Facilities Council (STFC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 03/2024 |
| End | 03/2027 |
| Description | Ultracold EEDM - Measuring The Electron's Electric Dipole Moment Using Ultracold Molecules |
| Amount | £2,222,103 (GBP) |
| Funding ID | EP/X030180/1 |
| Organisation | Engineering and Physical Sciences Research Council (EPSRC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 12/2023 |
| End | 11/2027 |
| Title | Electron correlation and relativistic effects in the excited states of radium monofluoride |
| Description | Experimental data included in the journal publication, Nat Commun 16, 2139 (2025). |
| Type Of Material | Database/Collection of data |
| Year Produced | 2025 |
| Provided To Others? | Yes |
| Impact | The research dataset can be used for further analysis of radium monofluoride molecule, which is a candidate for precision tests of fundamental physics. |
| URL | https://www.nature.com/articles/s41467-025-55977-w |
| Description | Interview for a magazine (Innovation News Network) |
| Form Of Engagement Activity | A magazine, newsletter or online publication |
| Part Of Official Scheme? | No |
| Geographic Reach | International |
| Primary Audience | Media (as a channel to the public) |
| Results and Impact | The activity was intended to introduce the funded project to the public through an article published in Innovation News Network, a magazine highlighting the latest innovations from the science, technology, and political spheres. |
| Year(s) Of Engagement Activity | 2021 |
| URL | https://www.innovationnewsnetwork.com/what-lies-beyond-the-standard-model-of-particle-physics/13296/ |
| Description | Mentoring to undergraduate/postgraduate students at UK universities |
| Form Of Engagement Activity | Participation in an activity, workshop or similar |
| Part Of Official Scheme? | No |
| Geographic Reach | National |
| Primary Audience | Postgraduate students |
| Results and Impact | 80 undergraduate/postgraduate students at UK universities attended the event held at UCL. I shared my research activities and personal experience as a research/academic in the UK coming from abroad and provided advice on career development. |
| Year(s) Of Engagement Activity | 2023 |
| Description | School Visit (London Korean School) |
| Form Of Engagement Activity | Participation in an activity, workshop or similar |
| Part Of Official Scheme? | No |
| Geographic Reach | Local |
| Primary Audience | Schools |
| Results and Impact | To approach and communicate the importance and excitement of science with the public, an underrepresented group in particular, I visited London Korean School as a Guest Teacher. With the theme of "What is the World Made of? - Atoms and Light", I introduced the concepts of atoms and light with simple demonstrations to about 20 pupils in Year 3 and Year 4 and their families. The pupils had made neverending questions, and the school reported positive feedback. I am developing the activity into a series of events in communication with the Director of Academic Affairs of the School. |
| Year(s) Of Engagement Activity | 2022 |