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Interference and Resonant Phenomena involving Antimatter

Lead Research Organisation: UNIVERSITY COLLEGE LONDON
Department Name: Physics and Astronomy

Abstract

Whilst the apparent imbalance between matter and antimatter in our universe remains a major puzzle in science, valuable insights into the basic interactions between the two have been gained by studying collisions of positrons and positronium with atoms and molecules. The proposed programme is focussed on advancing this knowledge.

Positrons are the antimatter counterpart to electrons with which they eventually annihilate releasing gamma-rays; positronium (Ps) is the atom-like bound state of a positron and an electron, analogous to hydrogen with the positron replacing the proton. In addition to their importance in the fundamental understanding of nature, studies of their interactions with matter allow us, for example, to investigate material properties and to obtain functional imaging of human organs as it is done in positron emission tomography (PET). Positronium formation is so probable that, for example, 80% of gamma-rays detected in PET and 95% of positron annihilations originating from the centre of the Milky Way are from Ps decays.

Lately, we discovered that positronium scatters in a manner similar to that of a bare electron at the same collision velocity (despite Ps being a neutral atom, twice the electron mass). This finding was entirely unexpected and it is guiding theory and experiment towards an accurate description of the interactions of this matter-antimatter hybrid with matter.

Two recent technical attainments are particularly pertinent to our future plans, namely the realization of a positronium beam now tuneable down to energies five times lower than previously obtained, and the development of a new high-resolution positron-beamline apt for inspecting collision dynamics.

These enhanced experimental capabilities have already started to bear fruit with first glimpses of subtle quantum mechanical effects, such as resonances and interference phenomena, previously beyond established observational power. We will probe the mechanisms giving rise to such effects in positron and positronium scattering and thus aid progress towards of a more profound understanding of matter-antimatter physics in general.

Planned Impact

Positrons and positronium are fundamental to our understanding of the physical universe. They have also become useful in practical applications ranging from material science to engineering and outstandingly powerful in the biomedical industry.

In this respect, there is currently an international drive towards the development of accurate dosimetry for Positron Emission Tomography (PET) and data for positron/Ps interactions with molecules of biological significance are particularly sought after for simulations of positron tracks in biological media. The clear motivation is that an increased understanding will lead to reduced damage of healthy tissue and, potentially, to efficient targeting (e.g. of cancerous growths). We regularly receive requests to provide cross-section data and we will alert scientists working in this field to our new findings as they emerge.

We will disseminate our experimental results by publishing in high-profile journals and by delivering invited talks and seminars. Additionally, research data will be placed online at UCL Discovery where free access to publications will be available. We will engage with key scientists by pro-actively fostering dialogues through exchange visits and focussed workshops.

Additional benefits will arise for the public/industrial sector through the training of scientists in performing world-class science and in developing a variety of skills (e.g. problem-solving, creative, communication, etc), crucial in innovative endeavours in academia and industry. Mentoring and support for career development will be provided to staff involved in the project throughout its duration, also through the provisions of the UCL Doctoral Skills Development Programme. Recent members of the group have gone on to work at prestigious research labs (e.g. CERN, RIKEN, ETH), in the UK Industry (e.g. AWE, Health Protection Agency, BAE Systems Detica, Thermo Fisher Scientific) and in the financial sector.

Antimatter is a powerful vehicle for stimulating interest and promoting understanding in physics and science by the general public and especially by young people. In the framework of the departmental "Science for the Public" initiatives, we shall strive to generate broader awareness through publications of broader reach and on UCL websites (with the support and advice from the UCL Public Engagement Unit), by arranging school visits to our labs and delivering popular lectures/talks at schools or interested societies.

Publications

10 25 50

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Kadokura R (2019) Angle-Resolved Electron Scattering from H_{2}O near 0°. in Physical review letters

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Laricchia G (2018) A statistical description of scattering at the quantum level. in Scientific reports

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Loreti A (2016) High-Resolution Measurements of e^{+}+H_{2}O Total Cross Section. in Physical review letters

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Newson D (2023) Statistical nature of secondary electron emission in Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

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Newson D (2023) Low-energy positronium scattering from O 2 in Physical Review A

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Schippers S (2019) Roadmap on photonic, electronic and atomic collision physics: II. Electron and antimatter interactions in Journal of Physics B: Atomic, Molecular and Optical Physics

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Shipman M (2017) Resonant scattering of positronium as a quasifree electron in Physical Review A

 
Description These may be grouped into three main areas:

(I) Positron and Electron Scattering from H2O

It is difficult to overestimate the importance of water in our Universe and to life as known. Now, for the first time, the total cross section of positrons scattering from H2O has been measured with a high-angular discrimination (~1°) against forward scattered projectiles. Results have been obtained in the energy range (10-300) eV and significant deviations (up to 100%) from previous measurements have been found which are, if ascribed entirely to the angular acceptances of various experimental systems, in quantitative accord with ab initio theoretical predictions of the differential elastic scattering cross section.
With some modifications, the technique has been extended to electron projectiles, yielding high-resolution measurements which (i) resolve discrepancies among earlier experiments, (ii) confirm a structure at intermediate energies in the total cross-section, and (iii) provide the first verification of theoretical predictions for the associated differential elastic cross-section at any angle smaller than 10°.

(II) Collisions involving Positronium

The absolute differential positronium-formation cross sections near 0o for Ne, Ar, Kr, and Xe have been obtained and compared with theory where available. The forward collimation of the positronium produced has also been examined and trends among targets found when considered as a function of the reduced total energy. Structures in the form of shallow dips have been noted at low energies and the question raised as to whether they may be indicative of quantum vortices at larger angles.
In order to clarify the physics underlying the observations of the electronlike behavior of positronium and its resonant scattering from CO2, we have measured the Ps + N2 total cross section and found it also to exhibit significant structure in the vicinity of the resonance in the corresponding electron data. Analysis of the resonances reveals that Ps is distorted in the collisions with the electron on average closer to the target than the positron, which may in turn bind resonantly to the ensuing temporary negative ion. This description of the nature of Ps resonances confirms long-standing theoretical predictions.
From the point of view of resonance scattering, the O2 molecule is of special interest. While for N2 and CO2, low-energy resonances have been observed and confirmed by calculations for both electron and Ps scattering, the low-energy resonance in electron + O2 scattering is extremely narrow and only detected in experiments with high-energy resolution. We measured the total cross section of positronium scattering from molecular oxygen in the velocity range 0.27-1.50 a.u. and found it to be close to the corresponding equivelocity electron cross section above 0.87 a.u., as uncovered in our previous work. However, below this energy, the cross section for positronium has been found to exceed that for electrons by up to a factor of 4 at the lowest energy. Measurements have been compared to the predictions of low-energy resonant peaks in the elastic-scattering cross section calculated within a free-electron-gas model. In addition, the cross sections for positronium breakup and O2- formation have been calculated using a classical trajectory Monte Carlo approach. At its peak, the latter is predicted to be around 35 times less likely than elastic scattering.

(III) Statistical Description of Inelastic Scattering at the Quantum Level

Quantum physics is undoubtedly the most successful theory of the microscopic world, yet its application even to simple atomic and molecular systems is a formidable task and approximations are often employed, the validity of which may be restricted to given energy regimes and/or targets and/or projectiles.
Now we have discovered that the lognormal function, widely used for the probability distribution of macroscopic stochastic events (as diverse as periods of incubation of and recovery from diseases, size of grains, abundance of species, fluctuations in economic quantities, etc.) may also be employed to describe the energy dependence of inelastic collisions at the quantum level (including ionization, electron capture and excitation by electrons, positrons, protons, antiprotons, etc.), simply by allowing for the relevant threshold energy.
The generality of this finding, namely its independence from the nature of the interactions at play, is reinforced by its applicability also to nuclear and solid state physics (e.g. non-resonant nuclear reactions and the emission of secondary electrons). Our discovery is expected to impact also on the fundamental understanding of the interface between the classical and quantum domains.
Exploitation Route Engagement with other scientists is crucial, especially theorists with whom our experimental data can be used to test hypotheses, modellers of atmospheric and astrophysical events, plasma diagnostics and radiobiological processes who input cross-section data in their computations. We also disseminate our results by publishing in high-profile journals (e,g, PRL, Nature Group), by delivering invited talks at the major conferences in the field (e.g. ICPEAC, ICPA, POSMOL) as well as providing data on UCL Discovery where free access to publications is also available.
Sectors Chemicals

Environment

Healthcare

URL http://www.ucl.ac.uk/positron-physics/title.html
 
Description The interactions of positrons and positronium with matter are fundamental to our understanding of the physical universe and applications ranging from material science to engineering and medicine. The outcomes of our research impact on both aspects with advances in knowledge of basic collision physics (e.g. resonances, interference effects, quantum vortices, statistical description) and their relevance to instruments and techniques (e.g. charge particle detectors, scanning electron microscopes, particle accelerators, extreme ultraviolet lithography, positron-emission-tomography and positronium imaging). Moreover the public/industrial sectors continue to gain greatly from the training of research students and associates in performing world-class science through the acquisition of valuable transferable skills (e.g. critical thinking, problem-solving, analysis and synthesis, communication), essential for innovation in academia and industry. Recent members of the group have gone on to work at prestigious research labs and universities around the world as well as for the UK industry, financial sector and civil service. We continue to alert the general public to the outcomes of our research through publications of broader reach on UCL websites, by arranging school visits to our labs and delivering popular lectures/talks at schools and interested societies.
First Year Of Impact 2016
Sector Chemicals,Healthcare
Impact Types Cultural

Societal

 
Description EPSRC DTP 2018-22
Amount £800,000 (GBP)
Funding ID EP/R513143/1 
Organisation University College London 
Sector Academic/University
Country United Kingdom
Start 09/2018 
End 09/2022
 
Description UCL RCIF Capital Equipment Fund
Amount £30,000 (GBP)
Funding ID
Organisation University College London 
Sector Academic/University
Country United Kingdom
Start 07/2018 
End 07/2019
 
Title A statistical description of scattering at the quantum level 
Description Data supporting the findings of Laricchia et al. (2018) Scientific reports, 8(1), pp. 15056. doi: 10.1038/s41598-018-33425-8 
Type Of Material Database/Collection of data 
Year Produced 2018 
Provided To Others? Yes  
Impact External downloads; invited talks and seminars; application and general extension of method to other systems and processes in physics. 
URL http://discovery.ucl.ac.uk/10057312/
 
Title Angle-resolved electron scattering from H2O near 0o 
Description Data supporting the findings of Kadokura et al. (2019) Physical review letters, 123(3), pp. 033401. doi: 10.1103/PhysRevLett.123.033401 
Type Of Material Database/Collection of data 
Year Produced 2019 
Provided To Others? Yes  
Impact External downloads; invited talks; potential application and extension of method to other targets, especially polar molecules. 
URL https://discovery.ucl.ac.uk/id/eprint/10074515/
 
Title Detection of low-energy charged particles by channel electron multipliers 
Description The data supporting the findings of D.M. Newson et al 2022 JINST 17 P11026 
Type Of Material Database/Collection of data 
Year Produced 2022 
Provided To Others? Yes  
Impact External downloads, invited talks. Channel electron multipliers are important tools in the detection of particles in a variety of environments on Earth and in space from the impact of ions, atoms and molecules. The generality of our findings is expected to assist these endeavors. 
URL https://discovery.ucl.ac.uk/id/eprint/10158097/
 
Title Differential positronium-formation cross sections for Ne, Ar, Kr, and Xe 
Description The data supporting the findings of Fayer et al (2019) Physical Review A, 100, 062709 doi: 10.1103/physreva.100.062709 
Type Of Material Database/Collection of data 
Year Produced 2019 
Provided To Others? Yes  
Impact External downloads; invited talks; application and extension of method to other targets, including molecules; theoretical developments. 
URL https://discovery.ucl.ac.uk/id/eprint/10088167/
 
Title High-Resolution Measurements of e^{+}+H_{2}O Total Cross Section 
Description Data supporting the findings of Loreti et al. (2016). Physical review letters, 117(25), pp. 253401 10.1103/PhysRevLett.117.253401 
Type Of Material Database/Collection of data 
Year Produced 2016 
Provided To Others? Yes  
Impact External downloads; invited talks; application and extension of method to electron + H2O scattering, and potentially to other polar molecules. 
URL http://discovery.ucl.ac.uk/1529854/
 
Title Low-Energy Positronium Scattering from O2 
Description The data that support the findings of Newson et al PHYSICAL REVIEW A 107, 022809 (2023) 
Type Of Material Database/Collection of data 
Year Produced 2023 
Provided To Others? Yes  
Impact External downloads, invitations to conferences. Because of the importance of this molecule and special interest, particularly from the point of view of resonance scattering, it is expected that our O2 results will stimulate further theoretical and experimental investigations. 
URL https://discovery.ucl.ac.uk/id/eprint/10164844/
 
Title Resonant scattering of positronium as a quasi-free electron in collisions with N2 and CO2 
Description Data supporting the findings of Shipman et al. (2017). Physical review A 95, 032704. DOI: https://doi.org/10.1103/PhysRevA.95.032704 
Type Of Material Database/Collection of data 
Year Produced 2017 
Provided To Others? Yes  
Impact Invited talks; application and extension of method to positronium scattering from other molecular systems, e.g. O2 10.1103/PhysRevA.107.022809. 
URL https://doi.org/10.5522/04/28451729.V1
 
Title Statistical nature of secondary electron emission 
Description The data supporting the findings of Newson, D., Kadokura, R., Brawley, S., Shipman, M., & Laricchia, G. (2023). Statistical nature of secondary electron emission. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms. doi:10.1016/j.nimb.2023.01.008 
Type Of Material Database/Collection of data 
Year Produced 2023 
Provided To Others? Yes  
Impact External downloads, invited talks. Secondary electron emission is relevant to a wide- range of applications including scanning electron microscopes, particle accelerators and detectors, extreme ultraviolet lithography. 
URL https://discovery.ucl.ac.uk/id/eprint/10163263/
 
Description ATOMKI 
Organisation Hungarian Academy of Sciences (MTA)
Country Hungary 
Sector Academic/University 
PI Contribution Positron physics expertize
Collaborator Contribution Ion collision physics expertize
Impact Record 1 of 4 Title: Low-energy positronium scattering from O2 Author(s): D. M. Newson , R. Kadokura, H. Allen , S. E. Fayer, S. J. Brawley , M. Shipman , and G. Laricchia *; R. S. Wilde, I. Fabrikant, L. Sarkadi Source: PHYSICAL REVIEW A 107, 022809 (2023); https://journals.aps.org/pra/pdf/10.1103/PhysRevA.107.022809 Addresses: [D. M. Newson , R. Kadokura, H. Allen , S. E. Fayer, S. J. Brawley , M. Shipman , and G. Laricchia], Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT, United Kingdom; [R. S. Wilde] Department of Natural Sciences, Oregon Institute of Technology, Klamath Falls, Oregon 97601, USA [I. Fabrikant] Department of Physics and Astronomy, University of Nebraska, Lincoln, Nebraska 68588-0299, USA [L. Sarkadi] ATOMKI, Institute for Nuclear Research, H-4026 Debrecen, Bem ter 18/c, Hungary Title: Angle-Resolved Electron Scattering from H2O near 0 degrees Author(s): Kadokura, R (Kadokura, R.); Loreti, A (Loreti, A.); Kover, A (Kover, A.); Faure, A (Faure, A.); Tennyson, J (Tennyson, J.); Laricchia, G (Laricchia, G.) Source: PHYSICAL REVIEW LETTERS Volume: 123 Issue: 3 Article Number: 033401 DOI: 10.1103/PhysRevLett.123.033401 Published: JUL 16 2019 Addresses: [Kadokura, R.; Loreti, A.; Tennyson, J.; Laricchia, G.] UCL, UCL Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Kover, A.] MTA Inst Nucl Res Atomki, Bem Ter 18-c, H-4026 Debrecen, Hungary. [Faure, A.] Univ Grenoble Alpes, 621 Ave Cent, F-38400 St Martin Dheres, France. Reprint Address: Kadokura, R (reprint author), UCL, UCL Dept Phys & Astron, Gower St, London WC1E 6BT, England Experiment & Theory Title: Resonant scattering of positronium as a quasifree electron Author(s): Shipman, M (Shipman, M.); Brawley, SJ (Brawley, S. J.); Sarkadi, L (Sarkadi, L.); Laricchia, G (Laricchia, G.) Source: PHYSICAL REVIEW A Volume: 95 Issue: 3 Article Number: 032704 DOI: 10.1103/PhysRevA.95.032704 Published: MAR 21 2017 Addresses: [Shipman, M.; Brawley, S. J.; Laricchia, G.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Sarkadi, L.] Hungarian Acad Sci ATOMKI, Inst Nucl Res, Pf 51, H-4001 Debrecen, Hungary. Experiment & Theory Title: High-Resolution Measurements of e(+) + H2O Total Cross Section Author(s): Loreti, A (Loreti, A.); Kadokura, R (Kadokura, R.); Fayer, SE (Fayer, S. E.); Kover, A (Kover, A.); Laricchia, G (Laricchia, G.) Source: PHYSICAL REVIEW LETTERS Volume: 117 Issue: 25 Article Number: 253401 DOI: 10.1103/PhysRevLett.117.253401 Published: DEC 16 2016 Addresses: [Loreti, A.; Kadokura, R.; Fayer, S. E.; Laricchia, G.] UCL, UCL Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Kover, A.] Hungarian Acad Sci, Inst Nucl Res, POB 51, H-4001 Debrecen, Hungary. Reprint Address: Laricchia, G (reprint author), UCL, UCL Dept Phys & Astron, Gower St, London WC1E 6BT, England. Title: Magnetic field-free measurements of the total cross section for positrons scattering from helium and krypton Author(s): Fayer, SE (Fayer, S. E.); Loreti, A (Loreti, A.); Andersen, SL (Andersen, S. L.); Kover, A (Koever, A.); Laricchia, G (Laricchia, G.) Source: JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS Volume: 49 Issue: 7 Article Number: 075202 DOI: 10.1088/0953-4075/49/7/075202 Published: APR 14 2016 Addresses: [Fayer, S. E.; Loreti, A.; Laricchia, G.] UCL, UCL Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Andersen, S. L.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Koever, A.] Hungarian Acad Sci, Inst Nucl Res, POB 51, H-4001 Debrecen, Hungary.
Start Year 2016
 
Description Curtin University, GPO Box U1987, Perth, WA 6845, Australia 
Organisation Curtin University
Country Australia 
Sector Academic/University 
PI Contribution Experimental positron and positronium scattering expertise.
Collaborator Contribution Theoretical positron and positronium scattering expertise.
Impact Interference effects in positronium formation from molecules, in preparation 2021
Start Year 2020
 
Description Oregon Institute of Technology, USA 
Organisation Oregon Institute of Technology
Country United States 
Sector Academic/University 
PI Contribution Experimental Positronium Scattering expertise
Collaborator Contribution Theoretical Positronium Scattering expertise
Impact Low-energy positronium scattering from O2, PHYSICAL REVIEW A 107, 022809 (2023)
Start Year 2020
 
Description University of Nebraska 
Organisation University of Nebraska-Lincoln
Country United States 
Sector Academic/University 
PI Contribution Experimental Positronium Scattering expertise
Collaborator Contribution Theoretical Positronium Scattering expertise
Impact Low-energy positronium scattering from O2, PHYSICAL REVIEW A 107, 022809 (2023)
Start Year 2020
 
Description "Maths formula links clouds, marriages and atoms" UCL MAPS Website 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach International
Primary Audience Public/other audiences
Results and Impact Maths formula links clouds, marriages and atoms: UCL scientists have made a new discovery that will help describe and predict how collision probabilities involving subatomic particles vary with energy.

The same mathematical formula which describes the probability distribution of phenomena such as periods of incubation of diseases, size of clouds, abundance of species, age of marriage, fluctuations in economic variables, etc, also applies at the quantum level, UCL scientists find.
The discovery, published today in Scientific Reports, will help in describing and predicting how collision probabilities involving subatomic particles vary with energy. It is expected to impact on a fundamental issue in physics, that of the boundary between the classical and quantum domains.
Professor Gaetana Laricchia (UCL Physics & Astronomy) who led the work, said: "The question of where the classical world ends and the quantum one begins is a major concern in physics. Our finding is particularly exciting because of its breadth and simplicity, and because it links systems normally described by quantum theories to those in the classical regime."
"Our initial investigation arose in the context of atomic collisions with positrons", the positron being the antimatter counterpart to the electron, that is the same mass but opposite charge.
"At first, we noticed similarities among different atoms. So we searched for a common mathematical expression and found that a formula - the "lognormal distribution" - widely used for large scale phenomena, unexpectedly worked well not only for different atomic targets but also different projectiles and processes."".
The prediction and measurement of collision probabilities at the quantum level engage theorists and experimentalists worldwide, quantum theoretical approaches requiring complex calculations and being currently restricted to given physical systems, processes or energy regimes.
In the present statistical description, observed to be valid over a broad energy range, the only quantum input is the minimum energy required for the process under consideration.
In analogy with studies of clouds and marriages, the authors conjecture that the behaviour arises if the outcome of the collision is the product of many independent random effects.
The generality of the analysis, namely its independence from the details of the forces at play, is reinforced by their finding that the formula also applies to solid state and nuclear physics problems.
Year(s) Of Engagement Activity 2018
URL https://www.ucl.ac.uk/mathematical-physical-sciences/news/2018/oct/maths-formula-links-clouds-marria...
 
Description IOP Conference of Physics and Astronomy Students 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Undergraduate students
Results and Impact Every year a university in the UK hosts the Conference of Physics and Astronomy Students, an Institute of Physics event. The stated aims are that "undergraduate students learn about the exciting cutting edge research undertaken by both distinguished professors from around the country and fellow physics colleagues alike; all the being able to network and get to know the other attendees through the various planned social events". I was invited by the Student Organizing Committee to deliver a 1-hr lecture on my research interests entitled "Collision involving antimatter".
Year(s) Of Engagement Activity 2017
URL http://www.ucl.iopcaps.co.uk/#theconference
 
Description Winter Research Symposium (Donovan Newson) 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach Local
Primary Audience Study participants or study members
Results and Impact Opportunity for postgraduate students and early career researchers to present their results to a broader research group.
Year(s) Of Engagement Activity 2021
 
Description Women's day seminar invitation 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach Local
Primary Audience Postgraduate students
Results and Impact Spectroscopy and Dynamics 'Supergroup' seminars for several chemistry department research groups to an audience of approx. 30 people.
Year(s) Of Engagement Activity 2019