Non-classical and non-Hermitian aspects of electron-electron correlation in strong-field physics

Lead Research Organisation: City, University of London
Department Name: Sch of Engineering and Mathematical Sci

Abstract

The quintessential example of electron-electron correlation in strong-field physics is laser-induced nonsequential double ionization (NSDI) (for a review, see [l]). Thereby, a key question is whether this correlation is quantum or classical. For over two decades, NSDI has been viewed as an essentially classical phenomenon, well described by the laser-assisted collision of an electron with its parent ion. This has been due to the success of classical models reproducing electron-momentum distributions in direct, electron-impact NSDI, for which the returning electron provides enough energy for the second to overcome the ionization potential of the parent ion. Without much evidence, this line of thinking has been extrapolated to below-threshold NSDI. In this case, the first electron promotes the second to an excited state, from which it subsequently tunnels. This mechanism is known as recollision-excitation with subsequent ionization (RESI). Recently, however, it was found that quantum interference in the below-threshold regime, for which RESI occurs, is more robust than previously thought, and may survive (a) focal averaging; (b) integration over transverse electron momenta [2]. Experimental evidence for quantum interference has been found in [3]. Discrepancies between experiment and theory do exist, however. This is due to the fact that the computations in [2] have been performed using the Strong-Field Approximation (SFA), which neglects the residual Coulomb potential when the electron is in the continuum.
In this project, we intend to identify and quantify entanglement in below-threshold NSDI. This is a cutting edge problem as most groups across the globe still regard NSDI as classical. The first step to be undertaken is to develop a Coulomb corrected semi-analytic approach for RESI, building up on existing one-electron approaches [4], which will be com-pared with ab-initio two electron models. Subsequently, the student will calculate the covariant matrix for position and momentum within the developed model [5]. This will provide a lower bound for separable states, which hopefully will help distinguish classi-cal and quantum correlation. Other entanglement criteria will also be explored. We will seek optimal conditions to observe quantum effects in RESI, together with the experimen-tal groups of Prof. Jens Biegert (Institute for Photonic Sciences, Barcelona), and Prof. Xiaojun Liu (Chinese Academy of Sciences, Wuhan).
Having identified laser-induced nonsequential double ionization as being of a truely quantum orgin we also plan to explore whether this effect also occurs in non-Hermitian quantum system. I will focus my investigations mainly on PT-symmetric or pseudo/quasi Hermitian quantum mechanics. The latter systems are distinct from 11 conventional11 non-Hermitian system by having real eigenvalue spectra and unitary time-evolution, i.e. they are not considered as open systems. Only recently [6, 7,8] the full-timedependent treatment of these systems has been fully understood, which opens up the possibility to investigate effects such as the one mentioned above.
[1] C. Faria and X. Liu, J. Mod. Opt. 58, 1076 (2011).
[2] A. S. Maxwell and C. Faria, Phys. Rev. Lett. 116, 143001 (2016).
[3] Wei Quan, et al, Phys. Rev. A 96, 032511 (2017).
[4] A: S. Maxwell, A. Al-Jawahiry, T. Das and C. Faria, Phys. Rev. A 96, 023420 (2017).
[5] A. Serafini, Quantum Continuous Variables ( CRC Press, Taylor and Francis, 2017).
[6] C. Faria and A. Fring, J. of Physics A39 (2006) 9269.
[7] A. Fring and M.H.Y. Moussa, Phys .. Rev. A 93, 042114 (2016)
[8] A. Fring and T. Frith, J. of Physics A: Math. and Theor. 51 (2018) 265301

Publications

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Studentship Projects

Project Reference Relationship Related To Start End Student Name
EP/R513015/1 01/10/2018 30/09/2023
2117785 Studentship EP/R513015/1 01/10/2018 30/09/2021 Rebecca Tenney
 
Description The work funded through this award has allowed for the development of new methods for solving time-dependent quantum systems. Initial work undertaken was to develop a new way to treat the phenomenon of nonsequential double ionization (NSDI). We wanted to use the method of Lewis Riesenfeld invariants to do this. This approach was not fruitful; however we were able to develop a new approximate method that allows one to reduce a time-dependent problem to a time-independent problem thus making it easier to solve. This was applied to two different systems and shown to be highly accurate and has the potential to be applied to many more. This outcome has been published in the European Physical Journal plus and can be found here: https://doi.org/10.1140/epjp/s13360-020-00143-y.

We then extended our study of time-dependent quantum systems to those which are non-Hermitian. A key quantity to be determined in the study of these systems is the Dyson Map which can then be used to construct the metric. These quantities are difficult to calculate exactly even in the time-independent setting and one must resort to perturbative methods. Initial focus was on a determining the time-dependent Dyson map for the time-dependent anharmonic oscillator as up to then only the time-independent Dyson map had been found. We were able to do this and have published the outcome in Physics Letters A and can be found here: https://doi.org/10.1016/j.physleta.2020.126530

We then wished to develop a way to determine the time-dependent metric in a perturbative way. No such approach existed in the time-dependent setting. We were able to construct a method which could be applied to a wide variety of problems. The effectiveness of the approach was demonstrated by applying it to two separate problems and lead to us finding exact metrics. Applying it to the problem of non-Hermitian time-dependent coupled harmonic oscillators allowed us to determine several different metrics for one problem. Whilst it was known that the metric is no unique it had not been demonstrated in the time-dependent setting. Further to this we also applied our method to the time-dependent anharmonic oscillator, we were able to reproduce our findings published in a previous paper. We have published this outcome in Physica Scripta and can be found here: https://doi.org/10.1088/1402-4896/abe259.

With the development of the perturbative approach we can now start to study more time-dependent non-Hermitian systems which currently have no known exact Dyson map.
Exploitation Route The outcomes of this funding can be used within the academic community. The funding has lead to the development of new approximate methods for time-dependent quantum systems and can be applied to many different problems specifically within the area of time-dependent non-Hermitian quantum systems.
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