Long-lived Radionuclides in the Surface Environment (LO-RISE)- Mechanistic Studies of Speciation, Environmental Transport and Transfer

Lead Research Organisation: Diamond Light Source
Department Name: Science Division

Abstract

The impact of radioactivity on humans and the wider environment is controlled by the behaviour of the radionuclides in groundwaters, soils and sediments, and this behaviour is dictated by the quantities of radionuclides, and their chemical forms. We will study some of the radionuclides which are particularly important because they are potentially present in relatively large quantities, are environmentally mobile, and are readily taken up by living organisms. The main radionuclides we are going to study are:

Carbon-14, which occurs in nature, but was produced back in the 1960s and 60s through nuclear weapons testing, and is also present in nuclear wastes; and

Uranium (together with its decay product radium) which is present in nature, and also in some nuclear wastes.

We will use four areas of the UK which contain elevated levels of these radionuclides as our study sites. These are South Terras (an old uranium mine in Cornwall), the Needle's Eye (a uranium mineral vein in SW Scotland), the Esk Estuary in NW England, and offshore sediments in the NE Irish Sea. At these last two sites, the sediments contain elevated levels of radioactivity from authorised Sellafield discharges, mainly in the 1970s.

As well as studying how radioactivity occurs in, and moves through, the soils, waters, plants and (in the offshore sediments) animals, we want to understand the environmental and biological processes which control this movement. To do this, we will do a series of laboratory experiments, looking at the way soil/sediment conditions influence the radionuclide concentrations in solution, the form of the radionuclides in the solution, the way radionuclides are taken up into plants and animals, and the way they are distributed in plant tissues.

We will use the results from our field and laboratory studies to develop and test mathematical models of radionuclide transport and transfer processes. These are important because they allow us to predict behaviour, rather than having to make measurements. These predictive models can be used in assessing environmental impacts, cleaning up contaminated land and predicting the long term impact of radioactive waste disposals.

Planned Impact

The risk of nuclear industry operations is always a major concern. Whether or not these perceptions of risk are justified, they influence the public and decision-makers very heavily. Moreover, there are major uncertainties associated with radioactivity and the environment, which may lead to a very conservative approach to risk. These conservatisms can lead to overestimation of risk, and costly over-engineering of projects. A proportionate understanding of risk in any nuclear programme is therefore essential for public acceptance, political support and proper cost-detriment analysis. Ultimately, the behaviour of radionuclides in the biosphere dictates the radiological risk they represent, and LO-RISE will substantially improve our understanding of this risk, and of conservatisms in risk assessments, so any organisation with responsibilities for assessing or limiting radiological impact will benefit from LO-RISE.

Two distinct groups of beneficiaries can be identified:

1. Government, Industry, and Regulators. Government sets policy for the UK nuclear industry and has clearly stated that the "safety and security of nuclear power is of paramount concern". Our findings will be disseminated both through our project partners and also by LO-RISE academics' involvement in policy and strategy activities, so that LO-RISE will inform and improve policy making. The owners and operators of nuclear licensed sites (NDA, its Site Licence Companies, MOD and its contractors), the implementers of geological disposal (NDA-RWMD); and the nuclear industry regulators (primarily EA in England and Wales, SEPA in Scotland, though ONR may also have an interest), are responsible for delivering Government's policy objectives, and LO-RISE will support development and delivery of Site Lifetime Plans, or equivalent. At the operational level, the nuclear industry relies heavily on a very diverse supply chain. LO-RISE will help these contractors develop and implement improved solutions at the project level, for deployment in the UK and overseas.

2. The Wider Stakeholder Community, and the Public. Even in 'nuclear' communities, new nuclear projects are controversial. This is clearly illustrated by, for example, 'Stop Hinkley' or the controversy around the MRWS process in west Cumbria. Objective research has a vital role in providing trusted information to inform these debates, and LO-RISE will contribute to this through specifically tailored outreach and impact activities.

Publications

10 25 50
 
Description The way uranium transports is the natural environment is rather different than might have been expected. (1 publication submitted)
Exploitation Route once published we will report to relavant bodies
Sectors Energy,Environment

URL https://www.bgs.ac.uk/rate/infoFiles/RATEProgrammeImpactsandLegacy.pdf
 
Description A series of natural laboratories (South Terras (Cornwall), Needle's Eye (Scotland), the Ravenglass Estuary (Cumbria), and various UK marine/coastal locations) were used to conduct experiments, to investigate the way soil/sediment conditions influence the radionuclide concentrations in solution, the form of the radionuclides, and the way radionuclides are taken up and distributed in the tissues of selected biota. The results from field and laboratory studies were used to develop and test mathematical models of radionuclide transport and transfer processes. The resulting models can be used in assessing environmental impacts, cleaning up contaminated land and predicting the long-term impact of radioactive waste disposal.
First Year Of Impact 2017
Sector Energy,Environment
Impact Types Societal

 
Description Compositional and Structural Evolution of Plutonium Dioxide: Underpinning Future Decisions
Amount £13,785 (GBP)
Funding ID EP/T013796/1 
Organisation Engineering and Physical Sciences Research Council (EPSRC) 
Sector Public
Country United Kingdom
Start 06/2020 
End 05/2024
 
Description Env-rad-net 2 STFC Network 
Organisation University of Manchester
Department Faculty of Medical and Human Sciences
Country United Kingdom 
Sector Academic/University 
PI Contribution Particpating in STFC funded env rad net mini project , which developed from initial Bigrad and Lorise activities. Aiming to develop methods to look at actinide containing particles on I18 and Iin particualr i14 beamline, notably from Fukashima environment.
Collaborator Contribution they are obtainign the samples from Japan through their collaboratiors, then both parties will collaborate on developing sample preparation mounting methods and in recording data at the synchrotron and it subsequent analysis
Impact no output yet, collaboration began september 2016
Start Year 2016