Positronium - Matter Interactions

Lead Research Organisation: University College London
Department Name: Physics and Astronomy

Abstract

The observed imbalance between matter and antimatter in our universe is one of the greatest mysteries in science. Positrons are the antimatter counterpart to electrons with which they annihilate releasing gamma-rays. In addition to their importance in our fundamental understanding of nature, studies of their interactions with ordinary everyday matter allow us, for example, to investigate crystal structures and to obtain functional images of human organs using the medical technique of positron emission tomography (PET). In many collisions of positrons with matter, positronium (Ps) is formed.

Positronium is a composite made of a positron and electron, analogous to the hydrogen atom with the positron replacing the proton. So often is Ps formed, that e.g. 80% of gamma-rays detected in PET, and 95% of all gamma-rays released from the galactic centre of the Milky Way are the result of Ps decay. Once formed, it has ample time to interact with matter before annihilating because its lifetime, although of the order of nanoseconds, is still millions of times longer than typical scattering times. For these reasons, knowledge of how Ps itself interacts with matter is important not only for collision physics but also, for example, so that we may improve radioprotection in PET, or learn about the environment in which positrons annihilate in outer space.

Since both experimental and theoretical studies with Ps projectiles are difficult, corresponding data are scarce or non-existent. Recently, however, we have discovered that positronium scatters from a wide variety of atomic and molecular targets in a similar manner to that of a bare electron at a given projectile velocity. This is not what was expected! And, whilst the reason is unclear, its ramifications at a fundamental and practical level might be far reaching. It looks like the positron in Ps is heavily screened (or "cloaked") from the target by its partner electron and we wish to understand why. In the process, through the proposed research, we shall charter the outcome of such collisions and glimpse into the formation of Ps resonances and possibly Ps compounds. From a practical viewpoint, the outcome of the project may feed directly into models of how Ps interacts with matter, encompassing interstellar clouds and the human body.

Planned Impact

The outcomes of the proposed studies are expected to impact primarily on the academic sector through the supply of unique data and to aid the understanding of atomic interactions involving antimatter. However, it is envisaged that our results will also serve as an input, for example, into simulations of Ps collisions with matter including industrially important materials and biological tissue.

Thus potential beneficiaries of the proposed research outside the academic sector may include those working, for example, in the materials and nuclear medicine industries, and of course their customers and patients. In particular for Positron Emission Tomography, an improved understanding of the microscopic distribution of the energy deposits along the positron tracks may result in improvement of imaging-resolution and more accurate radiation dosimetry. In the longer term, an advance of this type, leading to the development of better protocols for radioprotection and cancer radiotherapy, could benefit public health and hence society.

Economic benefits are also expected to arise for the public and private sectors through the training of talented young scientists in performing highly-skilled research and developing concomitant transferrable skills (e.g. numerical and computational, problem-solving, creative, communication, leadership) which are highly valued by businesses and organizations. Past group members have found employment in national and international laboratories, government departments, software development, scientific consulting and the finance sector, as well as in academia.

Research with antimatter continues to excite the imagination of the general public and mass media (from the matter-antimatter asymmetry to the recent discovery of antimatter-production in thunderstorms on Earth). It thus represents a powerful vehicle for stimulating further interest and promoting understanding in physics and science, especially among young people. In the framework of the departmental "Science for the Public" initiatives, we shall endeavour to promote public awareness and engagement with our research by delivering popular lectures, talks at schools and interested societies and through popular publications (e.g. last November our work featured in New Scientist and Physics World).

Publications

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Brawley S (2012) Electron-like and resonant scattering of positronium in Journal of Physics: Conference Series

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Brawley S (2012) The production of positronium and its resonant scattering in Journal of Physics: Conference Series

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Brawley SJ (2015) Positronium Production and Scattering below Its Breakup Threshold. in Physical review letters

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Fayer S (2015) Positronium beam production and scattering at low energies in Journal of Physics: Conference Series

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Laricchia G. (2012) Positronium collision physics in RIVISTA DEL NUOVO CIMENTO

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Schippers S (2019) Roadmap on photonic, electronic and atomic collision physics: II. Electron and antimatter interactions in Journal of Physics B: Atomic, Molecular and Optical Physics

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Shipman M (2017) Resonant scattering of positronium as a quasifree electron in Physical Review A

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Shipman M (2014) Collimated positronium production from gases in The European Physical Journal D

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Shipman M (2012) Production of collimated positronium by positron scattering from CO2, N2 and Xe in The European Physical Journal D

 
Description As well as probing matter-antimatter interactions, positrons (as positive electrons) have been employed to highlight charge and mass effects in the dynamics of collisions, including those resulting in the ionization of atoms and molecules. Positronium (Ps), the hydrogenic atom formed from the binding of a positron and an electron, is readily produced in the scattering of positrons from matter. Ps is quasi-stable with a lifetime against annihilation dependent upon its spin: ground-state para-Ps (1 1S0) has a lifetime t ? 125 ps, whilst ortho-Ps (1 3S1) is considerably longer lived (t ? 142 ns). The beam employed for the scattering work discussed in this chapter consists solely of ortho-Ps atoms. In a dense medium, Ps may undergo several cycles of formation and break-up prior to the annihilation of the positron. A quantitative understanding of this cycle is important also for practical applications such as nanodosimetry relating to positron emission tomography (PET). We have developed experimental methods to investigate positron and positronium impact ionization and fragmentation in collision with atoms and molecules, and associated results. In the case of positrons, an extensive database now exists of integral cross sections for the inert atoms, less so for molecules; differential data remain sparse . Our focus has been on the latter two topics as well as studies with positronium projectiles.

Cross-sections for positron-impact ionization leaving either the resultant ion or positronium atom in an excited state are presented. For atomic targets, excited-state positronium contributes significantly to the positronium formation cross-section, while for CO2 and N2 it appears suppressed. Instead, for these targets large cross-sections for ionization-excitation are noted.

Following our findings (Brawley et al. Science 330 2010) concerning the similarity in shape and magnitude of the total cross-sections for equivelocity Ps atoms and electrons, enhancements have been observed in the Ps total cross-section for CO2 at velocities close to those at which resonances occur in the case of electrons. Further comparisons are made between theoretical results for Ps scattering and experimental electron total cross-sections.

New data for positronium beam production efficiency are presented. As a converter of positrons to forward-going positronium, O2 has been found to be as good as CO2 from ~250 to 400 eV. Preliminary data is also presented for the production efficiency from Ar at 2.8 eV.

The first absolute experimental determinations of the differential cross sections for the formation of ground-state positronium are presented for He, Ar, H2, and CO2 near 0°. Results are compared with available theories. The ratio of the differential and integrated cross sections for the targets exposes the higher propensity for forward emission of positronium formed from He and H2.
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A new electrostatic positron beam at UCL is described. The beam incorporates a re-moderator to achieve brightness enhancement, time of flight facility for beam energy determination and improved signal to background ratio and a position sensitive detector for 2-D imaging of the beam spot. The apparatus is being employed for measuring the total cross section of positron scattering from krypton and helium in the energy range of (10 - 200) eV. Results will be presented at the conference.

We are now able to produce a positronium beam at energies in the range 1 - 400 eV, significantly lowering the previously achievable minimum of ~ 7 eV and opening up the possibility of investigating subtle quantum mechanical effects such as those which give rise to low energy electron scattering phenomena (e.g. resonances and 'barrier transparency').

Recent findings on the similarity between electron and positronium scattering at the same velocity [Brawley et al., Science 330, 789 (2010)] have guided us towards the realization of a detectable flux of positronium atoms at beam energies five times lower than previously obtained, enabling total cross sections to be measured in the energy range ~(1-7)
eV for the first time. In collision with Ar and Xe, the total cross sections of positronium are found to be smallest at the lowest energy probed, approaching those of the Ramsauer-Townsend minima for electron projectiles. Additional structure has been observed in the case of positronium scattering at incident energies around 5 eV.

In order to clarify the physics underlying the observations of the electronlike behavior of positronium (Ps) and its resonant scattering from CO2, we have measured the Ps+N2
total cross section and found it also to exhibit significant structure. Analysis of the resonances reveals that Ps is distorted in the collisions and classical trajectory Monte Carlo calculations indicate that the electron is on average closer to the target than the positron, which may in turn bind resonantly to the ensuing temporary negative ion. This description of the nature of Ps resonances agrees with long-standing theoretical predictions.
Exploitation Route The main beneficiaries of the outcomes of our research will be primarily other scientists, especially theorists who will use our experimental data to test their hypotheses , modellers of astrophysical events , plasma diagnostics and radiobiological processes who input cross-section data in their computations. In this respect, there is currently an international drive towards the development of accurate dosimetry for Positron Emission Tomography (PET), data for molecules of biological significance being particularly sought after for simulations of positron tracks in biological media. The clear motivation is that an increased understanding will lead to reduced damage of healthy tissue and, potentially, to efficient targeting (e.g. of cancerous growths). We regularly receive requests to provide cross-section data and we will alert scientists working in this field to our new findings as they emerge.
Sectors Chemicals,Environment,Healthcare

URL http://www.ucl.ac.uk/positron-physics/title.html
 
Description Positrons and positronium are fundamental to our understanding of the physical universe. They have also become exceptionally powerful in the biomedical industry and useful in practical applications ranging from material science to engineering . The main beneficiaries of the outcomes of our research are primarily other scientists, including modellers of astrophysical and radiobiological processes as well as plasma diagnostics . Benefits arise for the public/industrial sector also through the training of talented young scientists in performing world-class science and in developing a variety of skills (e.g. problem-solving, creative, communication, etc), crucial in innovative endevours in academia and industry. Recent members of the group are now working at prestigious research labs (e.g. CERN, RIKEN, ETH) , in the UK Industry (e.g. Health Protection Agency, BAE Systems Detica, Thermo Fisher Scientific) and the financial sector. Antimatter is a powerful vehicle for stimulating interest and promoting understanding in physics and science by the general public and especially by young people. In the framework of the departmental "Science for the Public" initiatives, we endeavour to generate public awareness and engagement through popular publications and by delivering popular lectures / talks at schools or interested societies.
Sector Chemicals,Education,Environment,Healthcare
Impact Types Cultural,Societal,Economic

 
Description Standard Research
Amount £560,729 (GBP)
Funding ID EP/P009395/1 
Organisation Engineering and Physical Sciences Research Council (EPSRC) 
Sector Public
Country United Kingdom
Start 11/2016 
End 10/2019
 
Description Aarhus University 
Organisation Aarhus University
Department Department of Physics and Astronomy
Country Denmark 
Sector Academic/University 
PI Contribution Testing the efficiency and characteristics of thin-film single-crystals to positron moderation and remoderation and training of student
Collaborator Contribution Provision of thin-film single-crystals for positron moderation and remoderation and secondment of student
Impact Magnetic field-free measurements of the total cross section for positrons scattering from helium and krypton S. E. Fayer, A. Loreti, S.L. Andersen, A. Kover and G. Laricchia J. Phys. B 49 (2016) 075202 http://iopscience.iop.org/0953-4075;jsessionid=45F26BC909B9E8C22C53723A042F5855.c1.iopscience.cld.iop.org Moderation and diffusion of positrons in tungsten meshes and foils A. I. Williams, D. J. Murtagh, S. E. Fayer, S.L. Andersen, J. Chevallier, A. Kover, P. Van Reeth , J.W. Humberston and G. Laricchia J. Appl. Phys. 118 (2015) 105302 An electrostatic positron beam for atomic and molecular collision experiments S E Fayer, A Loreti, A Kover, S L Andersen and G Laricchia Journal of Physics: Conference Series 635 (2015) 052070 http://iopscience.iop.org/article/10.1088/1742-6596/635/5/052070/meta http://scitation.aip.org/content/aip/journal/jap/118/10/10.1063/1.4930033
Start Year 2011
 
Description IOP Conference of Physics and Astronomy Students 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Undergraduate students
Results and Impact Every year a university in the UK hosts the Conference of Physics and Astronomy Students, an Institute of Physics event. The stated aims are that "undergraduate students learn about the exciting cutting edge research undertaken by both distinguished professors from around the country and fellow physics colleagues alike; all the being able to network and get to know the other attendees through the various planned social events". I was invited by the Student Organizing Committee to deliver a 1-hr lecture on my research interests entitled "Collision involving antimatter".
Year(s) Of Engagement Activity 2017
URL http://www.ucl.iopcaps.co.uk/#theconference
 
Description Szeged 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Annual Congress of the Hungarian Physical Society. Receipt of the award of an Honorary Fellowship of the Roland Eotvos Physical Society of Hungary.
Year(s) Of Engagement Activity 2016
URL http://titan.physx.u-szeged.hu/fizikus_vandorgyules_2016/node/6
 
Description UCL MAPS Website 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Public/other audiences
Results and Impact Revealed: positronium's behaviour in particle billiards
Collision physics can be like a game of billiards. Yet in the microscopic world, the outcome of the game is hard to predict.
Fire a particle at a group of other particles, and they may scatter, combine or break apart, according to probability distributions governed by quantum mechanics. These processes can tell us about fundamental properties of matter and, if antimatter projectiles are used, also about matter-antimatter interactions. Scientists at UCL have finally answered one of the basic questions that has remained outstanding until now: if, in a collision with matter, a positron - the antimatter counterpart of electrons - captures an electron, in which directions are the two likely to travel, and with what probability?
All matter particles - electrons, protons, neutrons - have an antimatter counterpart. Antiparticles have very similar properties to particles, but the opposite electrical charge. Although they are eventually annihilated when they come into contact with matter, antiparticles can briefly interact with particles to form very short-lived matter-antimatter hybrids, atoms in which one of the component particles has been replaced with an antiparticle. Of these, positronium - one electron and one positron in orbit around each other - is the most studied.
"Positrons and positronium are important for our understanding of the physical universe," says Gaetana Laricchia (UCL Physics & Astronomy), who led the study. "They are also useful for applications such as probing the properties of materials, as well as for medical diagnostics. Yet there is much that we still do not know about their interactions with ordinary matter."
In the study, published in the journal Physical Review Letters, Laricchia and colleagues have used UCL's Positronium Beam - a facility unique in the world - to investigate the behaviour of the positronium as it is created, and have finally been able to compare with theoretical predictions which have been developed over the past 40 years.
The Positronium Beam works by producing a beam of positrons from a radioactive source, passing it through a chamber full of hydrogen, where the positrons bind to electrons to form positronium. The resulting beam of positronium is then usually used to bombard other targets placed downstream. In this study, though, the team examined the formation of the positronium atoms themselves - much like using a microscope to study the way light passes through lenses.
"From the collision, the positronium atoms may emerge forward, sideways or backwards. The absolute proportions had never been measured," says Laricchia. "We sought to analyse this because it tells you important information about how positrons collide in gases, how positronium behaves once it has formed and because it is a very sensitive test of theoretical models."
As well as the hydrogen gas that is usually used in the Positronium Beam, the team also measured the emission of positronium created when hydrogen was replaced with argon, helium and carbon dioxide. They found that in the case of helium and hydrogen, the emission of positronium was broadly in line with a small subset of theories; for argon, the behaviour seems similar to that created in hydrogen and helium and quite different from theoretical predictions. For CO2, there is no prediction to test, and this experiment provides the first data of any kind.
In all four cases, there was a strong preference for the positronium to be emitted in the forward direction, particularly when the positrons were hitting the gas at high speed.
The team hope to carry out further investigations of positronium formation, particularly at lower energies which should provide even better calibration for the theoretical models
Year(s) Of Engagement Activity 2015
URL http://www.ucl.ac.uk/mathematical-physical-sciences/maps-news-publication/maps1539
 
Description UCL MAPS Website 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Public/other audiences
Results and Impact First direct sightings of low-energy positronium collisions

Positrons are the antimatter counterpart to electrons with which they annihilate releasing gamma-rays. In addition to their importance in our fundamental understanding of nature, studies of their interactions with ordinary everyday matter allow us, for example, to investigate crystal structures and to obtain functional images of human organs using the medical scan technique of positron emission tomography (PET). In many collisions of positrons with matter, positronium (Ps) is formed.

Positronium is a hybrid made of a positron and an electron, analogous to the hydrogen atom with the positron replacing the proton. So often is Ps formed, that e.g. 80% of gamma-rays detected in PET, and 95% of all gamma-rays released from the galactic centre of the Milky Way are the result of Ps decay.

Once formed, Ps has ample time to interact with matter before annihilating because its lifetime, although of the order of nanoseconds, is still millions of times longer than typical scattering times. For these reasons, knowledge of how Ps itself interacts with matter is important not only for collision physics but also, for example, so that we may improve radioprotection in PET, or learn about the environment in which positrons annihilate in outer space.

UCL researchers have now generated an energy-tunable beam of Ps atoms at energies five times lower than ever obtained before and made direct measurements of Ps scattering probabilities within the range 1.4-7 eV for the first time.

In the study, just published in the journal Physical Review Letters, Gaetana Laricchia and her team have found that the probabilities of Ps scattering from argon and xenon decrease with decreasing energy in a similar way to that of electron projectiles for which a quantum mechanical phenomenon (the Ramsauer-Townsend effect) results in "target transparency". Professor Laricchia explained that this result contradicts the available predictions and poses a significant challenge to theories.

The work will aid scientists in better understanding the subtle collision effects for low energy Ps, its fundamental properties and develop accurate descriptions of matter-antimatter interactions and atomic collisions in general.
Year(s) Of Engagement Activity 2015
URL http://www.ucl.ac.uk/mathematical-physical-sciences/maps-news-publication/maps1560
 
Description Women's day seminar invitation 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach Local
Primary Audience Postgraduate students
Results and Impact Spectroscopy and Dynamics 'Supergroup' seminars for several chemistry department research groups to an audience of approx. 30 people.
Year(s) Of Engagement Activity 2019