Electrodeposited 2D Transition Metal Dichalcogenides on graphene: a novel route towards scalable flexible electronics
Lead Research Organisation:
Imperial College London
Department Name: Materials
Abstract
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Publications
Xu L
(2022)
On-chip integrated graphene aptasensor with portable readout for fast and label-free COVID-19 detection in virus transport medium.
in Sensors & diagnostics
Wang Y
(2023)
Toward Fabrication of Devices Based on Graphene/Oxide Multilayers
in ACS Applied Electronic Materials
Thomas S
(2023)
Electrodeposition of Transition Metal Dichalcogenide Thin- Films from Non-Aqueous Solvents
in ECS Meeting Abstracts
Moorsom T
(2024)
Analysis of plasmon modes in Bi2Se3/graphene heterostructures via electron energy loss spectroscopy
in Scientific Reports
Huang W
(2024)
Integrated Rayleigh wave streaming-enhanced sensitivity of shear horizontal surface acoustic wave biosensors
in Biosensors and Bioelectronics
Thomas S
(2024)
Electrodeposition of 2D layered tungsten diselenide thin films using a single source precursor
in Journal of Materials Chemistry C
Wu Q
(2024)
Photothermal Ferrotherapy - Induced Immunogenic Cell Death via Iron-Based Ternary Chalcogenide Nanoparticles Against Triple-Negative Breast Cancer.
in Small (Weinheim an der Bergstrasse, Germany)
Cheng G
(2025)
Photo-Rechargeable Sodium-Ion Batteries with a Two-Dimensional MoSe2 Crystal Cathode.
in Nano letters
| Description | The project developed a scalable method for integrating transition metal dichalcogenides (TMDCs) onto graphene, creating heterostructures with promising electronic and optoelectronic properties. A key achievement is the controlled deposition of various TMDCs onto graphene, coupled with an understanding of the interface and defect formation. Furthermore, the project has also revealed the electronic properties and charge transport mechanisms within these heterostructures. These findings have been validated through the fabrication of high-performance photodetectors, demonstrating the potential of this approach for next-generation devices. |
| Exploitation Route | This EPSRC project has put the basis for a scalable process of fabricating TMDCs on graphene, thoroughly investigated the structural, electrical, and optical properties of the resulting heterostructures, and demonstrated their potential in device application. These outcomes provide a foundation for future research and development, enabling others to build upon our findings and develop new device applications. Specifically, the project's outputs can be taken forward and put to use by others in the following ways: * Scalable manufacturing platform: This project's key achievement is developing a foundational process for the scalable fabrication of TMDCs on graphene. This process is crucial for translating laboratory-scale demonstrations into industrially relevant manufacturing processes. * Driving application development: The characterisation of structural, electrical, and optical properties and the successful demonstration of device applications provide researchers and industry with critical data and insights. This data can help to optimise the heterostructures to develop a range of device applications including low-power electronic devices, photonic devices, and potential integration in quantum devices. * Extending to a Broader Range of 2D Materials: The scalable process developed in this project is not limited to TMDCs. It can be extended and adapted for the deposition of other 2D materials onto graphene, creating a versatile platform for exploring a wide range of heterostructures and their potential applications. This adaptable methodology will be of significant value to material scientists and engineers working with 2D materials beyond those studied in this project. |
| Sectors | Digital/Communication/Information Technologies (including Software) Electronics Healthcare |
| Description | Development of heterostructures and electronic devices based on CVD graphene and electrodeposited layers of TMDCs (transition metal dichalcogenides) |
| Organisation | University of Southampton |
| Department | School of Electronics and Computer Science Southampton |
| Country | United Kingdom |
| Sector | Academic/University |
| PI Contribution | Within an extensive collaboration between the group at SOTON an my group at Imperial (jointly funded through the EPSRC grant), we are developing heterostructures based on CVD graphene and electrodeposited layers of TMDC and develop and test novel electronic device such as transistors, barristors, and tunnelling devices. Imperial's main contributions: CVD graphene deposition and transfer, transfer of TMDC flakes, device design, electrical characterization and modelling, biosensor applications. |
| Collaborator Contribution | Within an extensive collaboration between the group at SOTON an my group at Imperial (jointly funded through the EPSRC grant), we are developing heterostructures based on CVD graphene and electrodeposited layers of TMDC and develop and test novel electronic device such as transistors, barristors, and tunnelling devices. SOTON's main contributions: precursor development and optimization of electrodeposition processes of various TMDC materials, Raman and TEM investigation (the latter with a partner at University of Warwick), transistor fabrication and charactrization. |
| Impact | Joint publications: Noori YJ, Thomas S, Ramadan S, Greenacre VK, Abdelazim NM, Han Y, Zhang J, Beanland R, Hector AL, Klein N, Reid G, Bartlett PN, de Groot CH, 2022, Electrodeposited WS2 monolayers on patterned graphene, 2D MATERIALS, Vol: 9, ISSN: 2053-1583 Noori YJ, Thomas S, Ramadan S, Smith DE, Greenacre VK, Abdelazim N, Han Y, Beanland R, Hector AL, Klein N, Reid G, Bartlett PN, de Groot CHK, 2020, Large-Area Electrodeposition of Few-Layer MoS2 on Graphene for 2D Material Heterostructures, ACS APPLIED MATERIALS & INTERFACES, Vol: 12, Pages: 49786-49794, ISSN: 1944-8244 |
| Start Year | 2022 |