Hybrid Cavity-QED with Rydberg Atoms and Microwave Circuits

Lead Research Organisation: University College London
Department Name: Physics and Astronomy

Abstract

Atoms and molecules in highly-excited Rydberg states can exhibit very large electric dipole moments, on the order of 1000 Debye. These large dipole moments make them very well suited to studies of light-matter interactions at microwave frequencies, and long-range dipolar interactions in free-space and close to surfaces. They also make samples in high Rydberg states states very amenable to manipulation and trapping using inhomogeneous electric fields.

The recent development of a new chip-based experimental architecture which exploits these large electric dipole moments to control the translational motion and internal quantum states of Rydberg atoms and molecules close to surfaces has opened up new opportunities in (i) the development of hybrid approaches to quantum information processing in which gas-phase and solid-state systems are combined, (ii) studies of long-range interactions between Rydberg atoms/molecules and surfaces, and (iii) the preparation and study of gas-phase molecular samples at low temperatures. In the work described in this proposal it is planned to exploit, and further develop, this architecture, in a manner which encompasses the first two of these areas, to perform experiments in a setting which can be described as a hybrid between traditional cavity-quantum-electrodynamics (cavity-QED), involving three-dimensional resonators and two-level quantum systems in the gas-phase, and purely solid-state circuit-QED.

To achieve this helium atoms will be prepared in long-lived, circular Rydberg states. These states will then be coupled to microwave fields in the vicinity of chip-based co-planar microwave waveguides to study their coherence times and long-range Rydberg-atom--surface interactions. The off-resonant interaction of these atomic samples with chip-based superconducting microwave resonators will then be exploited for the realisation of new chip-based devices for non-destructive detection of the Rydberg samples.

In the long term it is foreseen to use the gas-phase Rydberg atoms in this hybrid system as long-coherence-time quantum memories which are coupled via the chip-based microwave resonators to superconducting circuits in which fast operations can be performed. In this way, the challenges associated with exploiting each system individually for applications in quantum information processing will be circumvented.

Planned Impact

The research described here involves bringing together gas-phase and solid-state quantum systems for fundamental studies of atom/molecule-surface interactions and the development of new chip-based devices for the non-destructive detection of atoms and molecules. This work represent the stepping stones toward the future implementation of hybrid approaches to quantum information processing in which gas-phase atoms are used as long-coherence time quantum memories that are coupled via chip-based microwave resonators to superconducting circuits in which fast operations can be performed. Hybrid approaches, of this kind, to quantum information processing seek to combine two complimentary quantum systems to overcome potential limitations associated with each individual system in terms of their coherence times, scalability, or the rate at which operations can be preformed. From this perspective the research described will contribute to the UK-based development of new quantum technologies. As outlined in the outcome of the 'EPSRC Grand Challenges Survey', in addition to the economic benefit arising from the development of new high-tech industries based upon quantum technologies, there is significant potential for impact in society given the role that electronic devices play in our lives today.

Further impact of this research is associated with the education and training of undergraduate and graduate students, and postdoctoral researchers in the skills necessary to make a significant contribution to, and lead, future developments in the UK (i) in academic research, (ii) in research and development in industry, in particular in the identification and manufacture of new quantum devices, and (iii) in analysis and risk assessment in the financial services sector. With the growing importance of new quantum technologies in society today, the training of personnel with appropriate skills to contribute to and support this area in the UK, in government research laboratories and in the industrial sector, is essential.

The unusual and often surprising properties of quantum systems, of the kind which will be investigated through this grant, form a wonderful platform form which to generate interest among the general public in the physical sciences. To continue the efforts I have made in the past to share the excitement of scientific research with the public, both in Switzerland and in the UK, we plan to participate in several outreach activities throughout the period of this grant. These include lecturing to A-level students at The Science Center at UCL, working with the UCL public engagement unit to take part in outreach programs directed toward school children, and participating in public open days. By doing this it is hoped that we will inspire young students to develop an interest in the physical sciences, and support the government's effort to prioritise the increased uptake in STEM (Science, Technology, Engineering and Mathematics) subjects by young people.

Publications

10 25 50
 
Description 1. We have developed a new set of chip-based electrical devices for transporting, manipulating and trapping gas-phase atoms and molecules. When trapped using these devices the samples can be used to investigate the properties of, and probe, the chip surfaces, and may be exploited as quantum memories for applications in quantum information processing.

2. We have also demonstrated the use of atoms in very highly excited states as sensitive microscopic probes of broadband radio-frequency radiation. Because of their very small size these atomic antennas cause minimal distortions to the electromagnetic environment in which they are located. This is particularly beneficial when detecting very weak radio-frequency fields with great sensitivity.

3. We have studied, by high-resolution microwave spectroscopy, the role that electric-dipole interactions between atoms can have on the decoherence of quantum systems involving highly excited electronic quantum states. The outcomes of this work will be of importance in the use of atoms in these states for applications in quantum information processing.

4. We have prepared samples of helium atoms in highly excited circular quantum states, which, because of their two-level character and extreme sensitivity to resonant microwave radiation are particularly well suited for use as quantum bits (qubits), and applications as quantum memories in quantum information processing.

5. We have developed a unique quarter-wave superconducting co-planar microwave resonator design which is well suited to hybrid quantum information processing with Rydberg atoms and microwave circuits.

6. We have performed the first experiments to demonstrate control over resonant energy transfer in collisions of Rydberg atoms with polar ground state molecules using electric fields. This work has opened a range of new opportunities for studies of atom-molecule interactions at low temperature in which long-range dipole-dipole interactions may be exploited to regulate access to short-range chemical processes.

7. We have developed and realised a new and original approach to matter-wave interferometry with atoms in highly excited Rydberg states. These experimental methods are of interest for quantum sensing. They exploit coherent superpositions of internal and external quantum states of atoms.

8. We have demonstrated for the first time a coherent interface between gas-phase Rydberg and superconducting microwave circuits. This work has application in quantum computing, quantum communication and quantum sensing.
Exploitation Route In addition to being of interest for applications in quantum information processing, the devices we have developed for transporting, manipulating and trapping gas-phase atoms and molecules have applications in studies of collisions and decay processes of importance in the chemistry of the upper atmosphere of the Earth. The microscopic atomic sensors for radio-frequency electric fields that we have developed will be used to probe and characterise devices in which we plan to exploit atoms in highly excited circular electronic quantum states for applications in quantum information processing. Results on the control of resonant energy transfer in collisions of Rydberg atom with polar ground state molecules have allowed a new understanding of effects of collisions on decoherence of high Rydberg states and open new opportunities for studies of atom-molecule interactions at low temperatures. The recent development of a new approach to matter-wave interferometry with highly excited atoms is an example of a quantum sensor that exploits coherent superpositions of internal and external quantum states of atoms. The work we have done on coherent coupling gas-phase Rydberg atoms to superconducting microwave circuits opens a range of new possibilities in areas including quantum computing, quantum communication and quantum sensing.
Sectors Digital/Communication/Information Technologies (including Software),Electronics,Environment

URL https://www.ucl.ac.uk/phys/amopp/people/stephen_hogan
 
Description Outcomes from this award - in particular those associated with the first demonstration of the coherent coupling of gas-phase atoms in Rydberg states to microwave fields in chip-based superconducting microwave resonators - are of interest to the public and private sectors in areas related to microwave field sensing for applications in security, and test and measurement. The method of Rydberg-atom matterwave interferometry developed with the support of this award represents a new research area that links work, and experimental techniques, previously associated with studies of cold atoms/molecules and quantum optics, to research in physical chemistry and antimatter physics.
First Year Of Impact 2019
Sector Aerospace, Defence and Marine,Electronics,Security and Diplomacy
 
Title Demonstration of coherent interface between Rydberg atoms with superconducting microwave circuits 
Description We have demonstrate, for the first time, coherent coupling of gas-phase Rydberg atoms to microwave fields in superconducting co-planar waveguide resonators. 
Type Of Material Technology assay or reagent 
Year Produced 2019 
Provided To Others? Yes  
Impact Manuscript available on arxiv and under review at journal. Applications of this work lie in the areas of quantum memories, optical-to-microwave photon conversion for quantum communication, and quantum non-demolition detection of atoms and molecules. 
URL https://arxiv.org/abs/1911.05513
 
Title Matter-wave interferometry with atoms in high Rydberg states 
Description We have recently invented a new and original approach to matter-wave interferometry with atoms in highly excited quantum states. This method opens new opportunities for quantum sensing with superposition states. 
Type Of Material Technology assay or reagent 
Year Produced 2019 
Provided To Others? Yes  
Impact Manuscripts published. 
 
Title Transmission line guides, beamsplitters, decelerators and traps for Rydberg atoms 
Description We have developed a unique set of chip-based electric guides, beamsplitters, decelerators and traps for atoms and molecules in highly excited Rydberg states. The electrode geometries of these devices are similar to those of co-planar microwave waveguides/transmission lines. Because of this the can be readily integrated with these devices for applications in cold chemistry and quantum information processing. 
Type Of Material Technology assay or reagent 
Year Produced 2016 
Provided To Others? Yes  
Impact These devices we have developed in my group have opened new opportunities for experiments in cold chemistry and quantum information processing. 
 
Description ECAMP conference 2017 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Dissemination of research outcomes at international conference
Year(s) Of Engagement Activity 2017
 
Description Advanced SRitp and GiRYD School on Giant Interactions in Rydberg Systems, Weizmann Institute of Science, Israel (2018) 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Postgraduate students
Results and Impact Invited lectures at international postgraduate student workshop
Year(s) Of Engagement Activity 2018
URL http://www.weizmann.ac.il/conferences/SRitp/September2018/advanced-sritp-and-giryd-school-giant-inte...
 
Description CCMI conference Athens, Georgia, USA (2018) 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Invited conference talk
Year(s) Of Engagement Activity 2018
URL http://www.ccmi2018.com/
 
Description Department Gala Lecture 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach Local
Primary Audience Undergraduate students
Results and Impact Public lecture
Year(s) Of Engagement Activity 2016
 
Description Edinburgh seminar 2017 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Postgraduate students
Results and Impact Invited seminar - dissemination of research outcomes
Year(s) Of Engagement Activity 2017
 
Description Orsay seminar (2017) 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Postgraduate students
Results and Impact Invited seminar at Institut des Sciences Moléculaires d'Orsay
Year(s) Of Engagement Activity 2017
 
Description Seminar University College Dublin (2018) 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Postgraduate students
Results and Impact Research seminar - dissemination of research outcomes
Year(s) Of Engagement Activity 2018
 
Description Strathclyde seminar 2016 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Postgraduate students
Results and Impact Invited seminar - dissemination of research outcomes
Year(s) Of Engagement Activity 2017
 
Description iCOMET conference Innsbruck (2017) 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Professional Practitioners
Results and Impact Hot topic talk at international conference - dissemination of research outcomes
Year(s) Of Engagement Activity 2017