Controlling Environmental Interactions for Novel Solid-State Quantum Technologies
Lead Research Organisation:
University of Sheffield
Department Name: Physics and Astronomy
Abstract
Quantum dots (QDs) are nanoscale regions of semiconductor, embedded within a much larger host of a second semiconductor. The differing properties of the two semiconductors mean that single particles of charge (electrons) can be trapped within a QD, allowing for study of light-matter interactions on a single particle level. In particular, QDs form an excellent source of the quantum states of light (photons) that are required for many exciting new quantum technologies such as secure communication and enhanced sensing.
A consequence of the solid-state host is that the QD interacts with its local environment, a particularly important example being quantised vibrations of the lattice, termed phonons. These interactions have typically been considered an unwelcome but unavoidable consequence of working with QDs and other similar solid-state systems. This proposal aims to demonstrate that through appropriate nano-fabrication and control of the QD geometry, the interaction of the QD with both its optical (photonic) and vibrational (phononic) environments can be controlled. By realising such control over environmental interactions, the impact of phonon interactions on the photons emitted can be almost eliminated, increasing the efficiency and quality of the QD photon source to support new applications. Furthermore, the need for extreme cryogenic cooling can be greatly reduced, removing a significant barrier to quantum technologies applications.
Harnessing these developments, several novel quantum technologies will be developed based on the QD platform. Quantum 2-photon microscopy offers the potential to perform imaging of delicate samples that would be damaged by the intense light fields required for current methods. Meanwhile, high sensitivity optical sensing can be realised by using phonon interactions to "squeeze" the uncertainty in photons emitted by the QD. Finally, quantum data locking offers the potential for quantum-secured communication with a significantly higher efficiency than existing methods.
A consequence of the solid-state host is that the QD interacts with its local environment, a particularly important example being quantised vibrations of the lattice, termed phonons. These interactions have typically been considered an unwelcome but unavoidable consequence of working with QDs and other similar solid-state systems. This proposal aims to demonstrate that through appropriate nano-fabrication and control of the QD geometry, the interaction of the QD with both its optical (photonic) and vibrational (phononic) environments can be controlled. By realising such control over environmental interactions, the impact of phonon interactions on the photons emitted can be almost eliminated, increasing the efficiency and quality of the QD photon source to support new applications. Furthermore, the need for extreme cryogenic cooling can be greatly reduced, removing a significant barrier to quantum technologies applications.
Harnessing these developments, several novel quantum technologies will be developed based on the QD platform. Quantum 2-photon microscopy offers the potential to perform imaging of delicate samples that would be damaged by the intense light fields required for current methods. Meanwhile, high sensitivity optical sensing can be realised by using phonon interactions to "squeeze" the uncertainty in photons emitted by the QD. Finally, quantum data locking offers the potential for quantum-secured communication with a significantly higher efficiency than existing methods.
Publications
Brash A
(2023)
Nanocavity enhanced photon coherence of solid-state quantum emitters operating up to 30 K
in Materials for Quantum Technology
Javadi A
(2023)
Cavity-enhanced excitation of a quantum dot in the picosecond regime
in New Journal of Physics
Phillips CL
(2024)
Purcell-enhanced single photons at telecom wavelengths from a quantum dot in a photonic crystal cavity.
in Scientific reports
Sheldon S
(2024)
Optical spin initialization and readout with a cavity-coupled quantum dot in an in-plane magnetic field
in Physical Review B
Siampour H
(2023)
Observation of large spontaneous emission rate enhancement of quantum dots in a broken-symmetry slow-light waveguide
in npj Quantum Information
| Description | Submission of evidence on Commercialising Quantum Technologies to Parliamentary Science, Innovation and Technology Committee |
| Geographic Reach | National |
| Policy Influence Type | Participation in a guidance/advisory committee |
| URL | https://committees.parliament.uk/writtenevidence/120823/pdf/ |
| Description | INTEGRATED QUANTUM NETWORKS (IQN) RESEARCH HUB |
| Amount | £21,272,349 (GBP) |
| Funding ID | EP/Z533208/1 |
| Organisation | Engineering and Physical Sciences Research Council (EPSRC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 12/2024 |
| End | 11/2029 |
| Description | Rapid Spend Capital Fund |
| Amount | £202,000 (GBP) |
| Organisation | Engineering and Physical Sciences Research Council (EPSRC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 02/2023 |
| End | 07/2023 |
| Description | Super-Sensitive Optical Quantum Metrology with an Efficient Solid-State Photon Source |
| Amount | £62,500 (GBP) |
| Funding ID | ST/Y005031/1 |
| Organisation | Science and Technologies Facilities Council (STFC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 12/2023 |
| End | 03/2024 |
| Description | Tailoring Phonon Interactions Through Control of Quantum Dot Morphology |
| Amount | £70,000 (GBP) |
| Funding ID | RG\R2\232470 |
| Organisation | The Royal Society |
| Sector | Charity/Non Profit |
| Country | United Kingdom |
| Start | 12/2023 |
| End | 05/2025 |
| Title | Nanocavity enhanced photon coherence of solid-state quantum emitters operating up to 30 K |
| Description | Data from the manuscript "Nanocavity enhanced photon coherence of solid-state quantum emitters operating up to 30 K".Abstract:Solid-state emitters such as epitaxial quantum dots have emerged as a leading platform for efficient, on-demand sources of indistinguishable photons, a key resource for many optical quantum technologies. To maximise performance, these sources normally operate at liquid helium temperatures (~4 K), introducing significant size, weight and power requirements that can be impractical for proposed applications. Here we experimentally resolve the two distinct temperature-dependent phonon interactions that degrade indistinguishability, allowing us to demonstrate that coupling to a photonic nanocavity can greatly improve photon coherence at elevated temperatures compatible with compact cryocoolers. We derive a polaron model that fully captures the temperature-dependent influence of phonons observed in our experiments, providing predictive power to further increase the indistinguishability and operating temperature of future devices through optimised cavity parameters. |
| Type Of Material | Database/Collection of data |
| Year Produced | 2023 |
| Provided To Others? | Yes |
| URL | https://figshare.shef.ac.uk/articles/dataset/Towards_Generating_Indistinguishable_Photons_from_Solid... |
| Title | Towards Generating Indistinguishable Photons from Solid-State Quantum Emitters at Elevated Temperatures |
| Description | Data from the manuscript "Towards Generating Indistinguishable Photons from Solid-State Quantum Emitters at Elevated Temperatures". Abstract: Solid-state emitters such as epitaxial quantum dots have emerged as a leading platform for efficient, on-demand sources of indistinguishable photons, a key resource for many optical quantum technologies. To maximise performance, these sources normally operate at liquid helium temperatures (~ 4 K), introducing significant size, weight and power requirements that can be impractical for proposed applications. Here we experimentally resolve the two distinct temperature-dependent phonon interactions that degrade indistinguishability, allowing us to demonstrate that coupling to a photonic nanocavity can greatly improve photon coherence at elevated temperatures compatible with compact cryocoolers. We derive a polaron model that fully captures the temperature-dependent influence of phonons observed in our experiments, providing predictive power to further increase the indistinguishability and operating temperature of future devices through optimised cavity parameters. |
| Type Of Material | Database/Collection of data |
| Year Produced | 2023 |
| Provided To Others? | Yes |
| URL | https://figshare.shef.ac.uk/articles/dataset/Towards_Generating_Indistinguishable_Photons_from_Solid... |
| Description | Sheffield - Manchester Quantum Theory |
| Organisation | University of Manchester |
| Country | United Kingdom |
| Sector | Academic/University |
| PI Contribution | My team in Sheffield has been performing quantum optics experiments using resonantly driven quantum dots. |
| Collaborator Contribution | The team in Manchester (Jake Iles-Smith and Ahsan Nazir) have provided theoreticcal modelling to describe our experimental results and predict optimal parameter regimes. |
| Impact | 10.1088/2633-4356/acf5c0 (2023) |
| Start Year | 2018 |
| Title | SINGLE PHOTON SOURCES |
| Description | A single photon source comprises a photon emitter (10), an excitation waveguide (30) arranged to direct excitation photons having a first polarisation direction into the photon emitter, and a collection waveguide (42) arranged to collect photons having a second polarisation direction from the photon emitter. The first polarisation direction is coupled to a first exciton state of the photon emitter and the second polarisation direction is non-parallel to the first polarisation direction and is coupled to a second exciton state of the photon emitter, and the first and second exciton states have substantially equal energies. |
| IP Reference | US2022381979 |
| Protection | Patent / Patent application |
| Year Protection Granted | 2022 |
| Licensed | Yes |
| Description | Materials for Quantum Network Launch Event |
| Form Of Engagement Activity | Participation in an activity, workshop or similar |
| Part Of Official Scheme? | No |
| Geographic Reach | National |
| Primary Audience | Other audiences |
| Results and Impact | Attended Materials for Quantum (M4QN) network launch event with ~170 attendees from Academia, Industry and Policy. Participated in several Materials Interest Groups (Semiconductor Photonics, Spin Qubits) and the Outreach and Education Thematic Interest Group. Plans have been made for subsequent meetings of these interest groups to develop new collaborative activities with the UK quantum research community. |
| Year(s) Of Engagement Activity | 2023 |
| URL | https://m4qn.org/ |
