Integrated Research Observation System for Clean Air (OSCA)

Lead Research Organisation: King's College London
Department Name: Analytical & Environmental Sciences

Abstract

"Poor air quality is the largest environmental risk to Public Health in the UK" (DEFRA, 2017) and is consequently a focus of a range of regional and national policy interventions. However, since our transport systems, the way we heat our homes, our energy supply, our use of solvents and our agricultural systems are all changing, we know that profound changes in emissions and trends in air pollutants are likely in the coming years and indeed are already taking place. We need to understand our changing atmospheric composition, to ensure air quality policy has maximum benefit for the protection of human and environmental health.

The Clean Air: Analysis and Solutions Programme identifies the need for new capability to predict future changes in the sources, emissions and atmospheric processes responsible for air pollution. The OSCA project addresses this need through a multidisciplinary research activity, combining state-of-the-science atmospheric observations, laboratory studies, new data processing tools and integrated scientific synthesis to deliver new understanding of urban air pollution. OSCA will:

-Deliver improved quantification of emissions, combining lab measurements of brake & tyre wear sources, and measurements of the total fluxes of particulate matter (PM) and nitrogen dioxide (NO2) from the BT Tower in London. Nonexhaust emissions comprise up to 70% of traffic-derived PM10, are poorly quantified, and whose relative importance will increase with UK fleet decarbonisation. Real-world emission measurements underpin air quality predictions and avoid dependence upon manufacturer data.

-Provide a definitive, state-of-the-science assessment of UK urban air quality through exploitation of the new RCUK-funded urban air quality Supersites in London, Birmingham and Manchester to deliver comprehensive, continuous and long-term measurements of atmospheric composition. These data will characterise the changing UK pollution climate, identify subtle emission trends during implementation of regional air quality policies, and provide a key resource for evaluation of ongoing trends.

-Develop new mathematical analyses to identify emergent trends / responses to policies and apply these alongside established methods to address key science uncertainties - e.g.: to assess the trends and changing sources of NO2; to provide definitive quantification of the contributions of non-exhaust traffic, woodsmoke and cooking activities to PM; to identify trends in and contributions to ammonia emissions; to identify changes VOC emissions - precursors to ozone formation.

-Provide data and infrastructure to underpin the wider Clean Air Programme, including development and deployment of novel sensor networks (QUANT); data to validate models and health effect calculations (InSPIRE and DREaM); insight into air quality response to policy initiatives (ANTICIPATE); sensor testing and pollutant source identification (APEx).

-Enable community mobilisation through intensive field campaigns, targeted at understanding the changing gas-phase reactivity climate of the UK atmosphere (which governs production of secondary PM and ozone), and the sources and chemical composition of atmospheric aerosols.

OSCA findings will support policymakers through a range of established relationships the PIs already maintain. These include engagements within the supersite host cities, and links to relevant national bodies, including Defra, DfT, DoH, PHE and the EA. The OSCA deliverables provide important new data and novel scientific approaches central to the assessment of future changes in the sources, emissions and atmospheric processes governing air pollution in the UK - the core of WP1 of the Clean Air programme. OSCA is fully embedded into the wider programme, informing policy decisions, monitoring the impacts of decisions, and feeding public health research and outcomes.

Planned Impact

OSCA is an underpinning proposal to the UKRI Clean Air Programme and will deliver significant impact through support for multiple projects, whilst also generating wider impacts in its own right. The main direct beneficiaries of the research are the agencies invested in the activities of the programme, national and regional policy makers and public health professionals. Since the Met Office and STFC are delivering the Framework for Clean Air Analysis in WP4 they are clear beneficiaries of the outputs. The key stakeholders at national level are the Department for Environment Food and Rural Affairs; the
Department for Transport; and Public Health England. At regional level key stakeholders are the combined authorities in London; Manchester and Birmingham and Transport for Greater Manchester and Transport for London. PHE Consultants in the regions provide public health advice to regional government.

OSCA project outcomes result from PIs working closely with policy makers at regional and national level to identify key areas of concern. Emissions of NOx are of immediate and direct importance to UK air quality policy and evaluating ongoing changes in emissions has direct policy relevance given the traffic fleet is changing rapidly. Whilst particulate traffic

exhaust emissions are relatively well understood, the quantification of non-exhaust emissions that OSCA will deliver has direct benefit to national and regional policy making as the UK fleet electrifies and conventional exhaust emissions diminish. OSCA will provide policy makers with new information on the contributions to the urban mass burden from sources such as wood burning and cooking which can be used to base future decisions regarding PM control. OSCA will provide new data on urban ammonia and source attribution between agriculture and urban sources and so support policy makers in their prioritisation and strategies for reducing emissions.

Identifying the drivers of trends in pollutant concentrations and attributing changes to specific interventions and policies is extremely challenging, given the large number of confounders that exist. OSCA will develop approaches to tackle this problem, utilising a wide range of data currently available to assess the extent to which such causality can be attributed and will provide a framework for wider modelling work that will investigate this. Such tools will be widely disseminated for other stakeholders to use themselves.

OSCA measurements of the composition of air pollution, along with source attribution, will provide observational constraints to other projects within the Clean Air programme who are forecasting air quality, modelling policy interventions, assessing air quality sensor networks, measurement innovation, assessing exposure and identifying health impacts. The information and expertise from OSCA will therefore inform public health professionals investigating the health impacts of air quality in UK cities.

This work has the potential to generate significant impact with regional authorities in other areas of the UK, through the dissemination of findings, and the translation of tools. The project will seek out aspects of the research that have wider applicability to other cities and work to support decision-making more broadly in the UK.

Lastly, in many cases air quality improvements will not be delivered by policy alone but require public engagement, including technology uptake and behaviour change to deliver cleaner air. The willingness of the public to embrace change is very dependent on their knowledge of the problem, their trust in the solutions and engagement with the change process. By publicising our findings on local issues derived for example from local source apportionment, we have the potential to generate impact through region-specific public engagement, raising awareness of air pollution sources and the activities that drive emissions.
 
Description Over half of direct particle emissions from road traffic is from non-exhaust emissions such as brake and tyre wear and resuspension. Highly time resolved measurements of the increment of key tracers for these sources at the busy central roadside measurement site, above the urban background, were used to calculate improved assessments of emission factors for these sources. Brake wear was found to be the highest average non-exhaust emission source. During Covid lockdown, changes in traffic flow and dryer weather allowed us to demonstrate that the tyre and resuspension non-exhaust emissions were dependent upon speed and road surface wetness conditions.
Exploitation Route There is a high level of uncertainty in current emission factors for non-exhaust emissions. The novel use of the CO2 dilution method provides a method for similar work to be repeated in other other locations. The new emission factors can be used by other researchers and policy makers to assess the impact of non-exhaust emissions currently and in the future.
Sectors Energy,Environment,Government, Democracy and Justice,Transport

URL https://www.mdpi.com/2073-4433/12/2/190
 
Description COST Short Term Scientific Mission - Homogenized protocol to determine the source apportionment of fine organic aerosol and black carbon, based on real-time measurements of organic mass spectra and light absorption at different wavelengths
Amount £2,218 (GBP)
Funding ID ECOST-STSM-Request-CA16109-46006 
Organisation European Cooperation in Science and Technology (COST) 
Sector Public
Country Belgium
Start 03/2020 
End 04/2020
 
Description COST Short Term Scientific Mission - The long-term sources of non-refractory PM in Paris and London and their changes over time applying the new rolling PM algorithm to organic aerosol, implemented in SoFi-Pro
Amount € 2,100 (EUR)
Funding ID ECOST-STSM-Request-CA16109-44713 
Organisation European Cooperation in Science and Technology (COST) 
Sector Public
Country Belgium
Start 03/2020 
End 03/2020
 
Description COST Source Apportionment Training School
Amount £1,680 (GBP)
Funding ID COST-TS-ECOST-TRAINING_SCHOOLCA16109-280519-111341 
Organisation European Cooperation in Science and Technology (COST) 
Sector Public
Country Belgium
Start 05/2019 
End 05/2019
 
Description RI-URBANs
Amount £7,100,000 (GBP)
Funding ID 101036245 
Organisation European Commission H2020 
Sector Public
Country Belgium
Start 10/2021 
End 09/2025
 
Description Collaboration with Paul Scherrer Institut on development of source apportionment techniques for high time resolution XRF measurements of PM10 and PM2.5 
Organisation Paul Scherrer Institute
Department Laboratory of Atmospheric Chemistry
Country Switzerland 
Sector Charity/Non Profit 
PI Contribution We have shared data and helped to advance the analytical approach for source apportionment of measurements of elements in PM10 and PM2.5 in both London and Zurich. We have held several meetings where both research groups have presented data analysis and this had led to a joint publication on the Zurich data that is in the last stages of review. We have prepared a draft of a paper on the London data.
Collaborator Contribution PSI have shared data and helped to advance the analytical approach for source apportionment of measurements of elements in PM10 and PM2.5 in both London and Zurich. We have held several meetings where both research groups have presented data analysis and this had led to a joint publication on the Zurich data that is in the last stages of review.
Impact Publication completed https://doi.org/10.1016/j.aeaoa.2022.100165. This collaboration led to a deliverable in a Horizon 2020 grant (RI-URBANS) to develop this collaboration into a multi-national user group. Currently there are 52 participants in the group, covering 12 countries. The countries are mainly within Europe but also include Qatar. The aim is to standardise the analysis and source apportionment approaches for these new high time resolution XRF instruments to provide more consistent data for international analysis. Further, we are at the point of compiling the datasets available in Europe with a plan of writing an overview paper in summer 2023.
Start Year 2020
 
Description Field campaign in Barcelona 
Organisation Spanish National Research Council (CSIC)
Department Institute of Environmental Assessment and Water Research (IDAEA)
Country Spain 
Sector Public 
PI Contribution We transported research equipment to Barcelona to undertake a field campaign at a roadside site and augmented the urban background measurement station with additional instrumentation to allow a direct comparison between the two.
Collaborator Contribution At the roadside measurement station, CSIC provided power connection, paid for a subcontractor to install traffic counting and identification cameras and installed additional instrumentation to collect PM2.5 and PM10 for chemical analysis and to measure particle number concentrations. At the background station, CSIC provided technical support, hosted additional instrumentation and provided data for analysis.
Impact Data sets have been finalised and this has contributed valuable data to a PhD thesis from which further publications will follow
Start Year 2021
 
Description Guys and St Thomas' Trust Training 
Form Of Engagement Activity Participation in an activity, workshop or similar
Part Of Official Scheme? No
Geographic Reach Regional
Primary Audience Supporters
Results and Impact A workshop to broaden the knowledge of a funding agency into issues around air pollution
Year(s) Of Engagement Activity 2022