Multiscale in-situ characterisation of degradation and reactivity in solid oxide fuel cells
Lead Research Organisation:
University College London
Department Name: Chemical Engineering
Abstract
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Organisations
People |
ORCID iD |
Daniel Brett (Principal Investigator) |
Publications
Maher RC
(2016)
Reduction Dynamics of Doped Ceria, Nickel Oxide, and Cermet Composites Probed Using In Situ Raman Spectroscopy.
in Advanced science (Weinheim, Baden-Wurttemberg, Germany)
Manage M
(2014)
A modelling approach to assessing the feasibility of the integration of power stations with steam electrolysers
in Chemical Engineering Research and Design
Toleuova A
(2016)
Mechanistic Studies of Liquid Metal Anode SOFCs II: Development of a Coulometric Titration Technique to Aid Reactor Design
in Chemical Engineering Science
Tjaden B
(2016)
On the origin and application of the Bruggeman correlation for analysing transport phenomena in electrochemical systems
in Current Opinion in Chemical Engineering
Robinson J
(2015)
Detection of Internal Defects in Lithium-Ion Batteries Using Lock-in Thermography
in ECS Electrochemistry Letters
Toleuova A
(2013)
A Rotating Electrolyte Disc (RED) for Operation in Liquid Metal Anode SOFCs
in ECS Transactions
Toleuova A
(2015)
Mechanistic Considerations of Liquid Metal Anode SOFCs Fueled with Hydrogen
in ECS Transactions
Engebretsen E
(2017)
Electrochemical pressure impedance spectroscopy applied to the study of polymer electrolyte fuel cells
in Electrochemistry Communications
Zhang D
(2013)
Fair electricity transfer price and unit capacity selection for microgrids
in Energy Economics
Obeisun O
(2017)
Ex-situ characterisation of water droplet dynamics on the surface of a fuel cell gas diffusion layer through wettability analysis and thermal characterisation
in International Journal of Hydrogen Energy
Obeisun O
(2014)
Development of open-cathode polymer electrolyte fuel cells using printed circuit board flow-field plates: Flow geometry characterisation
in International Journal of Hydrogen Energy
Bharath V
(2017)
Effect of humidity on the interaction of CO2 with alkaline anion exchange membranes probed using the quartz crystal microbalance
in International Journal of Hydrogen Energy
Bharath V
(2017)
Alkaline anion exchange membrane degradation as a function of humidity measured using the quartz crystal microbalance
in International Journal of Hydrogen Energy
Meyer Q
(2015)
System-level electro-thermal optimisation of air-cooled open-cathode polymer electrolyte fuel cells: Air blower parasitic load and schemes for dynamic operation
in International Journal of Hydrogen Energy
Noorkami M
(2014)
Effect of temperature uncertainty on polymer electrolyte fuel cell performance
in International Journal of Hydrogen Energy
Obeisun O
(2015)
Study of water accumulation dynamics in the channels of an open-cathode fuel cell through electro-thermal characterisation and droplet visualisation
in International Journal of Hydrogen Energy
Robinson J
(2016)
Thermal Imaging of Electrochemical Power Systems: A Review
in Journal of Imaging
Bharath V
(2016)
Measurement of water uptake in thin-film Nafion and anion alkaline exchange membranes using the quartz crystal microbalance
in Journal of Membrane Science
Bailey JJ
(2017)
Laser-preparation of geometrically optimised samples for X-ray nano-CT.
in Journal of microscopy
Maskell W
(2013)
Improvements to Zirconia Thick-Film Oxygen Sensors
in Journal of Physics: Conference Series
Meyer Q
(2014)
Dead-ended anode polymer electrolyte fuel cell stack operation investigated using electrochemical impedance spectroscopy, off-gas analysis and thermal imaging
in Journal of Power Sources
Robinson J
(2015)
Investigating the effect of thermal gradients on stress in solid oxide fuel cell anodes using combined synchrotron radiation and thermal imaging
in Journal of Power Sources
Meyer Q
(2015)
Optimisation of air cooled, open-cathode fuel cells: Current of lowest resistance and electro-thermal performance mapping
in Journal of Power Sources
Engebretsen E
(2016)
Electro-thermal impedance spectroscopy applied to an open-cathode polymer electrolyte fuel cell
in Journal of Power Sources
Description | So far this project has allowed us to develop correlative metrology techniques for the analysis of solid oxide fuel cells. This includes the ability to examine the temperature distribution in electrode materials and relate this to strain within the structure. We have also developed an in-situ SOFC cell capable of viewing, with an infrared thermal camera, the temperature distribution within an operational system. We will use these results to inform model development in the next phase of work. |
Exploitation Route | Our thermal imaging technique will provide unparalleled insight into the internal workings of SOFCs and allow advanced models describing electro-thermal operation to be developed and validated, so leading to the development of commercial SOFC technology. |
Sectors | Energy |
URL | http://www.ucl.ac.uk/electrochemical-innovation-lab |
Description | Findings of the operation of solid oxide fuel cell materials under thermal gradients are being communicated to out industrial collaborator, Ceres Power, and we have recently applied for a Supergen H2FC Early Career Researcher award with Ceres to apply thermal imaging alongside X-ray computed tomography to help understand how electrodes function in devices. |
First Year Of Impact | 2014 |
Sector | Energy,Environment |
Impact Types | Societal,Economic |