A Diamond Detector for Monitoring Of Neutron Irradiation and Criticality

Lead Research Organisation: University of Bristol
Department Name: Physics

Abstract

Novel detector instrumentation systems are required to support the operation and decommissioning of our nuclear power stations, either based on fission or fusion technologies. In this project, synthetic diamond will be used as a radiation detector for the measurement of gamma and neutron radiation.

This project will commercialise a well-proven detector which has been used to make measurements inside some of the most hazardous buildings in the world, where fissile and radioactive materials are present.

Based on diamond technology first used in the Large Hadron Collider, this commercialisation project will take the technology from operational proof-of-principle demonstrators developed by the University of Bristol and Sellafield (and used inside reprocessing tanks) to a series of products which will be operated as a service by Cavendish Nuclear Limited.

To achieve commercialisation, this project has solicited support from a wide range of industrial and academic partners in the UK, Japan and Italy. Each member of this international team brings specific expertise and facilities, from Kyoto University's nuclear research reactor, where we will demonstrate the detector's capability to measure the reactor's power output (through neutron flux measurement), to Sellafield's Highly Active Storage Tanks, in which we will demonstrate real-time high gamma dose rate measurement.

Our industrial partners have requested a focus on neutron detection, an important capability they are currently struggling to achieve using existing technology. Neutron detection will be important to prevent accidental criticality and recover from any such event. Our Japanese partners have specifically requested this capability to allow them to safely remove the fuel from within the stricken nuclear reactors at Fukushima Daiichi, and it will be useful in UK facilities safely containing fissile material. A Criticality Incident Detection System (CIDS) is needed in any industrial facility holding fissile material, to mitigate risks to personnel in the event of an accidental criticality. This must detect a criticality and continue to measure afterwards in case of knock-on events. Further testing and development are still needed, but the potential for superseding existing CIDS technologies with a cheaper, more compact and robust alternative is exciting. Neutron detection alongside gamma detection would be highly desirable: on-going pulsed/continuous criticality is not measured by any current devices after an initial event; and there are a multitude of applications in gloveboxes and large facilities for a portable system.

There is equally a need for rapid neutron detection in reactor core environments (fission and fusion), where the neutron flux is far more sustained and intense. Diamond is potentially very well-suited to such applications, with a proven sensitivity to thermal and fast neutrons better than that of gamma radiation. Accordingly, the aim of the current proposal is to develop a diamond detector system capable of detecting moderate-to-high neutron fluxes in real time, with the operator and detection electronics at a safe remote working distance. This will build on the software and hardware already developed for high-dose gamma measurement, increasing the value of the detection system. Such technology will be invaluable for Gen IV fission reactor concepts, including small modular reactors, as well as future fusion reactors, including JET, ITER and DEMO projects, and the UKAEA's recently announced Small Tokomak for commercial Energy Production (STEP) programme.

Longer term, the measurement of neutron energies through spectroscopy will help enable fusion technologies to become realistic. Not only can we use the diamond neutron detectors being developed in this project to measure the reactor power (as above), but we will also be able to demonstrate that the operational fusion reactor is self-sufficient in tritium by breeding its own fuel!

Publications

10 25 50
 
Description AWE high energy imaging partnership 
Organisation Atomic Weapons Establishment
Department National Nuclear Security Programme
Country United Kingdom 
Sector Public 
PI Contribution For the AWE we have been providing expertise on laser-driven gamma and neutron pulses as well as novel fast neutron imaging technologies using Diamond with a scintillation backing material. We are also supporting them in the establishment of a national high energy imaging facility.
Collaborator Contribution The AWE have co-funded a Royal Academy of Engineering professorial fellowship for me to run for 5 years until February 2021. This is a financial contribution of £50,000 per year, plus additional funding specifically for projects and secondments of members of my team.
Impact Outputs have inlcuded: - A modelling study report on the use of diamond for fast neutron imaging - Conducting a joint experiment at the LANSCE neutron facility in the USA to test deuterium infused diamond with a scintillator backing material as a fast neutron imaging material. - Undertaking a deuterium infusion study of diamond (at the AWE) to determine the deuterium (H-2) solubility as a function of pressure and temperature. The collaboration is ongoing and we will conduct further experiments in the next 12 months.
Start Year 2017
 
Description Cavendish Nuclear - detectors partnership 
Organisation Cavendish Nuclear
Country United Kingdom 
Sector Private 
PI Contribution We have been partnering with Cavendish (formally) in order to provide a commercial user and vendor of our diamond detector technologies. We are providing the technology and knowhow and they are providing a manufacturing and marketing capability once a commercialisation agreement is in place. We have also partnered with them to win a Radiometric Measurements framework contract from Sellfafield ltd. which includes utilisation of our detector prototypes.
Collaborator Contribution As above, Cavendish have offered to act as commercialisation partner and included us in their framework team in support of Sellafield.
Impact As above
Start Year 2019
 
Description Japan Atomic Energy Agency 
Organisation Japan Atomic Energy Agency (JAEA)
Country Japan 
Sector Public 
PI Contribution The grant award has led to the establishment of a strategic partnership with the JAEA based around fallout and fuel debris analysis. There has been an MoU signed by both institutions to permit collaboration, exchange of personnel and samples. Subsequently, the remit of the MoU has been widened (2019) to include joint work on diamond battery (ASPIRE) technology, high dose-rate diamond detectors and radiation mapping robots. We have contributed expertise, consultancy, shared data recorded from Japanese samples and sites and have won several experimental sessions at the Diamond Light Source synchrotron facility for fallout particle analysis. JAEA colleagues have participated in all of our UK synchrotron experiments and participated and presented at UK workshops and conferences e.g.
Collaborator Contribution Already we have had over 15 visits from the JAEA since the start of the partnership as well as a suite of fallout samples from Fukushima and access to nuclear fallout storage sites and other restricted areas of the Fukushima fallout zone. The site access and samples provided are extremely valuable.
Impact Several joint publications. Widening of the relationship to cover other areas such as radiation detection, UAVs and most recently diamond batteries.
Start Year 2016
 
Description UKAEA Detection and Metrology Team 
Organisation Culham Centre for Fusion Energy
Country United Kingdom 
Sector Academic/University 
PI Contribution In relation to the development of the STEP programme we have been sharing aspects of the technology so that they can consider the technology for us in STEP and other associated fusion projects where live neutron dosimetry data, for example in a breeder blanket module, is required to support plant operations.
Collaborator Contribution UKAEA have been providing us with advice as to the operational parameters (especially environmental conditions) that a diamond detector would need to work in to be a useful tool in a fusion powerplant.
Impact Professor Thomas Scott has been awarded a 5-year Royal Academy of Engineering Professorial Research Fellowship, co-funded by UKAEA, to develop the fusion fuel cycle. As part of this fellowship the diamond detector technology is being further supported and developed in partnership with UKAEA, who see it as a potential technology to use within the STEP fusion powerplant.
Start Year 2021
 
Description University of Kyoto - Fukushima collaboration 
Organisation University of Kyoto
Country Japan 
Sector Academic/University 
PI Contribution The two teams (Bristol and Kyoto) have formed a collaboration to research aspects of the fallout material ejected from the Fukushima reactor explosions in March 2011. Specifically, Bristol have applied advanced materials analysis techniques to samples of fallout material to determine its physical size, structure, morphology, elemental composition and isotopic signature. Bristol has also gained STFC funding and established a secure database for the collection, sharing and analysis of data relating to fallout materials collected from different regions of the Fukushima fallout zone
Collaborator Contribution The Kyoto side have provided analysis, by electron microscopy, gamma spectrometry and laser techniques to determine the size, activity and fluorescence characteristics of fallout materials to complement the Bristol data. They have also collected other particle/fallout analysis data from other research groups in Japan to add to the database.
Impact This collaboration is multi-disciplinary but mainly focused around materials analysis and radiation mapping. The collaboration has led to joint UK-Japan nuclear research projects funded by EPSRC and MEXT. It has also led to STFC funding to form a collaborative 'nuclear particle forensics' database. This partnership has also led to the development of a partnership between Bristol and the Japan Atomic Energy Agency (JAEA).
Start Year 2013