Large deviations and dynamical phase transitions in open quantum systems: from mathematical theory to physical applications

Lead Research Organisation: University of Nottingham
Department Name: Sch of Mathematical Sciences

Abstract

We are currently entering a new technological era where quantum mechanics is used not only to predict physical behavior, but increasingly to exploit quantum resources in applications such as quantum communication and computation and quantum metrology. The last couple of decades have witnessed a revolution in the experimental realisation of quantum systems. Ultracold atomic gases are nowadays routinely created and used for the study of complex many body phenomena such as quantum phase transitions shedding light on open problems in condensed-matter physics.

Real quantum systems are "open" in the sense that they interact with their environment (be it a thermal bath or other components of a larger quantum system). This leads to an irreversible loss of coherence and to energy dissipation. The simplest analysis applied to this kind of problems is based on the Markov approximation in which the environment possesses no memory and interacts weakly with the system. The Markov formalism has been successfully applied to many physical problems, such as the treatment of continuous-time measurements and the existence of "quantum jumps". This lead to the development of the "quantum trajectories" theory describing the stochastic dynamics of quantum systems, conditioned on the random outcomes of indirect observations. Current advances in quantum engineering drive theoretical and experimental research towards a new synthesis of quantum dynamics and classical control engineering, called quantum control theory. The Markov set-up is perfectly suited for applying feedback control techniques, where a classical or quantum output signal is processed in real time and used to act back on the system according to a control strategy.

The quantum trajectories formalism is naturally connected to classical non-equilibrium statistical mechanics. Recently there has been much progress in our understanding of non-equilibrium systems, with many advances originating from the study of complex soft condensed-matter systems such as glasses. The mathematical language of statistical mechanics is large deviations (LD) theory, which was traditionally applied to the study of equilibrium phases and phase changes in many body systems. The LD formalism is now used to investigate the dynamical phases in non-equilibrium systems by treating ensembles of trajectories in the same way that equilibrium statistical mechanics treats ensembles of configurations. Important properties of classical non-equilibrium systems can be uncovered by exploiting this analogy. This new set of ideas and techniques has not yet been fully exploited in the quantum realm, and therefore much less is understood of quantum non-equilibrium dynamics. In this proposal we aim at building the mathematical foundation and identifying fundamental principles that will eventually allow us to construct a framework for a detailed and thorough description of quantum matter out of equilibrium.

The central goal of this proposal is to develop the LD theory of open quantum systems and use it to explore the phenomena of metastability and dynamical phase transitions. We aim to bridge the gap in understanding that exists between classical and quantum non-equilibrium systems, by applying and extending the most novel methods developed in non-equilibrium statistical mechanics, the theory of quantum Markov processes and stochastic Schrödinger equations. In parallel to developing the mathematical theory we will perform a detailed analysis of physically relevant models such as driven many-body systems and the micromaser. By combining statistical and probabilistic methods of Markov processes with quantum feedback control theory, we will study the large and moderate deviations behaviour of systems coupled with classical or quantum controllers, and apply the theory to topics such as system identification and quantum metrology.

Planned Impact

The proposed work is fundamental research. It is part of a plethora of worldwide activities which aim at understanding matter far from equilibrium. There is a strong belief that understanding and controlling matter in non-equilibrium states underpins both new science and new technologies. In this work we aim at building the mathematical foundations and identifying fundamental principles that will eventually allow us to construct a framework for a detailed and thorough description of quantum matter out of equilibrium. This will pave the way for the understanding and classification of non-equilibrium phenomena in the same spirit as statistical mechanics describes equilibrium systems. The insights gained from applying this methodology will potentially allow the design of new materials with yet unseen properties, e.g. highly efficient solar cells or ultrafast electronics. The proposed research will impact in the short-term on the UK society through advancement of our knowledge and understanding of nature and in the long-term through new potential technologies which could revolutionise e.g. energy production, transport, communications and quality of life as a result over the years to come.

Indeed, it is believed that the "second quantum revolution" will be responsible for most of the key physical technological advances in the XXI century. The UK boasts a strong research-active environment in theoretical and experimental aspects of Quantum Information and Technology. Our project will strengthen its position in areas such as non-equilibrium quantum dynamics and quantum control in which UK is underrepresented compared to France, Germany, Australia, Japan and US.

An integral part of the planned research is the envisaged strong collaboration with researchers of external research institutions. This serves a dual purpose: the project team will benefit from the expertise of some of the best researchers from the different fields involved in the project; and it creates awareness and engagement of scientists inside and outside the UK.

In terms of dissemination to the wider academic community we will pursue well established routes. We will provide seminar talks, workshop and conference presentations as well as publications in high impact journals such as Science, Nature, Phys. Rev. Lett., as well as open access journals such as New Journal of Physics and Physical Review X. The involvement of the academic community is a strategic step on the pathway from fundamental research to more applied research and from there into industry.

Both the Schools of Mathematics and Physics & Astronomy in Nottingham organise Open Days on a regular basis. These bring pupils into close contact with current research topics. This is essential to generate awareness for the complexity of processes in nature and to create curiosity, which is one of the driving forces for the development of a modern society. The team members will actively participate in this activity by giving lab tours and short presentations.

We will engage with the wider public by outreach activities such as presentations on the British Science Festival, a project webpage, and use of social media. This will help to motivate the need for fundamental research in the public and create enthusiasm for the physical sciences. At present, a very successful initiative for creating public awareness of science is the Sixty Symbols project of the University of Nottingham (www.sixtysymbols.com) of short films aimed at explaining physics to the general public.

Publications

10 25 50
 
Description The concept of phase transition is central to our understanding of a broad spectrum of phenomena in statistical mechanics, from transitions between gas, liquid and solid phases in thermodynamics, to transitions between ferromagnetic and paramagnetic phases of magnetic materials. The underlying mathematical theory is that of large deviations, dealing with the rare events of exponentially small probabilities.

Inspired by the successes of modern non-equilibrium statistical mechanics, the central goal of this proposal is to develop the large deviations theory of open quantum systems, i.e. systems in contact with the environment, and use it to explore the phenomena of metastability, and dynamical phase transitions. Quantum systems are very sensitive to interaction with the environment, leading to undesired effects such as decoherence and dissipation. Understanding such systems is therefore key for the successful implementation of quantum technology applications such as quantum computation, quantum simulation and quantum metrology.

Our first set of results includes a rigorous analysis of large deviations, dynamical phase transitions, and central limit theorems in a well known quantum dynamical system, the atom maser [1]. A detailed analysis of the system identification problem for the atom maser is carried out in [2,3]. This puts the basis of a general theory of system identification and local asymptotic normality [4], which extends results from the classical theory of hidden Markov chains to the quantum domain. In parallel to the general theory, our team has investigated several condensed matter interacting systems, such as a generalised Dicke model of dissipative spins coupled to phonon modes [5], spin chains with long range interactions [6] and single ion sources from a dipole-blockaded atomic ensemble [7]. A exciting ongoing direction is to exploit dynamical phase transitions occurring in open systems to achieve quantum enhanced precision in the measurement of dynamical parameters such as a phases, coupling parameters, hamiltonians or external fields [8]. The idea is that dynamical outputs (e.g. emitted photons) of systems at a phase transitions can exhibit superposition of macroscopically different states, which allows for the estimation of relative phase with precision close to the absolute quantum limit, or Heisenberg limit.


References:

[1] M. van Horssen, M. Guta, Large Deviations, Central Limit and dynamical phase transitions in the atom maser, arXiv:1206.4956

[2] C. Catana, M. van Horssen and M. Guta
Asymptotic inference in system identification for the atom maser
Philosophical Transactions of the Royal Society A 370, 5308-5323 (2012)

[3] Catalin Catana , Theodore Kypraios , Madalin Guta, Maximum likelihood versus likelihood-free quantum system identification in the atom maser. Journal of Physics A: Mathematical and Theoretical 47, 415302 (2014)

[4] M. Guta and J. Kiukas, Equivalence classes and local asymptotic normality in system identification for quantum Markov chains, arXiv:1402.3535, to appear in Commun. Math. Phys.

[5] S. Genway, W. Li, C. Ates, B. P. Lanyon and I. Lesanovsky
Generalised Dicke non-equilibrium dynamics in trapped ions, Physical Review Letters 112, 023603 (2014)

[6] E. Levi and I. Lesanovsky, Non-classical correlations in a class of spin chains with long-range interactions and exactly solvable ground states New Journal of Physics 16, 093053 (2014)

[7] C. Ates, I. Lesanovsky, C. S. Adams, and K. J. Weatherill, Fast and quasideterministic single ion source from a dipole-blockaded atomic ensemble
Physical Review Letters 110, 213003 (2013)

[8] C. Catana and M. Guta, Heisenberg versus standard scaling in quantum metrology with Markov generated states and monitored environment, Phys. Rev. A 90, 012330 (2014).
Exploitation Route The project is primarily focused on developing a mathematical and theoretical physics framework for dynamical quantum phase transitions. As this framework is built up, the next step is to explore concrete, realistic experimental implementations with a view on quantum technologies (sensing and metrology).
Sectors Aerospace, Defence and Marine,Digital/Communication/Information Technologies (including Software)

 
Description The impact of the proposal's results is primarily on academia, more concretely at the interface between quantum information, statistics and probability, and quantum technology. More specifically: - paper [1] has been highly influential in the quantum open dynamics community and received 125 citations (Google Scholar March 2022). The - paper [2] opened a new area of research at the intersection of quantum metrology and continuous time measurements with potential practical applications in high precision metrology - paper [3] is the first to develop fundamental mathematical theory of information geometry for quantum Markov chains [1] Towards a theory of metastability in open quantum dynamics K Macieszczak, M Guta, I Lesanovsky, JP Garrahan Physical review letters 116 (24), 240404 [2] Dynamical phase transitions as a resource for quantum enhanced metrology K Macieszczak, M Guta, I Lesanovsky, JP Garrahan Physical Review A 93 (2), 022103 [3] Information geometry and local asymptotic normality for multi-parameter estimation of quantum Markov dynamics M Guta, J Kiukas Journal of Mathematical Physics 58 (5), 052201
Sector Other