Super-Diffusion In Quantum Spin Chains
Lead Research Organisation:
University of Birmingham
Department Name: School of Physics and Astronomy
Abstract
A drop of ink in a glass of water will diffuse outwards with time, eventually colouring the whole of the water homogeneously. A ball on a billiard board, on the other hand, will roll around, colliding and scattering off other balls. Transport of mass, energy or other properties in nature seem to occur predominantly in either way, called diffusive and ballistic, respectively. They constitute our intuition into the natural world and universe. However, physicists suspect that there could be other new types of transport defying our common sense. For instance, the transport of magnetic fluctuations in certain materials could occur neither diffusively nor ballistically, but somewhat intermediate. This unconventional transport is called the super-diffusion and is predicted to occur in one-dimensional quantum magnetic materials. It is also exciting that such unconventional transport could occur at room temperature in contrast with our naïve expectation that unique behaviour from quantum systems should be only observed at extremely low temperature. This could be a useful aspect for potential application such as in Spnitronics.
In this research project, I aim to provide the first clear experimental evidence for super-diffusion in quantum magnets. More specifically, I will look into crystals where magnetic ions are predominantly coupled along one direction, rather than three directions. This allows the crystals essentially behave as a collection of one-dimensional chain of magnetic ions. I will use Nuclear Magnetic Resonance (NMR) technique, akin to MRI, to evidence that the transport of magnetic fluctuations in such one-dimensional quantum chain occurs as super-diffusion. Through this research, we will be able to better understand the properties of quantum materials, which will underpin the development of new quantum technologies such as quantum sensors or computers.
In this research project, I aim to provide the first clear experimental evidence for super-diffusion in quantum magnets. More specifically, I will look into crystals where magnetic ions are predominantly coupled along one direction, rather than three directions. This allows the crystals essentially behave as a collection of one-dimensional chain of magnetic ions. I will use Nuclear Magnetic Resonance (NMR) technique, akin to MRI, to evidence that the transport of magnetic fluctuations in such one-dimensional quantum chain occurs as super-diffusion. Through this research, we will be able to better understand the properties of quantum materials, which will underpin the development of new quantum technologies such as quantum sensors or computers.
| Description | Korea-Europe QSTCC |
| Geographic Reach | Asia |
| Policy Influence Type | Participation in a guidance/advisory committee |
| URL | https://k-erc.eu/ke-qstcc/ |
| Description | Korea-Europe QSTCC (2024) |
| Geographic Reach | Multiple continents/international |
| Policy Influence Type | Participation in a guidance/advisory committee |
| URL | https://k-erc.eu/ke-qstcc/ |
| Description | Magnetic Birmingham |
| Amount | £50,000 (GBP) |
| Funding ID | 24-25-ERC-43 (Enhancing Research Culture Fund, QR Research and Knowledge Exchange Funding) |
| Organisation | University of Birmingham |
| Sector | Academic/University |
| Country | United Kingdom |
| Start | 02/2025 |
| End | 07/2025 |
| Description | NMR for Quantum and Functional Materials |
| Amount | £9,980 (GBP) |
| Funding ID | PPHE25\100076 |
| Organisation | The British Academy |
| Sector | Academic/University |
| Country | United Kingdom |
| Start | 03/2025 |
| End | 02/2026 |
| Description | ULT-NMR |
| Amount | £2,017,614 (GBP) |
| Funding ID | EP/Z533300/1 |
| Organisation | Engineering and Physical Sciences Research Council (EPSRC) |
| Sector | Public |
| Country | United Kingdom |
| Start | 01/2025 |
| End | 12/2027 |
| Description | NMR for quantum materials |
| Organisation | Paul Scherrer Institute |
| Country | Switzerland |
| Sector | Academic/University |
| PI Contribution | We provide our expertise in NMR instrumentation to support their NMR capability development for quantum materials research at PSI. The PI spent a research visit to their group for two and a half months. We have further scheduled to send one PhD student (Mr Tom Brogan), via Turing Scheme, to help NMR and pressure instrumentation. |
| Collaborator Contribution | They provide support for our beam time application for the large-facility, complementary muon spin rotation and relaxation experiments. They will host and train the above mentioned PhD student for pressure instrumentation and guide through muSR experiments to complement the NMR. |
| Impact | 1. Two muSR proposals at PSI granted, scheduled in June: ID: 20241761, Spin super-diffusion in the S=1/2 Heisenberg antiferromagnetic chain KCuF3 ID: 20241750, Spin transport in the classical (S=5/2) Heisenberg spin chain TMMC 2. SNSF Scientific Exchange awarded to PSI to host the PI (IZSEZ0_226814 / 1): Dec. 2024 - Feb. 2025. |
| Start Year | 2024 |
| Description | Condensed Matter Seminar at the University of Leeds |
| Form Of Engagement Activity | A talk or presentation |
| Part Of Official Scheme? | No |
| Geographic Reach | Local |
| Primary Audience | Postgraduate students |
| Results and Impact | I gave a seminar talk on quantum magnetism in one dimension, to inform researchers from various sub field of condensed matter. |
| Year(s) Of Engagement Activity | 2023 |
| Description | Condensed Matter and Quantum Materials (CMQM) 2023 |
| Form Of Engagement Activity | Participation in an activity, workshop or similar |
| Part Of Official Scheme? | No |
| Geographic Reach | National |
| Primary Audience | Professional Practitioners |
| Results and Impact | I have organised a national conference with my colleagues from Physics and Chemistry, with delegates over 200 from across the field of quantum materials and beyond. As an organiser we encouraged and supported several special sessions including a memorial of Prof. Joe Vinen, materials for quantum technologies and application of national facilities, which received very positive feedback from the participants. |
| Year(s) Of Engagement Activity | 2023 |
| URL | https://iop.eventsair.com/cmqm2023/ |
| Description | KSEAUK |
| Form Of Engagement Activity | A talk or presentation |
| Part Of Official Scheme? | No |
| Geographic Reach | National |
| Primary Audience | Professional Practitioners |
| Results and Impact | I gave a plenary talk on Quantum Materials before the professional audience from diverse background (physics, biology, engineering etc.) at the annual meeting of the Korean Scientists and Engineers Association in the UK (KSEAUK) held at Chester. The talk received numerous positive feedback and helped increase awareness of quantum materials. |
| Year(s) Of Engagement Activity | 2023 |
| URL | https://www.kseauk.org |
| Description | Organising a workshop CRIM 2024 |
| Form Of Engagement Activity | Participation in an activity, workshop or similar |
| Part Of Official Scheme? | No |
| Geographic Reach | International |
| Primary Audience | Professional Practitioners |
| Results and Impact | I have organised a workshop, supported by Institute of Physics, at London which brought together leading international academics as well as aspiring early career scientists to discuss the latest experimental and theoretical advances in the field encompassing quantum spin liquids, 1D magnetism and new magnetic 2D van-der-Waals materials to incubate new collaborations and networks. Quantum magnets play host to a rich variety of exotic phases of matter, from quantum spin liquids to super solids, skyrmions and spin nematics. Restricting the dimensionality of a magnetic system, to 1D or 2D, pulls out the richness of quantum effects even further, with new topologies of interactions and enhanced densities of states - and potential to build new 2D nanoelectronics devices. Owing to the recent development of accurate theoretical and numerical methods, alongside novel materials discovery and a broad array of experimental probes, low-D quantum magnets now serve as a testbed for realising new quantum phases, transitions and many-body phenomena with far reaching impact in fields from correlated-electron physics, to materials chemistry, cold atoms and quantum technology. |
| Year(s) Of Engagement Activity | 2024 |
| URL | https://iop.eventsair.com/crim2024/ |
| Description | Physics Seminar at Cardiff University. |
| Form Of Engagement Activity | A talk or presentation |
| Part Of Official Scheme? | No |
| Geographic Reach | Local |
| Primary Audience | Postgraduate students |
| Results and Impact | I gave a seminar talk about quantum magnetism in one dimension, which increased awareness of the research field to a broader audience from condensed matter physics. |
| Year(s) Of Engagement Activity | 2024 |
| Description | Seminar at PSI, Switzerland |
| Form Of Engagement Activity | A talk or presentation |
| Part Of Official Scheme? | No |
| Geographic Reach | Local |
| Primary Audience | Postgraduate students |
| Results and Impact | About 20 people attended from various groups and teams at PSI, where I talked about quantum materials research and the plans at Birmingham. There is a strong alignment of activities between Birmingham and PSI, and there has been a discussion for future exchange of expertise and co-development of capability particularly with NMR. There comes up a discussion on grant application development for Horizon Europe by joining forces of multiple NMR groups from Birmingham, PSI and others in European countries (Slovenia, Croatia and France). |
| Year(s) Of Engagement Activity | 2025 |
