Exotic nuclear shapes with radioactive ion beams

Lead Research Organisation: University of Liverpool
Department Name: Physics

Abstract

Atomic nuclei, made up of protons and neutrons, are fundamental building blocks of nature that have been known to exist for more than 100 years. Yet, the structure of the nucleus is not even close to being understood, either in terms of its collective behaviour or individual nucleon interactions. We most often picture atomic nuclei as a spherical ball at the centre of orbiting electrons, completing the textbook version of the atom. However, what we do know is that this complex quantum system of protons and neutrons at the centre is almost never spherical, but deformed. Nuclei have shapes, from rugby-balls (prolate) and Smarties (oblate) to pears (octupole).

Predicting shapes is difficult, and nuclear theory cannot always predict the exotic shape phenomena that arise in experimental discoveries. The shape turns out to be a very sensitive test of nuclear-structure models. Shape can help distinguish which models perform best, and which ones are most reliable at predicting experimental findings in the heaviest (and newest!) elements, for example.
The most interesting shapes are often to be found in radioactive isotopes with very short half-lives. These exotic nuclei can be studied though, at facilities such as ISOLDE at CERN. Here, high-energy and high-intensity proton beams bombard targets of materials such as uranium carbide, to produce almost a thousand different isotopes. These are then filtered by mass and element before being transported and accelerated to various experimental stations where they can be studied. In this research, the radioactive beams need to be energetic so that secondary reactions can be induced. This is done by re-accelerating the extracted isotopes to around 10% of the speed of light and focusing the beam onto thin foils of isotopically pure materials.

Nuclear shape is important not only for nuclear-structure physics, but also for the study of fundamental symmetries in physics. The understanding of pear-shaped nuclei has strong implications in the search for atomic electric dipole moments (EDMs), where the reflection-asymmetric charge distribution in the nucleus enhances the EDM. A non-zero EDM would imply a violation of the charge-parity symmetry (CP-violation) and herald a new era of testing physics beyond the current standard model. The race is on for such a discovery, particularly in the odd-mass radon and radium isotopes, which form part of this study. Indeed, understanding CP-violation is seen as a route to the understanding of the observed matter/anti-matter asymmetry in the early universe, which led to our existence today.

Publications

10 25 50
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Barzakh A (2021) Large Shape Staggering in Neutron-Deficient Bi Isotopes. in Physical review letters

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Barzakh A (2022) Producing gold at ISOLDE-CERN in Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

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Butler P (2024) Studies of Re?ection Asymmetry in Heavy Nuclei in Physica Scripta

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Butler PA (2019) The observation of vibrating pear-shapes in radon nuclei. in Nature communications

 
Description A flexible open-access wire bonder for the ISOLDE Solenoidal Spectrometer upgrade project
Amount £72,993 (GBP)
Funding ID ST/W005670/1 
Organisation Science and Technologies Facilities Council (STFC) 
Sector Public
Country United Kingdom
Start 12/2021 
End 03/2022
 
Description New methods of detecting light ions in inelastic scattering reactions for nuclear shape studies
Amount £69,200 (GBP)
Funding ID RG\R1\241073 
Organisation The Royal Society 
Sector Charity/Non Profit
Country United Kingdom
Start 03/2024 
End 08/2025
 
Title ISOLDE Solenoidal Spectrometer Sort Code 
Description A code to read and process the raw data from the ISOLDE Solenoidal Spectrometer experiment at CERN. It builds physics events and performs correlations, producing a range of histograms for the user. 
Type Of Material Data analysis technique 
Year Produced 2021 
Provided To Others? Yes  
Impact First experiments of ISOLDE Solenoidal Spectrometer use this code for the online data viewing and offline analysis. 
URL https://github.com/ISOLDESolenoidalSpectrometer/ISSSort
 
Title Miniball Sort Code 
Description A data sorting and analysis code for Miniball experiments at ISOLDE. This code is designed to take the raw data files from the experiment and convert them to ROOT trees, then subsequently analyse them to produce particle-gated, Doppler corrected gamma-ray spectra for analysis. 
Type Of Material Data handling & control 
Year Produced 2018 
Provided To Others? Yes  
Impact This software is continually developed by myself by use for the whole collaboration, including our recent publications in Nature Communications and Physical Review Letters. The latest release should allow all experiments from 2017 and 2018, performed with Miniball to reach the publication-quality stage. 
URL https://github.com/Miniball/MiniballCoulexSort
 
Title Miniball Sort Code for new FEBEX DAQ 
Description A code to process the raw data from the new Miniball FEBEX DAQ and build time correlated events. In the end it also produces a range of physics histograms for the user to do the analysis. 
Type Of Material Data analysis technique 
Year Produced 2022 
Provided To Others? Yes  
Impact First test data of the new Miniball DAQ is being processed and visualised with this code. 
URL https://github.com/Miniball/MiniballSort
 
Title chisqsurface code for Gosia 
Description A technique and associated computer code for analysing a multi-dimensional chisq-surface originating from Coulomb-excitation experiments. The code uses the existing Gosia fortran code for Coulomb-excitation analysis and interfaces this with a C++ wrapper to handle the input files and produce the resulting surface in ROOT format. 
Type Of Material Data analysis technique 
Year Produced 2014 
Provided To Others? Yes  
Impact Multiple papers using results generated from this code, including on-going analysis. It was originally designed for experiments from ISOLDE, but has now been expanded over time to be more and more generic allowing a wider user base. 
URL https://github.com/lpgaff/chisqsurface
 
Title ISOLDESolenoidalSpectrometer/ISSSort: v3.0 
Description This release combines a large number of changes over the past year or so, some bug fixes and a couple of long-awaited enhancements. The main enhancements are in the ability to read simulated data from NPTool and PACE4. The histogrammer now makes a complete set of recoil time-random plots that can be used for subtraction, although the user must make the subtraction themselves. Some bug fixes included the n-side mapping, array histogram z bin limits, and some energy-loss and pulse-height-correction fixes. What's Changed Fixed missing dep for "make -j". by @hanstt in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/18 Silencing some compiler warnings. by @inkdot7 in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/19 Try a CI action file. by @inkdot7 in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/20 Add recoil E and dE eloss spectra. by @dj-clarke in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/21 Extend ex histograms by @ACeulemans in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/22 Print as (int) in error output. by @inkdot7 in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/24 Small bug fix and improvements to energy loss and pulse-height correction calculation by @berjones in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/25 B jones correct nside mapping by @berjones in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/23 Bug in autocal residuals plot by @dj-clarke in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/27 Fix bug #26 reported by Andreas Ceulemans by @lpgaff in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/28 Revert some changes and apply correct fix for issue #26 by @lpgaff in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/29 Update histogram limits for the z axis of the array by @lpgaff in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/30 Make -j fix by @inkdot7 in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/31 Correct the module indexing of detecors from nptool by @berjones in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/32 Histogrammer updates by @lpgaff in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/33 Set the Sumw2 method by default on histograms by @lpgaff in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/34 New Contributors @hanstt made their first contribution in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/18 @inkdot7 made their first contribution in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/19 @berjones made their first contribution in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/25 @lpgaff made their first contribution in https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/pull/28 Full Changelog: https://github.com/ISOLDESolenoidalSpectrometer/ISSSort/compare/v2.4...v3.0 
Type Of Technology Software 
Year Produced 2024 
Open Source License? Yes  
Impact All data from the ISOLDE Solenoidal Spectrometer is being analysed with this software. 
URL https://zenodo.org/doi/10.5281/zenodo.10694756
 
Title Miniball Sort Code 
Description A data sorting and analysis code for Miniball experiments at ISOLDE. This code is designed to take the raw data files from the experiment and convert them to ROOT trees, then subsequently analyse them to produce particle-gated, Doppler corrected gamma-ray spectra for analysis. 
Type Of Technology Software 
Year Produced 2019 
Impact This software is continually developed by myself by use for the whole collaboration, including our recent publication in Nature Communications. The latest release should allow all experiments from 2017 and 2018, performed with Miniball to reach the publication-quality stage. 
URL https://github.com/Miniball/MiniballCoulexSort
 
Title MiniballSort 
Description This release contains lots of changes during the 2023 experimental campaign. Some are mentioned from memory below, but the list is not exhaustive. The main reason for making a release at this point is to allow people to benchmark their analysis to a common version of the code. After the upcoming analysis meeting, there will be new suggestions and bug fixes that will go in to the next release. What's Changed Corrected some mistakes in the particle-gamma-gamma and particle-gamma-electron histogramming logic. Fixed a bug in the pBeta histograms that plots the velocity used for Doppler correction. Improved the EventBuilder to include a hit window for segments and addback. Added the pad detector to the particle events, so that ?E-E events can be constructed. Added a warning when multiple detectors are assigned to the same electronics channel. Implemented the correct CFD algorithm for traces. Geometry of the CD detector has been improved to better determine the phi angle. The converter for MIDAS files now tracks time warps and time jumps, printing warnings to the terminal. An option is available to discard corrupted buffers due to the July-September 2023 data readout bug in MIDAS. An extra command line option -ebis is available to discard data that is outside of the EBIS window, to speed up data sorting online. Many many bug fixes... New Contributors @konstantinstoychev made their first contribution in https://github.com/Miniball/MiniballSort/pull/5 @inkdot7 made their first contribution in https://github.com/Miniball/MiniballSort/pull/9 @lpgaff made their first contribution in https://github.com/Miniball/MiniballSort/pull/11 Full Changelog: https://github.com/Miniball/MiniballSort/compare/v1.0...v1.1 
Type Of Technology Software 
Year Produced 2023 
Impact All data from Miniball experiments running from 2022 onwards is being analysed with this software. 
URL https://zenodo.org/doi/10.5281/zenodo.7867978
 
Description Binding Blocks Summer Masterclass Webinar 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Schools
Results and Impact A webinar about experimental nuclear physics and studying exotic isotopes at the summer masterclass with the Binding Blocks team
Year(s) Of Engagement Activity 2022
URL https://sites.google.com/york.ac.uk/bindingblocks/pre-16/
 
Description Binding Blocks Winter Masterclass Webinar 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Schools
Results and Impact A webinar about experimental nuclear physics and studying exotic isotopes at the winter masterclass with the Binding Blocks team
Year(s) Of Engagement Activity 2022
URL https://sites.google.com/york.ac.uk/bindingblocks/post-16/webinars-winter-202223
 
Description Daresbury Open Days 
Form Of Engagement Activity Participation in an open day or visit at my research institution
Part Of Official Scheme? No
Geographic Reach Regional
Primary Audience Public/other audiences
Results and Impact Participation in the Daresbury laboratory open days for the general public to have access to the lab and experience some of the activities and research that goes on. I was taking part in an exhibition of the LEGO chart of nuclei as part of the binding blocks team, to enageg young people in the study of nuclear physics.
Year(s) Of Engagement Activity 2023
URL https://sci-techdaresbury.com/daresbury-open-day-2023/
 
Description I'm a Scientist, Get Me Out Of Here (CERN Zone) 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Schools
Results and Impact I am leader of the ISOLDE Team in the CERN Zone of I'm A Scientist Get Me Out Of Here, which directly engages Y10-13 students in online chats, Q&A forums, laboratory updates/tours, etc.
Year(s) Of Engagement Activity 2022,2023
URL https://cern22.imascientist.org.uk/team/isolde
 
Description I'm a Scientist, Get Me Out Of Here (November 2019) 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Schools
Results and Impact A two-week long event engaging with school classes in an online chatroom. Scientists were asked questions inside and outside of the chatroom giving the chance for school students to engage and understand/normalise science. It was really successful and the reports back from the schools involved were very positive on the impact it had for the students. One class also plans to visit CERN in the summer and I will meet them there to give them an extra tour of the ISOLDE facility.
Year(s) Of Engagement Activity 2019
URL https://about.imascientist.org.uk/2020/nuclear-zone-report-november-2019/
 
Description ISOLDE Virtual Visit for UK Schools 
Form Of Engagement Activity Engagement focused website, blog or social media channel
Part Of Official Scheme? No
Geographic Reach National
Primary Audience Schools
Results and Impact A virtual visit to the ISOLDE facility at CERN for UK schools as part of I'm A Scientist.
Year(s) Of Engagement Activity 2024
URL https://cern22.imascientist.org.uk/2024/03/07/isolde-tour/
 
Description Pizza night at University of Liverpool 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach Local
Primary Audience Undergraduate students
Results and Impact A talk to around 20 final-year undergraduate students about my research projects. The evening was catered with Pizza on behalf of the student office at the department of physics and the engagement was very positive. Around half the students stayed on after the talk to ask further questions and discuss options for PhD opportunities.
Year(s) Of Engagement Activity 2020
 
Description Pizza night at the University of Liverpool 
Form Of Engagement Activity A talk or presentation
Part Of Official Scheme? No
Geographic Reach Local
Primary Audience Undergraduate students
Results and Impact A talk to 6 final-year undergraduate students about my research projects. The evening took place on Zoom due to the pandemic, which would usually have encouraged participation by offering free pizza.
Year(s) Of Engagement Activity 2020