Topological Spintronics

Lead Research Organisation: Royal Holloway University of London
Department Name: Electronic Engineering

Abstract

"Spin" is an intrinsic form of angular momentum universally carried by elementary particles, composite particles, and atomic nuclei. It is a solely quantum phenomenon and has no counterpart in classical mechanics. Many fundamental questions of the electrons' spin remain open issues up to this date: the spin-orbital coupling, spin-photon interaction, and spin wave transmission to name a few. Significantly, the discovery of giant magnetoresistance effect, celebrated by the 2007 Nobel Prize, has generated a revolutionary impact on the data storage technologies. This triggered the rise of Spintronics (or Spin-Electronics), an interdisciplinary subject dedicated for the study of spin-based other than or in addition to charge-only-based physical phenomena of electronic systems.

The recently discovered topological phase has presented new possibilities for spintronics: even the insulating state of matter exhibits a conductivity at the edges of certain physical systems and such conductive states are nontrivial and robust. Their unique spin-lock behaviours not only enrich the world of low-dimensional physics, but also provide a platform for transformative technical innovations. Traditionally spin phenomena have long been investigated within the context of ferromagnetic metals and alloys, the study of spin generation, relaxation, and spin-orbit coupling in non-magnetic materials took off only recently with the advent of hybrid spintronics and it is here many novel materials and architectures can find their greatest potentials in both science and technology. In the pursuit for such goals, the intrinsic material properties (e.g. mobility, anisotropy, conductivity etc.) are important indicators and the artificially synthesized hybrid systems (e.g. multilayers, hybrid systems, and nano-structures etc.) are valuable models for studying the topologically protected spin phenomena and could potentially be used as actual components for an eventual logic device.

This project focuses on the experimental studies (nano-fabrication and characterisation) of magnetic topological insulators. They are expected to give rise to Quantum Anomalous Hall effect and further coherent spin transport phenomena, in which Joule heating are minimised and therefore can be used in the next generation energy-efficient electronics. This will be assisted via proximity to a high-Curie-temperature ferromagnetic insulator to boost the spin ordering temperature of the selected systems.

Planned Impact

The proposed project has an immediate impact on developing experimental approaches that can underpin the application of coherent spin phenomena, and understanding of the relevant scientific concepts. It directly addresses some of the grant challenges in Spintronics and Condensed Matter such as the demonstration of quantum anomalous Hall (QAH) effect and proximity effect with insulators. These capture state-of-the-art challenges across a range of fundamental questions related but not limited to topological spintronics.

There is a vision to advance, and to explore new materials, architectures and mechanisms to manipulate electrons spin transport, in which Joule heating and dissipation are minimised and therefore can be used in the next generation energy-efficient electronics. As such the proximity effect, as described in the proposal, offers tantalising possibilities of nontrivial phenomena that traditionally heavily rely on extreme physical conditions (high field and low temperature). This will not only provide opportunities to revolutionise the understanding of the fundamental science, but also a pathway to spintronic applications beyond cryogenic temperature.

Such energy-efficient electronics have been widely regarded as a 'general-purpose technology' - a technology that makes possible other important technologies, products and services, which will contribute greatly to economic growth and welfare. Today the semiconductor-based electronics industry is on the verge of entering uncharted territory for the first time in more than 50 years. By establishing UK as a leader in spintronics research, it will be at the forefront of a new wave of technological revolution, leading to significant international competitiveness. In this regard, this project will play the role of informing the society of the future trend, providing the relevant technical communities with the preliminary results, and providing information of the feasibility for mass productions.

Above can only happen in locations with a wide base of potential employees who are well versed in the relevant concepts, which are radically different to those involved in existing technologies. In this regard the project also has a primary impact in providing a strong stream of graduate and PhD students flowing from the university (the research group) into industry and commerce. The output of highly educated people rather than the research results themselves can be an even more effective knowledge transfer mechanism.
 
Description The recently discovered topological phase has presented new possibilities for Spintronics and Condensed Matter: even the insulating state of matter exhibits a conductivity at the edges of certain physical systems. They give rise to anomalous quantum Hall effect and other coherent spin transport phenomena, in which heat dissipation is minimized and therefore can be used in the next generation energy-efficient electronics. While the metallic surface states of TIs have been extensively studied, a direct comparison of the surface and bulk magnetic property of TIs remains barely explored. Here we report an unambiguous experimental observation of a distinctly enhanced surface magnetism in a prototype magnetic TI, Cr-doped Bi2Se3. Using the synchrotron-based X-ray technique, we demonstrate a 'three-steps-transition' model, in which a temperature window of ~15 K exists where the surface of the TI is magnetically ordered while the bulk is not. Understanding the dual magnetization process has strong implications in defining the physical model of magnetic TIs and lays the foundation for making use of them in information technology.
Exploitation Route We have defined and validated an experiential approach to determine the magnetic ground state in a 'surface-specific' manner using the synchrotron-based X-ray technique. Future work to explore the tuning of this 'window' and understand the dual magnetization process will have strong implementation in refining the physical model of magnetic TIs and lays the foundation for making use of them in the emerging spintronic technologies.
Sectors Electronics

 
Description Collaboration with Diamond Light Source 
Organisation Diamond Light Source
Country United Kingdom 
Sector Private 
PI Contribution Capacity building. We explored a new experimental set up of current-switching XMCD at I10 of Diamond Light Source.
Collaborator Contribution Diamond Light Source has supported a good number of shifts of beamtime for this project.
Impact Nature Communications 12, 2492 (2021).National Science Review 7, 745 (2020). 10 National Science Review 117, 2095 (2021). Advanced Functional Materials 32, 2202977 (2022). Nature Electronics in press (2023).
Start Year 2022
 
Title Planer spin valve 
Description A pin-hole free MTJ for universal memory. 
IP Reference 2302066.2 
Protection Patent / Patent application
Year Protection Granted 2023
Licensed No
Impact A pin-hole free MTJ for universal memory.