DEFECTS IN FRUSTRATED SYTEMS

Lead Research Organisation: Imperial College London
Department Name: Physics

Abstract

In a complex system made up of many smaller units, each element will interact with all of its neighbours, and the system tries to arrange itself so that the most favourable bond is formed with each neighbour. However, sometimes the neighbours have requirements that are mutually incompatible and a compromise must be found. If this is the case we describe the system as being frustrated. Frustration occurs widely in nature and is thought to be critical to our understanding of such questions as how do our brains work? and how do proteins fold? The frustrated biological systems described are so complex and so important that the science of frustration has become a major research area and there is great demand for simpler model systems where the interaction strength can be tuned, the model system size can be varied, defects can be introduced in a controlled manner and individual elements can be manipulated, removed or their individual state recorded. In such an ideal system one could unite theory and experiment and begin to understand the underlying physics within this complexity. Magnetic frustration has proved to be the most successful area for finding model systems. Traditionally these were magnetic crystals prepared by solid-state chemistry. However it has recently been shown that it is possible to use nanotechnology to make arrays of magnetic bars sufficiently small and sufficiently close together that the magnetic interactions between them becomes very significant, and that novel geometries can be designed where the magnetic interactions cannot all be satisfied. This development opens up broad new avenues of research in model frustrated systems. In solid-state chemistry one is limited by nature in the geometrical arrangements that are possible, whereas with nanotechnology any pattern that will tessellate can be fabricated into an array, on any length-scale down to the minimum feature size of the lithography. Here I propose to study such ideal systems that are based on frustrated magnetic nanostructures. Our experience from frustrated magnetic chemical structures tells us that triangles and hexagons are the building blocks that favour magnetic frustration. The initial work was done on arrays of magnetic bars that were isolated from one another, but I plan to focus on electrically continuous lattices, such as the hexagonal honeycomb structure so that electrical current can pass through it. The electrical properties of magnetic materials are sensitive to the magnetic structure and so this gives a direct probe of the frustrated structure and one can study its dynamic response to changes in temperature and magnetic field. Magnetic force microscopy (MFM) and scanning Hall probe imaging will be used to image the magnetic structure during these experiments. These in-situ measurements will allow the change in electrical response to be correlated directly with the change in magnetic structure, and will provide important information of the nature of the coupling between the magnetic and electrical properties of ferromagnetic metals, and the role of topology, which is currently very important for new spin-based electronics or spintronics technology. In addition to improving knowledge of diverse other fields, the magnetic arrays that I will make are exciting in their own right. Their unusual and sensitive response to magnetic fields might be useful in sensors. Furthermore the strong coupling between all the elements, and the fact that the magnetic state of individual elements can be both written (changed by applying a magnetic field) and read, means they could potentially be used for novel types of computation, often described as neural networks because they work more like the brain than like a conventional computer.

Publications

10 25 50
 
Description The goal of this project was to engineer arrays of ferromagnetic bars to induce a type of magnetic frustration known as the Ice rules. The Ice rules were initially used to describe the disorder in the hydrogen ion position in water ice, which has finite residual entropy at zero temperature. They also describe the local ordering principle of the spin in spin ice materials such as Ho2Ti2O7 and certain arrays of ferromagnetic nanobars "artificial spin ice." We discovered that we were able to observe magnetic monopole defects in artificial spin ices using magnetic force microscopy. We also discovered that we can control the direction that the magnetic charges move through the arrays be using magnetic fields, and also by exploiting a property of domain walls knows as their chirality. We also found that the arrays exhibit rather unusual collective behaviour at low temperatures which might a new way to store data.
Exploitation Route Domain wall manipulation technologies are becoming widespread commercial products, such as in the spin transfer torque based MRAM devices. Our work using domain wall chirality to control of the magnetic charge propagation through artificial spin ice (Nature Scientific Reports 2013) has moved the work much closer to domain-wall spintronics applications, as illustrated by the very similar findings of the IBM group on artificial spin ice later in the same year. (Pushp, Nature Physics 2013). These applications are at the forefront of energy efficient computation. Our work also has more general application in furthering capability in nanofabrication of magnetic devices and in particular understanding how to limit and control the interactions between magnetic devices at the nanoscale. We have developed a new technique for manipulating the magnetic state of nanostructures, Magnetic Topological Writing (Nature Nanotechnology 2018.)
Sectors Digital/Communication/Information Technologies (including Software),Energy,Environment,Manufacturing, including Industrial Biotechology

URL https://www.imperial.ac.uk/people/w.branford
 
Description There has been widespread public interest in our work on magnetic monopoles and low temperature phases in artificial spin ice. For example the press release of magnetic monopoles has had >22000 views and the copy of the video story we made on the Imperial YouTube channel has had >18000 hits. (https://www.youtube.com/watch?v=l5xSjCePgEQ) The story was covered by the newspaper Spiegel and by websites including 'PhysOrg, Science Daily, Insciences, PopSci and pro-physik. The Science story on collective phenomena has had >2300 views on the imperial website and was highlighted on the EPSRC website. https://www.epsrc.ac.uk/newsevents/news/sciencejournal/
First Year Of Impact 2012
Sector Other
Impact Types Societal

 
Description EPSRC coverage of Low Temperature Artificial Spin Ice 
Form Of Engagement Activity A press release, press conference or response to a media enquiry/interview
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Media (as a channel to the public)
Results and Impact The Science story on collective phenomena has had <2300 views on the imperial website and was highlighted on the EPSRC website.
Press release:
http://www3.imperial.ac.uk/newsandeventspggrp/imperialcollege/newssummary/news_30-3-2012-15-43-46
Year(s) Of Engagement Activity 2012
URL https://www.epsrc.ac.uk/newsevents/news/sciencejournal/
 
Description Public engagement online 
Form Of Engagement Activity A press release, press conference or response to a media enquiry/interview
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Public/other audiences
Results and Impact There has been widespread public interest in our work on magnetic monopoles and low temperature phases in artificial spin ice. For example the press release of magnetic monopoles has had >22000 views and the copy of the video story we made on the Imperial YouTube channel has had >18000 hits.
(https://www.youtube.com/watch?v=l5xSjCePgEQ)
The story was covered by the newspaper Spiegel and by websites including 'PhysOrg, Science Daily, Insciences, PopSci and pro-physik.
Year(s) Of Engagement Activity 2011,2012,2013
URL http://www.youtube.com/watch?v=l5xSjCePgEQ