Tracer-free, non-intrusive, time- and space-resolved temperature and scalar measurements

Lead Research Organisation: University of Cambridge
Department Name: Engineering

Abstract

The growth in air transport, and the need for base and balance thermal power in an electricity-powered future centres creates a pressing need for low emission, high efficiency gas turbines, particularly regarding NO, CO and soot. The key variables determining the production of these pollutants in the product gases are the local instantaneous product gas temperature and the local fuel fraction. The large fluctuations in gas temperature, and the exponential dependence of pollutant production on temperature means that predictions of NO, CO and soot in combustion are not possible without suitable accurate statistics of instantaneous local temperature measurements. Yet there are very few such measurements in practical devices to validate models. Local instantaneous temperature measurements in high pressure radiant devices require optical techniques which are rather complex for industrial laboratories. This proposal aims to extend a much simpler technique for the purpose to allow tracer free local measurements of temperature, pressure and water vapour.

Laser-induced grating spectroscopy (LIGS) has been shown to work even in highly radiant, soot-prone environments, and may also enable local measurements of additional target scalars (water vapour, pressure) using the easily accessible Nd:YAG laser wavelength of 1064 nm. The technique uses both the electrostrictive mode and weak absorption spectral lines in this wavelength range to enable measurements of both temperature and relative water concentrations in realistic devices. The signal to noise of the technique improves with pressure, a significant advantage for realistic devices, especially in environments such as gas turbines, which are prone to large amounts of radiant luminosity. The project will extend the current capabilities of the technique from point measurements to spatially resolved line measurements. Finally, it will extend the pump laser wavelength into near infrared, which will unlock the ability of the technique to use strong absorption lines for a range of widely available species (water, carbon dioxide and hydrocarbons), using industrial lasers at high repetition rates.

The final outcome of the project will be the development of an instrument and method for non-intrusive temperature and species measurements in high temperature, high pressure practical reacting flows, requiring only a fraction of the cost of previous techniques of comparable precision. Demonstration measurements will be produced in a high pressure, high temperature, realistic industrial facility. Data produced during these measurements will also allow researchers and developers to review and validate robust reacting flow models for industry and open up the possibilities for optimisation of clean energy conversion devices.

The plan for technology transfer is ensured by partnering with a company (Dantec) that has already packaged and commercialised similar instruments. An extension of the validation measurements to other industrial facilities at Rolls-Royce is planned once the instrument development and demonstration has been successfully concluded. Finally, the project will also offer opportunities to PhD students associated with the Energy CDT at Cardiff.

Planned Impact

The UK continues to invest strategically in the aerodynamics and propulsion area, via the Aerospace Technology Institute, and the National Combustion Facility. The UK is one of the leading suppliers of gas turbine and automotive engines components and associated engineering services, both in manufacture as well as simulations, which rely on the continuing development of high-end capabilities. These will be challenged given the aggressive targets of reduction of aeroengine and industrial NOx, CO2 and and soot emissions.

The proposed project will further develop and demonstrate the non-intrusive laser-induced grating spectroscopy technique for temperature and water mass fraction measurements, which offers the best precision for practical high pressure systems, and which can be disseminated through the gas turbine, automotive and other propulsion systems.

The main impact of the project will be the development of an instrument and method for non-intrusive temperature measurements in high temperature, high pressure practical reacting flows, requiring only a fraction of the cost of previous techniques of comparable precision. The accurate and precise measurement of local and instantaneous temperatures in gas turbines and engines is key to understanding how to improve their energy conversion and emissions performance, leading to lower soot and nitric oxide emissions.

The use of the fundamental and easily accessible 1064 nm wavelength with laser induced grating spectroscopy opens up the application of the technique to a much wider range of researchers. The technique uses both the electrostrictive mode and weak absorption spectral lines in this wavelength range to enable measurements of both temperature and relative water concentrations in realistic devices, including those that may have significant amounts of luminous soot.

Data extracted by the technique will allow researchers and developers to review and validate robust reacting flow models for industry and open up the possibilities for optimization of clean energy conversion devices. Immediate benefits will accrue from the deployment of the technique to generate a database of temperature maps in a realistic gas turbine test facility; downstream benefits will arise from the eventual packaging and commercialisation of the instrument undertaken by one of the partners in the project. Finally, an exploratory extension into near infrared excitation may eventually yield a more powerful technique which would work with a larger number of species at lower energies.
 
Description The measurement of instantaneous (as opposed to time-averaged) temperatures is key to the performance and pollutant formation in gas turbines. High instantaneous temperatures lead to the formation of high concentrations of nitric oxides. We have implemented and adapted an instrument to measure instantaneous temperatures and molar fractions of water inside a gas turbine combustor simulator. The Laser Induced Grating Spectroscopy (LIGS) technique was used because it offers robust, simple and quantitative measurements of the absolute flame temperature, which cannot be easily obtained by other methods.

The measurements at the Gas Turbine Research Combustion Facility at Cardiff. were made in premixed and partially premixed swirl-stabilised flames obtained with a range of mixtures of methane and hydrogen, at starting temperatures around 500 K and pressures around 3 bar. These results show the technique is well suited to the measurements of temperature and water vapour molar fraction, providing data which can be compared to simulations for validation of computational models of flames. The measurement campaign also showed some of the limitations of the technique associated with spatial resolution of the probe, as well as with the requirements for the facility regarding probe alignment. These are being tackled in the next phase of the campaign.

A second campaign produced measurements in a small scale pressurised facility at Cambridge was designed to determine how well the technique could be used in flames with soot, such as is the case in liquid fuel spray flames in gas turbine combustors. Although soot is usually undesirable, it shows up in intermediate locations of combustors. Its intense luminosity means that other optical techniques do not work well compared to the LIGS technique, and that soot is an excellent absorber, allowing temperatures to be extracted. The experiments have been concluded, showing how the LIGS signal quantitatively varies with the concentration of soot, and demonstrated the ability of the technique to extract temperature measurements from unsteady flames with and without soot. These findings will be reported in journals over the coming months.
Exploitation Route 1/ Experimental database: the experimental data and the associated geometric and flow details for the measurements are being packaged for archival storage for use by CFD modellers interested in reproducing the results, along with other results obtained in different campaigns at Cardiff.
2/ Commercialisation: The plan is to attract a potential commercial partner (originally Dantec) to package the instrument as a turnkey platform for temperature measurements in high temperature high pressure environments.
Sectors Aerospace, Defence and Marine,Energy

 
Title Pressurised flame facility 
Description A new facility has been commissioned for studying Laser Induced Grating Spectroscopy (LIGS) for measurement temperature and water vapour in the presence of soot. The technique uses a pulsed beam at 1064 nm to excite either air or water molecule lines to produce a density grating and an associated pressure pulse. The resulting density pattern is probed using a continuous wave laser. The technique has been initiated in a previous EPSRC funded (EP/K02924X/1) project, in a collaboration with Oxford and Cardiff Universities. The current version of the technique offers sufficient signal from 3 bar upwards for measurement of product temperatures. The new facility will enable the study of laminar and turbulent flame measurements at pressures up to 5 bar, and burning powers of the order of kW. The vessel has four air-purged windows arranged at 90 degrees for optical access. 
Type Of Material Improvements to research infrastructure 
Year Produced 2022 
Provided To Others? No  
Impact The facility allows optical access in a pressurised vessel with combustion, allowing the study of temperatures in laminar and turbulent flames using LIGS (and other) optical techniques. 
URL http://www-g.eng.cam.ac.uk/reactingflows/projects/diagnostics/ligs/
 
Description Press release from Cardiff GTRC on preliminary LIGS experiments at the high pressure combustion facility 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Public/other audiences
Results and Impact Laser Induced Grating Spectroscopy (LIGS) measurements taken at the @GTRC

(includes video)

https://www.linkedin.com/feed/update/ugcPost:6907987131495788546

@GTRC hosted researchers @lweller2016 and @Priyav Shah from @Cambridge University and @Oxford University as part of an @EPSRC project "Tracer-free, non-intrusive, time- and space-resolved temperature and scalar measurements", Principal Investigator @Simone Hochgreb
The need for low emission combustion technology requires an understanding of the local gas temperature. In-flame, non-intrusive temperature measurement in pressurised highly radiant flames typically requires complex optical techniques.
LIGS is a non-linear laser optical diagnostic technique which can be used to measure the temperature, pressure or species concentration at a point. The technique uses a pulsed laser to create a laser-induced grating, and a continuous wave laser to measure the transient properties of the grating. LIGS is a robust option for challenging 'dirty' environments, excels at elevated pressures and is computationally inexpensive compared to similar diagnostics.
(https://link.springer.com/article/10.1007/s00340-003-1282-8)
This test campaign showed that a LIGS signal could be measured in a 75kWth methane flame at 4bar. Future test campaigns aim to extend this to higher pressures and powers, and provide valuable experimental data to validate combustion models.
#Netzero
#Hydrogen
#Industrial Decarbonisation
#Emissions
#Gas Turbines
#Instrumentation
Year(s) Of Engagement Activity 2022
URL https://www.linkedin.com/feed/update/ugcPost:6907987131495788546