CBET-EPSRC: Droplet Impact on Fluid Interfaces: 3D Effects Across Scales
Lead Research Organisation:
University of Oxford
Department Name: Engineering Science
Abstract
Over the past several decades there has been persistent and broad interest in the elucidation of drop impact problems. In the present work, we propose an integrated experimental, numerical, and analytical investigation of droplet impact on fluid interfaces with a focus on three-dimensional effects. Arguably, the required algorithms and associated computing power needed to accurately investigate 3D impacts are only just starting to mature in recent years due to the highly multi-scale nature of the fluid flow and strongly non-linear interfacial deformations. Similarly, recent advances in visualization and flow measurement have now made such investigations possible in the lab. Our ambitious project brings together a diverse set of young leaders in fluid dynamics to tackle this exciting and pressing research topic, and develop new transformative frameworks to study this challenging set of problems with cutting-edge tools and methodologies.
Droplet-liquid impacts are fundamental to a range of industrial applications such as spray cooling, fuel injection, agricultural applications such as pesticide spray, and rain droplet impact, infectious disease transmission, manufacturing applications such as inkjet printing and droplet-based 3D printing, and environmental applications such as oil spill remediation. The bulk of prior work on droplet-liquid and droplet-solid impact focuses on axisymmetric, normal impacts due to the relative simplicity of experimental characterization and visualization and reduced computational demands. In practice, non-axisymmetric droplet-interface impacts are far more common and thus broadening the current understanding to include explicit three-dimensional effects is of critical and timely importance to unlocking and advancing applications. The objective in each constituent study will be focused on delineating parametric thresholds between the impact regimes of rebound, coalescence, and splashing. These efforts will be accompanied by the development of reduced-order models (guided and benchmarked by experiment and high-fidelity simulation) to extend the practical applicability of our results.
The highly collaborative research program proposed herein will fully span low-energy to high-energy impacts under a single framework and allow the development of a single, consistent, physical picture for droplet impacts on liquid layers of the same fluid, with an unprecedented focus on three-dimensional effects, the role of the ambient gas, and the depth of the fluid layer. The research outputs are anticipated not only to include the specific scientific discoveries, but also benchmarked and documented experimental and computational tools and datasets to strengthen the broad global research efforts in the area.
Moreover, the PIs will jointly develop new experimental and simulation data visualization activities related to the proposed work for the promotion of science, outreach purposes, and access initiatives in both the UK and USA. Several established artists have agreed to participate in visualisation of fluids events, open studio sessions and competitions, which will be organised by the PIs, building on their collective record of success in scientific visualisation.
Droplet-liquid impacts are fundamental to a range of industrial applications such as spray cooling, fuel injection, agricultural applications such as pesticide spray, and rain droplet impact, infectious disease transmission, manufacturing applications such as inkjet printing and droplet-based 3D printing, and environmental applications such as oil spill remediation. The bulk of prior work on droplet-liquid and droplet-solid impact focuses on axisymmetric, normal impacts due to the relative simplicity of experimental characterization and visualization and reduced computational demands. In practice, non-axisymmetric droplet-interface impacts are far more common and thus broadening the current understanding to include explicit three-dimensional effects is of critical and timely importance to unlocking and advancing applications. The objective in each constituent study will be focused on delineating parametric thresholds between the impact regimes of rebound, coalescence, and splashing. These efforts will be accompanied by the development of reduced-order models (guided and benchmarked by experiment and high-fidelity simulation) to extend the practical applicability of our results.
The highly collaborative research program proposed herein will fully span low-energy to high-energy impacts under a single framework and allow the development of a single, consistent, physical picture for droplet impacts on liquid layers of the same fluid, with an unprecedented focus on three-dimensional effects, the role of the ambient gas, and the depth of the fluid layer. The research outputs are anticipated not only to include the specific scientific discoveries, but also benchmarked and documented experimental and computational tools and datasets to strengthen the broad global research efforts in the area.
Moreover, the PIs will jointly develop new experimental and simulation data visualization activities related to the proposed work for the promotion of science, outreach purposes, and access initiatives in both the UK and USA. Several established artists have agreed to participate in visualisation of fluids events, open studio sessions and competitions, which will be organised by the PIs, building on their collective record of success in scientific visualisation.
Publications
Quetzeri-Santiago MA
(2021)
Scientific reports controlling droplet splashing and bouncing by dielectrowetting.
in Scientific reports
Fudge BD
(2021)
Dipping into a new pool: The interface dynamics of drops impacting onto a different liquid.
in Physical review. E
Constante-Amores C
(2022)
Direct numerical simulations of turbulent jets: vortex-interface-surfactant interactions
Constante-Amores C
(2022)
Role of surfactant-induced Marangoni stresses in retracting liquid sheets
in Journal of Fluid Mechanics
Constante-Amores C
(2022)
Impact of droplets onto surfactant-laden thin liquid films
Constante-Amores C
(2022)
Role of surfactant-induced Marangoni stresses in retracting liquid sheets
Alventosa L
(2022)
Inertio-capillary rebound of a droplet impacting a fluid bath
Sykes TC
(2022)
Droplet splashing on curved substrates.
in Journal of colloid and interface science
Constante-Amores C
(2023)
Direct numerical simulations of turbulent jets: vortex-interface-surfactant interactions
in Journal of Fluid Mechanics
Sykes T
(2023)
Droplet impact dynamics on shallow pools
in Journal of Fluid Mechanics
Constante-Amores C
(2023)
Impact of droplets onto surfactant-laden thin liquid films
in Journal of Fluid Mechanics
Holland J
(2023)
Surface tension measurement and calculation of model biomolecular condensates.
in Soft matter
Fudge BD
(2023)
Drop splashing after impact onto immiscible pools of different viscosities.
in Journal of colloid and interface science
Alventosa L
(2023)
Inertio-capillary rebound of a droplet impacting a fluid bath
in Journal of Fluid Mechanics
Fudge BD
(2024)
Drop impact onto immiscible liquid films floating on pools.
in Scientific reports
Varghese N
(2024)
Effect of Surfactants on the Splashing Dynamics of Drops Impacting Smooth Substrates.
in Langmuir : the ACS journal of surfaces and colloids
| Description | Great progress has been made in all the objectives of the proposal. The main discoveries so far have been made in the micromchanics of splashing. 1) Penetration speed of droplets impacting pools of the same fluid or different liquids. Using a combination of experiments, theory, and numerical simulation, we developed a mathematical model that can predic the penetration speed of drops impacting pools. This work corrected a long-standing 'misunderstanding' in the field which the assumption was that the penetration speed was 1/2 od the impact speed of the drop, regardless of the properties of the target. 2) Control of splashing characteristics by varying the dept of the pool. Combining high-resolution numerical simulations and high-speed imaging, we demonstrated (and mapped) the key role that the presence of the bottom of the pool has on the final splashing phenomena. 3) Drop splashing upon impact on a pool of a different fluid. By using experiments, numerical simulation, and theory, we developed a model that can predict the splash transition of drops impacting a pool of a different (immiscible) fluids. While most of the existing literature focused on drops impacting the same fluids, our advances in numerical schemes and experimental techniques allowed us to provide a powerful model that can be used to predict the final outcome of such scenarios.# These results have implication on a variety of areas, from inkjet printing, pesticide-sprying, spreading of disease to a better undersanding of oil spills and ocean spume. |
| Exploitation Route | The results of our investigations have form the basis of investigation by collegues elswehere working on the impact of drops at different regimes. For instance, the group at KAUST, let by Prof. S Thoroddsen explored a region in parameter space where inertia (very high impact speeds) is dominant. Our work on the penetration speed of drops onto pools has already been citated by several groups, including the PoF group at Twente University, where they apply our predictive (and experimentally validated) formula to better understand the dynamics of supersonic liquid jets impacting pendant drops and gels. |
| Sectors | Agriculture Food and Drink Chemicals Education Environment Manufacturing including Industrial Biotechology |
| Description | Quantitative measurement of droplet impact dynamics |
| Amount | £9,950 (GBP) |
| Funding ID | 0014320 |
| Organisation | University of Oxford |
| Sector | Academic/University |
| Country | United Kingdom |
| Start | 01/2024 |
| End | 07/2025 |
| Title | Numerical model and test cases |
| Description | The numerical model is made public for researchers around the world to test it under their particular conditions. It is a three-phase code in Basilisk, for the study of drop impact onto immiscible layers in the presence of a surrounding gas. |
| Type Of Material | Computer model/algorithm |
| Year Produced | 2023 |
| Provided To Others? | Yes |
| Impact | It is the first publicly available model to deal with three phase flows in the context of drop impact. |
| URL | https://github.com/rcsc-group/DropImpactViscousPool |
| Title | Shallow Pool Impact - Open-source simulation package and experiment analysis code |
| Description | Open-source code to study shallow pool impact within the Basilisk computational framework. All code required, a descriptive README, and example/tutorial cases are provided to enable other researchers to reproduce and extend our work on fast droplet impact onto shallow pools (accompanying the paper J. Fluid Mech. paper published in 2023). Furthermore, CAD models of the 3D-printed experiment pieces, code to analyse data from a confocal sensor to determine pool depth, and various pieces of experiment and simulation data in an accessible (csv) format. |
| Type Of Material | Computer model/algorithm |
| Year Produced | 2022 |
| Provided To Others? | Yes |
| Impact | The data in this repository will enable researchers (now and in the future) to easily reproduce and extend our work. |
| URL | https://github.com/OxfordFluidsLab/ShallowPoolImpact/ |
| Description | AeroTex UK |
| Organisation | AeroTex UK |
| Country | United Kingdom |
| Sector | Private |
| PI Contribution | Twice yearly discussions on the state of the art in modelling and simulation of drop dynamics to inform the partners of latest work in this area and explore opportunities for knowledge transfer. |
| Collaborator Contribution | Twice yearly discussions on relevant experimental (e.g. wind tunnel) opportunities and results in this space, as well as significant efforts in industry that may feed into future capability deployment. |
| Impact | Co-organisation of annual UCL Anti-Icing workshop (together with Prof. Manish Tiwari and Prof. Frank Smith at University College London, and AeroTex as supporting partner), bringing together approximately 50 early career researchers and colleagues working on topics related to drop dynamics and aircraft icing prevention. Programme contains scientific talks and lab visits, with interesting follow-on discussions about funding opportunities that have been initiated after the December 2023 workshop. |
| Start Year | 2021 |
| Description | Collaboration with Leibniz Institute for Polymer Research Dresden (IPF) |
| Organisation | Leibniz Association |
| Department | Leibniz Institute for Polymer Research |
| Country | Germany |
| Sector | Charity/Non Profit |
| PI Contribution | We were contacted by researchers at IPF on the basis of work funded by this project, who were interested in the work and keen to initiate a collaboration. We visited IPF in December 2023, and are hosting one of their PhD students in Oxford for 3 months (March - May 2024). |
| Collaborator Contribution | IPF invited us (AACP and TCS) to Dresden to deliver a colloquium in December 2023 and further discuss our nascent collaboration. One of their PhD students will be working in Oxford for 3 months (March - May 2024) for a placement with us. The Dresden group are experts in viscoelastic liquids; this collaboration will benefit the project (and our groups more generally) through helping us expand in this area, which is highly relevant to modern processes like 3D printing. |
| Impact | Multidisciplinary: Engineering, Chemistry, Mathematics (modelling), and Physics. Invited colloquium at IPF Dresden, delivered by AACP and TCS, "Drops: generation, pinch-off, impact and splashing". |
| Start Year | 2023 |
| Description | Outreach Event |
| Form Of Engagement Activity | Participation in an activity, workshop or similar |
| Part Of Official Scheme? | No |
| Geographic Reach | Regional |
| Primary Audience | Public/other audiences |
| Results and Impact | This was carried out while visiting our partner institution in the US (This is an NSF(US)-EPSRC(UK) Lead Agency project grant) while the "Girls Get Math" outreach event. As the name indicates, it is aimed at encouraging female applicants to consider STEM topics and careers. The Oxford-based PDRA helped built hands-on experiments to be used by the attendants. |
| Year(s) Of Engagement Activity | 2023 |
| URL | https://icerm.brown.edu/girlsgetmath/ |
