The helium atom in intense UV and XUV laser fields: rescattering-induced double ionization and ionization scaling laws
Lead Research Organisation:
Queen's University Belfast
Department Name: Sch of Mathematics and Physics
Abstract
At sufficiently high laser intensities, multi-electron atoms undergonon-sequential double ionization (NSDI), a process in which electronsare ejected near-simulteously in highly correlated (entangled) pairs.Helium, the simplest of all multi-electron atoms, presentstheorists with a unique opportunity to study these highly correlatedintense-field processes with an unprecedented accuracy. Despite therelatively simple structure of helium, the helium-laser Schroedingerequation, governing the dynamics of the system, admits few if anyapproximations in the limit of high intensity laser radiation. In theintense fields used to create NSDI, all terms of the helium-laserSchroedinger equation and all degrees of freedom are exercisedsimultaneously. The only reliable treatment of this problem has provedto be via high-accuracy numerical solution of the full Schroedinger equation.Over the last decade we have developed the computational methods, and thecomputer codes necessary to solve this problem on parallel computers.Our code is capable of solving the full (time-dependent and full-dimensional)helium-laser Schroedinger equation over a wide range of laserfrequencies and intensities. We have no rivals in this capability world-wide.Our code is still alone in its ability to generate accurate reliable solutionsat frequencies that range from the optical to the XUV, and atlaser intensities as high as can be achieved in practical experiments.Our intention is to calculate the detailed ionization dynamics of laser-drivenhelium in the UV to XUV range of laser wavelengths (roughly 100 nm to 7nm).In the intense field limit, this is very much uncharted territory,because until very recently it was impossible to build intense-fieldlasers at these wavelengths. Six months ago this changed with thecompletion of the first phase of DESY Free Electron Laser (FEL) nearHamburg. Another more ambitious FEL is under construction at Stanford.As just one illustration of the high importance of atom-laser physicsin this limit, we note a recent successful practical application of thenon-sequential double ionization (NSDI) mentioned above, in which trainsof light pulses of duration 100 attoseconds (the shortest everobserved) were created as a direct result of NSDI and used toperform time-resolved measurements of the same order. The laserused to drive the NSDI was 800nm. The prospect of producing evenshorter pulses by using intense UV lasers is a particularly exciting potentialapplication of laser-driven helium in the UV.
Organisations
Publications
Armstrong G
(2011)
Double-electron above-threshold ionization resonances as interference phenomena
in New Journal of Physics
Emmanouilidou A
(2011)
Direct versus delayed pathways in strong-field non-sequential double ionization
in New Journal of Physics
Nikolopoulos L
(2008)
Combined R -matrix eigenstate basis set and finite-difference propagation method for the time-dependent Schrödinger equation: The one-electron case
in Physical Review A
Parker J
(2009)
From the UV to the static-field limit: rates and scaling laws of intense-field ionization of helium
in Journal of Physics B: Atomic, Molecular and Optical Physics
Parker J
(2007)
Single-ionization of helium at Ti:Sapphire wavelengths: rates and scaling laws
in Journal of Physics B: Atomic, Molecular and Optical Physics